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arXiv:2111.10129 · Physical Review Letters

Quantum Non-Gaussianity of Multiphonon States of a Single Atom

Lukáš Podhora, Lukáš Lachman, T. Pham, Adam Lešundák, Ondřej Čı́p, L. Slodička, Radim Filip

Published Jun 28, 2022• 28 citations
arXivHTMLPDF

Abstract

Quantum non-Gaussian mechanical states are already required in a range of applications. The discrete building blocks of such states are the energy eigenstates-Fock states. Despite progress in their preparation, the remaining imperfections can still invisibly cause loss of the aspects critical for their applications. We derive and apply the most challenging hierarchy of quantum non-Gaussian criteria on the characterization of single trapped-ion oscillator mechanical Fock states with up to 10 phonons. We analyze the depth of these quantum non-Gaussian features under intrinsic mechanical heating and predict their requirement for reaching quantum advantage in the sensing of a mechanical force.

DOI
10.1103/physrevlett.129.013602

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Quantum non-Gaussian mechanical states are already required in a range of applications. The discrete building blocks of such states are the energy eigenstates-Fock states. Despite progress in their preparation, the remaining imperfections can still invisibly cause loss of the aspects critical for their applications. We derive and apply the most challenging hierarchy of quantum non-Gaussian criteria on the characterization of single trapped-ion oscillator mechanical Fock states with up to 10 phonons. We analyze the depth of these quantum non-Gaussian features under intrinsic mechanical heating and predict their requirement for reaching quantum advantage in the sensing of a mechanical force.
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Quantum coherence between energy eigenstates of harmonic oscillators is essential for quantum physics. Even the most elementary binary superpositions of the ground and the higher eigenstate are highly required for quantum sensing, thermodynamics, and computing. We derive upper bounds for quantum coherences achieved by classical and Gaussian states and operations and, subsequently, obtain a hierarchy of the thresholds for the off-diagonal elements necessary to reach genuine quantum non-Gaussian coherences. The presented analysis demonstrates that certification based solely on estimation of coherences can cover the quantum non-Gaussian states, which are undetectable by the criteria based solely on the estimation of the corresponding state populations. We experimentally demonstrate the unambiguous observation of quantum non-Gaussian coherences in mechanical vibrations of a single calcium ion up to the superposition of zero and six phonons. The analysis of the robustness with respect to pure dephasing in a motional Ramsey experiment demonstrates the feasibility of their storage for up to more than 20 ms for superpositions with a large energy difference of participating number states. The presented observations prove that atomic oscillations go deeply into a diverse area of discrete quantum non-Gaussian coherent phenomena critical for their applications.
Massive mechanical oscillators couple directly to forces, accelerations and gravity, making them attractive probes of new physics and of quantum mechanics at macroscopic scales. Pushing sensitivities beyond the standard quantum limit for signals of unknown phase requires non-Gaussian quantum states, whose metrological advantage has so far been confined to lighter systems such as trapped ions. Here we operate a microgram-scale acoustic mode of a high-overtone bulk acoustic wave resonator as a phase-insensitive quantum-enhanced sensor. A transmon qubit prepares the mode in Fock states of up to seven phonons by optimal control, and resolves its phonon-number distribution after interaction with a weak resonant signal. Bayesian analysis yields a Fisher information five times the vacuum value, a 7.0 dB gain in signal-amplitude sensitivity over any classical probe state, irrespective of its energy, currently limited by state preparation infidelities. We then train a neural network on the measured sensor response to perform Bayesian estimation without any analytical model of the system, showing the same sensitivity gain with half the systematic bias. Our results establish acoustic resonators prepared in non-Gaussian states as quantum-enhanced probes for high-frequency gravitational waves, dark matter and wave-function collapse.
Fock states of the quantum harmonic oscillator are fundamental to quantum sensing and information processing, serving as key resources for exploiting bosonic degrees of freedom. Here, we prepare high Fock states in a high-overtone bulk acoustic wave resonator by coupling it to a superconducting qubit and applying microwave pulses designed using quantum optimal control. We characterize the experimentally realized states by employing a criterion for genuine quantum non-Gaussianity (QNG) designed to reveal multiphonon contributions. Although energy relaxation and decoherence limit the achievable fidelities, we demonstrate genuine QNG features compatible with a Fock state |6⟩, confirming that the prepared states cannot be generated through Gaussian operations on states with up to Fock state |5⟩ contributions. We further investigate the robustness of these QNG features to losses and their utility in sensing displacement amplitudes. In particular, we introduce a hierarchy based on the quantum Fisher information and show that, despite decoherence and measurement imperfections, the prepared states achieve a displacement sensitivity surpassing that of an ideal Fock state |3⟩. Our results have immediate applications in quantum sensing and simulations with high-overtone bulk acoustic wave resonator devices.
Abstract Quantum non-Gaussian states of phononic systems coupled to light are essential for fundamental studies of single-phonon mechanics and direct applications in quantum technology. Although nonclassical mechanical states have already been demonstrated, the more challenging quantum non-Gaussianity of such states remains limited. Using photon counting detection, we propose the quantum non-Gaussian generation of few-phonon states of low-temperature vibrating superfluid Helium. We predict the quantum non-Gaussian depth of such phononic states and investigate their robustness under relevant mechanical heating. As the quality of such phononic states is very high, we confirm a single-phonon bunching capability to further classify such states for future mechanical experiments. Moreover, we predict increasing capability for force sensing and thermometry for increasing heralded phonon numbers.