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arXiv:2411.08236 · Physical Review Letters

Enhancement of Rydberg Blockade via Microwave Dressing

Deniz Kurdak, Patrick Banner, Yaxin Li, Sean R. Muleady, Alexey Vyacheslavovich Gorshkov, S. L. Rolston, J. V. Porto

Published Mar 27, 2025• 12 citations
arXivHTMLPDF

Abstract

Experimental control over the strength and angular dependence of interactions between atoms is a key capability for advancing quantum technologies. Here, we use microwave dressing to manipulate and enhance Rydberg-Rydberg interactions in an atomic ensemble. By varying the cloud length relative to the blockade radius and measuring the statistics of the light retrieved from the ensemble, we demonstrate a clear enhancement of the interaction strength due to microwave dressing. These results are successfully captured by a theoretical model that accounts for the excitation dynamics, atomic density distribution, and phase-matched retrieval efficiency. Our approach offers a versatile platform for further engineering interactions by exploiting additional features of the microwave fields, such as polarization and detuning, opening pathways for new quantum control strategies.

DOI
10.1103/physrevlett.134.123404

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Experimental control over the strength and angular dependence of interactions between atoms is a key capability for advancing quantum technologies. Here, we use microwave dressing to manipulate and enhance Rydberg-Rydberg interactions in an atomic ensemble. By varying the cloud length relative to the blockade radius and measuring the statistics of the light retrieved from the ensemble, we demonstrate a clear enhancement of the interaction strength due to microwave dressing. These results are successfully captured by a theoretical model that accounts for the excitation dynamics, atomic density distribution, and phase-matched retrieval efficiency. Our approach offers a versatile platform for further engineering interactions by exploiting additional features of the microwave fields, such as polarization and detuning, opening pathways for new quantum control strategies.
Advances in the coherent control of Rydberg atoms have led to an explosion in their use in a wide range of topics, including quantum computation, simulation, sensing, and networking. More specifically, Rydberg-coupled ensembles of atoms interfaced with a single mode of light have enabled studies of fundamental light-matter interactions at the single-photon level and have emerged as a promising platform to realize scalable quantum networking nodes. In the first part of this thesis, we utilize Rydberg blockade to generate large ensembles that host a single Rydberg excitation and use the collective state as a resource to efficiently generate single photons. We further investigate the shelving of the collective Rydberg excitations to the ground-state manifold, where we observe an order of magnitude increase in the coherence time of the excitation. In the latter half of the thesis, we use near-resonant microwave fields to generate microwave-dressed Rydberg states, where we utilize the degrees of freedom of the microwave field to tune the strength, form, and angular dependence of the dipole-dipole interactions. To this end, we develop a robust and highly tunable microwave polarization control system. We use a set of in-vacuum electrodes as microwave antennas. We measure the microwave polarizations produced by each source at the positions of the atoms using a Rydberg EIT-based polarimetry technique. By characterizing the three imperfect sources, we find the control settings necessary to produce \sigma_-, \pi, and \sigma_+ polarized microwaves with >99 % fidelity. We extend our purification techniques to frequencies away from Rydberg resonances by utilizing an auxiliary microwave field, generating two-photon microwave resonances. The high-fidelity microwave polarizations are used to resonantly admix opposite-parity Rydberg states, generating dressed states with dipole-dipole interactions that are longer range and stronger than the bare van der Waals interactions. To characterize the strength of the interactions, we measure the photon-number statistics of the light generated by the ensemble of atoms. By varying the cloud length relative to the blockade radii, we demonstrate a clear enhancement of the interaction strength due to microwave dressing. Our platform enables further engineering of interactions by exploiting the polarization and frequency degrees of freedom of the microwave fields, opening pathways for new quantum control strategies in many different experimental platforms.
