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arXiv:2412.20971 · Physical Review Letters

Genuine Quantum Non-Gaussianity and Metrological Sensitivity of Fock States Prepared in a Mechanical Resonator

Q. Rumman Rahman, Igor Kladarić, Max-Emanuel Kern, Lukáš Lachman, Yiwen Chu, Radim Filip, Matteo Fadel

Published May 5, 2025• 22 citations
arXivHTMLPDF

Abstract

Fock states of the quantum harmonic oscillator are fundamental to quantum sensing and information processing, serving as key resources for exploiting bosonic degrees of freedom. Here, we prepare high Fock states in a high-overtone bulk acoustic wave resonator by coupling it to a superconducting qubit and applying microwave pulses designed using quantum optimal control. We characterize the experimentally realized states by employing a criterion for genuine quantum non-Gaussianity (QNG) designed to reveal multiphonon contributions. Although energy relaxation and decoherence limit the achievable fidelities, we demonstrate genuine QNG features compatible with a Fock state |6⟩, confirming that the prepared states cannot be generated through Gaussian operations on states with up to Fock state |5⟩ contributions. We further investigate the robustness of these QNG features to losses and their utility in sensing displacement amplitudes. In particular, we introduce a hierarchy based on the quantum Fisher information and show that, despite decoherence and measurement imperfections, the prepared states achieve a displacement sensitivity surpassing that of an ideal Fock state |3⟩. Our results have immediate applications in quantum sensing and simulations with high-overtone bulk acoustic wave resonator devices.

