Non-reciprocal propagation of energy and information is fundamental to a wide range of quantum technology applications. In this work, we explore the quantum many-body dynamics of a qubit ensemble coupled to a shared bath that mediates coherent and dissipative inter-qubit interactions with both symmetric and anti-symmetric components. We find that the interplay between anti-symmetric (symmetric) coherent and symmetric (anti-symmetric) dissipative interactions results in non-reciprocal couplings, which, in turn, generate a spatially asymmetric emission pattern. We demonstrate that this pattern arises from non-reciprocal interactions coupling different quantum many-body states within a specific excitation manifold. Focusing on solid-state baths, we show that their lack of time-reversal and inversion symmetry is a key ingredient for generating non-reciprocal dynamics in the qubit ensemble. With the plethora of quantum materials that exhibit this symmetry breaking at equilibrium, our approach paves the way for realizing cooperative non-reciprocal transport in qubit ensembles without requiring time-modulated external drives or complex engineering. Using an ensemble of nitrogen-vacancy (NV) centers coupled to a generic non-centrosymmetric ferromagnetic bath as a concrete example, we demonstrate that our predictions can be tested in near-future experiments. As the spatial asymmetry in the relaxation dynamics of the qubit ensemble is a direct probe of symmetry breaking in the solid-state bath, our work also opens the door to developing model-agnostic quantum sensing schemes capable of detecting bath properties invisible to current state-of-the-art protocols, which operate solid-state defects as single-qubit sensors.
Non-reciprocal propagation of energy and information is fundamental to a wide range of quantum technology applications. In this work, we explore the quantum many-body dynamics of a qubit ensemble coupled to a shared bath that mediates coherent and dissipative inter-qubit interactions with both symmetric and anti-symmetric components. We find that the interplay between anti-symmetric (symmetric) coherent and symmetric (anti-symmetric) dissipative interactions results in non-reciprocal couplings, which, in turn, generate a spatially asymmetric emission pattern. We demonstrate that this pattern arises from non-reciprocal interactions coupling different quantum many-body states within a specific excitation manifold. Focusing on solid-state baths, we show that their lack of time-reversal and inversion symmetry is a key ingredient for generating non-reciprocal dynamics in the qubit ensemble. With the plethora of quantum materials that exhibit this symmetry breaking at equilibrium, our approach paves the way for realizing cooperative non-reciprocal transport in qubit ensembles without requiring time-modulated external drives or complex engineering. Using an ensemble of nitrogen-vacancy (NV) centers coupled to a generic non-centrosymmetric ferromagnetic bath as a concrete example, we demonstrate that our predictions can be tested in near-future experiments. As the spatial asymmetry in the relaxation dynamics of the qubit ensemble is a direct probe of symmetry breaking in the solid-state bath, our work also opens the door to developing model-agnostic quantum sensing schemes capable of detecting bath properties invisible to current state-of-the-art protocols, which operate solid-state defects as single-qubit sensors.
Advancing quantum sensing tools for investigating atomic and nanoscale systems is crucial for the progress of quantum technologies. While many protocols use quantum probes to extract information from stationary or weakly coupled environments, challenges intensify at the atomic scale and the nanoscale, where the environment is inherently out of equilibrium and/or strongly coupled with the sensor. In this work, we demonstrate that time-reversal symmetry in the control dynamics of a quantum sensor is broken when the qubit sensor interacts with environments that are out of equilibrium (with nonstationary fluctuations), contain quantum non-Gaussian correlations, or exhibit intrinsic time-reversal symmetry breaking. Leveraging this phenomenon, we introduce a quantum sensing paradigm based on time-asymmetric dynamical control sequences, enabling the probing of the distance of an environment from equilibrium, its time-reversal symmetry-breaking behavior, or its quantum non-Gaussian nature. Additionally, we propose sensing strategies to distinguish between these different sources of symmetry breaking. We validate our approach through proof-of-principle experimental quantum simulations using solid-state nuclear magnetic resonance, where we drive the environment of a qubit sensor out of equilibrium and use our protocol to quantify the nonstationary characteristics of the generated states. Our findings highlight the potential of this framework for quantifying nonstationary behavior, designing tailored pump-probe experiments (including measurements of quantum information scrambling), and detecting quantum states that exhibit time-reversal symmetry breaking, time-crystal structures, or quantum non-Gaussian fluctuations. Overall, this work constitutes a step forward in designing quantum devices for atomic scale and nanoscale sensing, broadening their applicability to complex and dynamic quantum environments.