Control of the polarization of microwave fields is a key experimental capability for a number of atomic physics platforms. However, producing high-fidelity microwaves requires a well-controlled microwave environment, where reflections that distort the polarization must be avoided or well characterized, a constraint that often conflicts with other experimental design considerations. Here we demonstrate a microwave control system capable of producing high-fidelity microwave polarizations in a Rydberg-ensemble experiment. We use three in-vacuum DC electrodes, repurposed as microwave antennae, to produce imperfect and initially unknown polarizations. Each source is driven with independent phase and amplitude control to generate the desired microwave fields. We probe the fields produced at the position of the atoms using Rydberg-EIT spectroscopy of the microwave-induced avoided crossings. We produce σ−σ_-σ−​, πππ, and σ+σ_+σ+​ polarized microwaves with > 99 % fidelity and generate their combinations. We extend our purification techniques to frequencies away from Rydberg resonances by utilizing an auxiliary microwave field, generating two-photon microwave resonances. The techniques developed here will facilitate the engineering of dipolar interactions in atomic and molecular physics experiments.
We report for the first time the theoretical and experimental research on Rydberg electromagnetically induced transparency and second-order fluorescence dressing evolution by Rabi frequency control in thermal atomic vapors, in which the controlled results are well explained by the dressing effect and the Rydberg excitation blockade. Based on the certification of the Rydberg excitation blockade fraction through the dependence on principle quantum number n, we obtain dressing evolution curves, consisting of single-dressing and double-dressing in local and nonlocal blockade samples by scanning the probe and dressing fields. In addition, the competition between the Rydberg dressing second-order fluorescence and fourth-order fluorescence is first investigated. A corresponding theory is presented, which is consistent with the experimental results. Such blockade evolution regularity has potential applications in quantum control, and the Rydberg dressing may be useful for investigating multiple-body interactions, as well as for inducing short range interactions in Bose-Einstein condensates.
We demonstrate a coherent microwave manipulation of a single optical photon based on a single Rydberg excitation in an atomic ensemble. Due to the strong nonlinearities in a Rydberg blockade region, a single photon can be stored in the formation of Rydberg polariton using electromagnetically induced transparency (EIT). The manipulation of the stored single photon is performed by applying a microwave field that resonantly couples the nS 1/2 and nP 3/2 , while the coherent readout is performed by mapping the excitation into a single photon. We achieve a single photon source with g (2) (0) = 0.29 ± 0.08 at 80 S 1/2 without applying microwave fields. By implementing the microwave field during the storage time and retrieval process, we show the Rabi oscillation and modulation of stored photons that can be controlled to retrieve early or late. Rapid modulation frequencies up to 50 MHz can be obtained. Our experimental observations can be well explained via numerical simulations based on an improved superatom model accounting for the dipole-dipole interactions in a Rydberg EIT medium. Our work provides a way to manipulate the stored photons by employing the microwave field, which is significant for developing quantum technologies.
The power broadening of a coupling laser can be converted into two-photon detuning by electromagnetically induced transparency (EIT), resulting in a residual Doppler effect. The residual Doppler effect in a ladder-type EIT in a room-temperature atom ensemble is further amplified through a wavelength mismatch effect between the probe and coupling laser beams, which reduces the atomic coupling of light or microwaves. We measured the Rydberg spectra of the electric dipole (E1) and electric quadrupole (E2) microwave transitions, demonstrating that the reduction in the Rydberg EIT signal can be recovered through far-off-resonance E2 microwave transition dressing and achieving an 8-dB enhancement in the Rydberg EIT signal. The frequency-dependent dressing of the E2 transition enables the shift of the dressed Rydberg states to be tuned, thereby providing a scalable approach to optimize the interaction between the Rydberg state and microwave field.
We investigate the interaction between Rydberg atoms, whose electronic states are dressed by multiple microwave fields. Numerical calculations are used for an exact description of the microwave induced interactions, and employed to benchmark a perturbative treatment that yields simple insights into the involved mechanisms. Based on this theory, we demonstrate that microwave dressing provides a powerful approach to control dipolar as well as van der Waals interactions and even permits us to turn them off entirely. In addition, the proposed scheme also opens up possibilities for engineering dominant three-body interactions.