DOI
10.1103/physrevlett.134.180801

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Fock states of the quantum harmonic oscillator are fundamental to quantum sensing and information processing, serving as key resources for exploiting bosonic degrees of freedom. Here, we prepare high Fock states in a high-overtone bulk acoustic wave resonator by coupling it to a superconducting qubit and applying microwave pulses designed using quantum optimal control. We characterize the experimentally realized states by employing a criterion for genuine quantum non-Gaussianity (QNG) designed to reveal multiphonon contributions. Although energy relaxation and decoherence limit the achievable fidelities, we demonstrate genuine QNG features compatible with a Fock state |6⟩, confirming that the prepared states cannot be generated through Gaussian operations on states with up to Fock state |5⟩ contributions. We further investigate the robustness of these QNG features to losses and their utility in sensing displacement amplitudes. In particular, we introduce a hierarchy based on the quantum Fisher information and show that, despite decoherence and measurement imperfections, the prepared states achieve a displacement sensitivity surpassing that of an ideal Fock state |3⟩. Our results have immediate applications in quantum sensing and simulations with high-overtone bulk acoustic wave resonator devices.
Massive mechanical oscillators couple directly to forces, accelerations and gravity, making them attractive probes of new physics and of quantum mechanics at macroscopic scales. Pushing sensitivities beyond the standard quantum limit for signals of unknown phase requires non-Gaussian quantum states, whose metrological advantage has so far been confined to lighter systems such as trapped ions. Here we operate a microgram-scale acoustic mode of a high-overtone bulk acoustic wave resonator as a phase-insensitive quantum-enhanced sensor. A transmon qubit prepares the mode in Fock states of up to seven phonons by optimal control, and resolves its phonon-number distribution after interaction with a weak resonant signal. Bayesian analysis yields a Fisher information five times the vacuum value, a 7.0 dB gain in signal-amplitude sensitivity over any classical probe state, irrespective of its energy, currently limited by state preparation infidelities. We then train a neural network on the measured sensor response to perform Bayesian estimation without any analytical model of the system, showing the same sensitivity gain with half the systematic bias. Our results establish acoustic resonators prepared in non-Gaussian states as quantum-enhanced probes for high-frequency gravitational waves, dark matter and wave-function collapse.
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The development of quantum acoustics has enabled the cooling of mechanical objects to their quantum ground state, generation of mechanical Fock-states, and Schrödinger cat states. Such demonstrations have made mechanical resonators attractive candidates for quantum information processing, metrology, and macroscopic tests of quantum mechanics. However, generating large-amplitude phonon states in quantum acoustic systems has been elusive. In this work, a single superconducting qubit coupled to a high-overtone bulk acoustic resonator is used to generate a large phonon population in an acoustic mode of a high-overtone resonator. We observe extended ringdowns of the qubit, confirming the generation of a large amplitude phonon state, and also observe an upper threshold behavior, a consequence of phonon quenching predicted by our model. This work provides a key tool for generating arbitrary phonon states in circuit quantum acoustodynamics, which is important for fundamental and quantum information applications.
Quantum non-Gaussian mechanical states are already required in a range of applications. The discrete building blocks of such states are the energy eigenstates-Fock states. Despite progress in their preparation, the remaining imperfections can still invisibly cause loss of the aspects critical for their applications. We derive and apply the most challenging hierarchy of quantum non-Gaussian criteria on the characterization of single trapped-ion oscillator mechanical Fock states with up to 10 phonons. We analyze the depth of these quantum non-Gaussian features under intrinsic mechanical heating and predict their requirement for reaching quantum advantage in the sensing of a mechanical force.
As superconducting quantum computing devices grow more and more powerful [1–3], the quest to connect them over large-scale distances [4] becomes increasingly relevant. Microwave-to-optical transducers offer a pathway for such connections via a low-loss and thermal noise-free optical fiber network. However, achieving simultaneously high efficiency and low added noise is currently limited by a trade-off between both quantities due to pump absorption heating [5–9]. High-overtone bulk acoustic-wave resonators (HBARs) promise a solution to this problem due to their crystalline material and low surface-to-bulk ratio. In this thesis, we introduce an HBAR-based microwave-to-optical transducer to achieve quantum state transfer. As a first milestone, we build a Brillouin-optomechanical cavity that self-aligns when cooled down and is relatively insensitive to vibrations, which allows optomechanical coupling in an environment that is compatible with superconducting circuits. We measure the phonon mode occupation of the HBAR to be below 0.5, demonstrating the heaviest mechanical object measured in the quantum ground state to date. In addition, we show that the mode occupations are insensitive to laser pump power, indicating negligible absorption heating and confirming the unique advantage of this system. We then build a transducer device which combines Brillouin-optomechanical coupling and piezo-electromechanical coupling to a superconducting qubit in one geometry. We can align the optical cavity mode to pass through the ring-shaped antenna of the superconducting qubit without affecting the optical finesse. This allows us to measure optomechanical coupling in this device as a next milestone towards high-efficiency, low noise microwave-to-optical transduction.
Quantum metrology enables sensitivity to approach the limits set by fundamental physical laws. Even a single continuous mode offers enhanced precision, with the improvement scaling with its occupation number. Due to their high information capacity, continuous modes allow for the engineering of quantum non-Gaussian states, which not only improve metrological performance but can also be tailored to specific experimental platforms and conditions. Recent advancements in control over continuous platforms operating in the quantum regime have renewed interest in sensing weak forces, also coupling to massive macroscopic objects. In this work, we investigate a force-sensing scheme where a physical process completely randomizes the direction of the induced phase-space displacement, and the unknown force strength is inferred through excitation-number-resolving measurements. We find that N-spaced states, where only every N^{th} Fock state occupation is nonzero, approach the achievable sensing bound. Additionally, non-Gaussian states are shown to be more resilient against decoherence than their Gaussian counterparts with the same occupation number. While Fock states typically offer the best protection against decoherence, we uncover a transition in the metrological landscape-revealed through a tailored decoherence-aware Fisher-information-based reward functional-where experimental constraints favor a family of number-squeezed Schrödinger cat states. Specifically, by implementing quantum optimal control in a minimal spin-boson system, we identify these states as maximizing force sensitivity under lossy dynamics and finite system controllability. Our results provide a pathway for enhancing force sensing in a variety of continuous quantum systems, ranging from massive systems like mechanical oscillators to massless systems such as quantum light and microwave resonators.