The authors develop here a theoretical framework for the quantum many-body dynamics of a qubit array interacting via the electromagnetic noise of a shared solid-state bath. Applied to an NV-center ensemble coupled to a YIG film, this study demonstrates that robust many-body effects, such as superradiance and subradiance, are within experimental reach, opening new opportunities for engineering collective quantum phenomena in solid-state platforms and advancing multi-qubit quantum sensing approaches.
Enhanced interaction between two two-level emitters (e.g., atoms) by nonreciprocal photonic media can be of benefit to broad areas, from quantum information science to biological detection. Here we provide a detailed analysis on why nonreciprocal photon-mediated interaction enhances interatomic excitation transport efficiency. We investigate a system consisting of two two-level emitters embedded in a generic photonic environment. By comparing symmetric and asymmetric photon exchange, we analytically show that breaking electromagnetic reciprocity makes it possible for the cooperative decay rate to exceed the spontaneous decay rate, even in a translation-invariant homogeneous system. This means that the excitation of an emitter must decay mostly into the other emitter rather than leaking and dissipating into the reservoir photonic modes. We also provide an example where a chain of two-level emitters dominantly interacts via the reciprocal modes of a plasmonic waveguide. We then show that breaking reciprocity in such a system via driving a dc current through the plasmonic material can drastically increase the probability of photon emission from one emitter to another, leading to an order-of-magnitude enhancement in quantum energy-transport efficiency.
Electronic spins of nitrogen vacancy (NV) centers in diamond constitute a promising system for micro- and nano-scale magnetic sensing, due to their operation under ambient conditions, ease of placement in close proximity to sensing targets, and biological compatibility. At high densities, the electronic spins interact through dipolar coupling, which typically limits but can also potentially enhance sensing performance. Here we report the experimental demonstration of many-body signal amplification in a solid-state, room temperature quantum sensor. Our approach utilizes time-reversed two-axis-twisting interactions, engineered through dynamical control of the quantization axis and Floquet engineering in a two-dimensional ensemble of NV centers. Strikingly, we observe that the optimal amplification occurs when the backward evolution time equals twice the forward evolution time, in sharp contrast to the conventional Loschmidt echo. These observations can be understood as resulting from an underlying time-reversed mirror symmetry of the microscopic dynamics, providing key insights into signal amplification and opening the door towards entanglement-enhanced practical quantum sensing.
Controlling the dynamics of targeted quantum correlations is a central goal across many disciplines of quantum science. For applications in nanoscale quantum sensing, nitrogen-vacancy (NV) centers in diamond have recently emerged as a leading platform due to their atom-like nature, exquisite magnetic sensitivity and well-developed coherent control techniques under ambient conditions. However, harnessing the entanglement structure required to improve this sensitivity beyond the standard quantum limit (SQL) from the native dipolar interactions between NV centers is challenging due to their strong positional disorder, three-dimensional geometry and low-fidelity readout. Coupled tightly to proof of principle experimental demonstrations, this thesis provides a theoretical blueprint to realize practical, entanglement-enhanced quantum sensing in the solid-state via far-from-equilibrium dynamics of dense ensembles of NV centers in diamond. Our most fundamental contribution is to identify a universal mechanism exploiting the thermalization of long-wavelength spin textures to generate scalable spin squeezing in the absence of finite temperature symmetry breaking. We further develop a novel sensing protocol based on asymmetric time-reversal capable of rapidly breaking the SQL without high-fidelity readout. Challenging long-standing beliefs in the field, these results open the door to a new era of entanglement-enhanced sensing under ambient conditions, with applications ranging from nanoscale imaging of biological structures to covariance magnetometry of exotic quantum materials.
The dispersive interaction between a qubit and a cavity is ubiquitous in circuit and cavity quantum electrodynamics. It describes the frequency shift of one quantum mode in response to excitations in the other and, in closed systems, is necessarily bidirectional, i.e., reciprocal. Here, we present an experimental study of a nonreciprocal dispersive-type interaction between a transmon qubit and a superconducting cavity, arising from a common coupling to dissipative intermediary modes with broken time reversal symmetry. We characterize the qubit-cavity dynamics, including asymmetric frequency pulls and photon shot noise dephasing, under varying degrees of nonreciprocity by tuning the magnetic field bias of a ferrite component in situ. We introduce a general master equation model for nonreciprocal interactions in the dispersive regime, providing a compact description of the observed qubit-cavity dynamics agnostic to the intermediary system. Our result provides an example of quantum nonreciprocal phenomena beyond the typical paradigms of non-Hermitian Hamiltonians and cascaded systems.