Enhanced interaction between two two-level emitters (e.g., atoms) by nonreciprocal photonic media can be of benefit to broad areas, from quantum information science to biological detection. Here we provide a detailed analysis on why nonreciprocal photon-mediated interaction enhances interatomic excitation transport efficiency. We investigate a system consisting of two two-level emitters embedded in a generic photonic environment. By comparing symmetric and asymmetric photon exchange, we analytically show that breaking electromagnetic reciprocity makes it possible for the cooperative decay rate to exceed the spontaneous decay rate, even in a translation-invariant homogeneous system. This means that the excitation of an emitter must decay mostly into the other emitter rather than leaking and dissipating into the reservoir photonic modes. We also provide an example where a chain of two-level emitters dominantly interacts via the reciprocal modes of a plasmonic waveguide. We then show that breaking reciprocity in such a system via driving a dc current through the plasmonic material can drastically increase the probability of photon emission from one emitter to another, leading to an order-of-magnitude enhancement in quantum energy-transport efficiency.
Enhanced interaction between two two-level emitters (e.g., atoms) by nonreciprocal photonic media can be of benefit to broad areas, from quantum information science to biological detection. Here we provide a detailed analysis on why nonreciprocal photon-mediated interaction enhances interatomic excitation transport efficiency. We investigate a system consisting of two two-level emitters embedded in a generic photonic environment. By comparing symmetric and asymmetric photon exchange, we analytically show that breaking electromagnetic reciprocity makes it possible for the cooperative decay rate to exceed the spontaneous decay rate, even in a translation-invariant homogeneous system. This means that the excitation of an emitter must decay mostly into the other emitter rather than leaking and dissipating into the reservoir photonic modes. We also provide an example where a chain of two-level emitters dominantly interacts via the reciprocal modes of a plasmonic waveguide. We then show that breaking reciprocity in such a system via driving a dc current through the plasmonic material can drastically increase the probability of photon emission from one emitter to another, leading to an order-of-magnitude enhancement in quantum energy-transport efficiency.
Photon-mediated interaction between quantum emitters in engineered photonic baths is an emerging area of quantum optics. At the same time, non-Hermitian (NH) physics is currently thriving, spurred by the exciting possibility to access new physics in systems ruled by non-trivial NH Hamiltonians—in particular, photonic lattices—which can challenge longstanding tenets such as the Bloch theory of bands. Here, we combine these two fields and study the exotic interaction between emitters mediated by the photonic modes of a lossy photonic lattice described by a NH Hamiltonian. We show in a paradigmatic case study that structured losses in the field can seed exotic emission properties. Photons can mediate dissipative, fully non-reciprocal interactions between emitters with range critically dependent on the loss rate. When this loss rate corresponds to a bare-lattice exceptional point, the effective couplings are exactly nearest neighbor, implementing a dissipative, fully non-reciprocal Hatano–Nelson model. Counterintuitively, this can occur irrespective of the lattice boundary conditions. Thus photons can mediate an effective emitter’s Hamiltonian which is translationally invariant despite the fact that the field is not. We interpret these effects in terms of metastable atom–photon dressed states, which can be exactly localized on only two lattice cells or extended across the entire lattice. These findings introduce a paradigm of light-mediated interactions with unprecedented features such as non-reciprocity, non-trivial dependence on field boundary conditions, and range tunability via a loss rate.
In recent years, the study of quantum electrodynamics (QED) in light-matter interactions has discovered various interesting phenomenons that orient many applications. However, due to the ambient entanglement among photons and atoms, few-particle dynamics remains challenging to analyze precisely and limits the progress in several fields. In few-particle systems, different number of atoms interacting with the light field generates drastically different results, even when there is only a single photon involved in the system. The interference between individual atom’s spontaneous emission wavefunctions can cooperatively alter the effective atom-light coupling strength. Depending on the spatial distance between individual of atoms and the involved cavities in the interaction progresses, the collective spontaneous emission rate can alter drastically from superradiance, where the emission rate is enhanced to a high value proportional to the atom number, to subradiance, where the excited atom ensemble stays in a dark state with the light trapped forever. Superradiance provides a promising mechanism to create an ultra-strong light-matter coupling environment, which is an important ingredient for the design of ultra-fast optical devices, frequency comb generation and quantum mirrors. The dark state of subradiance, on the other hand, is essential for the quantum memory implementation. Also, nontrivial phenomenons also occur when multiple photons interacting with a single atom simultaneously. When a finite number of photons incidents on an atom, their scattering through an atom is highly nonlinear, and one special eigenstate component of such nonlinear process, namely photonic bound states, exhibits many interesting properties in nonlinear quantum optical systems. The photons in such state are strongly bunched with each other, as if a virtual attractive force is in effect. Also, the frequency of photons are anti-correlated so that their total frequency remains a constant value, no matter how arbitrary the frequency of any individual is. Thesefeatures benefit certain nonlinear quantum processes for quantum computing and quantum imaging. Specially for two-photon excitation imaging, the same-parity two-level fluorophore molecules suffers from extremely low excitation efficiencies due to the far off-resonant intermediate states. However, by replacing the current commonly used ultrashort laser pulse illuminations with two photon bound state photon pairs, namely photonic dimers, the efficiency can be enhanced to orders of magnitude higher. Such exceptionally high excitation efficiency can potentially bring the current in vivo deep brain imaging depth from millimeter level to several centimeters. To obtain a stable source of such photonic dimers, it is found that a laser structure with gain medium of two-photon emission materials is capable of generating the coherent state of photonic dimer and can serve as a promising light source for nonlinear quantum optical devices.
We investigate entanglement mediated by DC current induced nonreciprocal graphene plasmon polaritons. Nonreciprocal systems are ideal for the enhancement, control, and preservation of entanglement due to the potential for unidirectional beam-like wave propagation, i.e., efficiently transporting photons from one emitter to another. Using a quantum master equation and three-dimensional Green's function analysis, we investigate a system consisting of two two-level emitters dominantly interacting via electric current induced nonreciprocal plasmonic modes of a graphene waveguide. We use concurrence as a measure of entanglement. We show that nonreciprocal graphene plasmon polaritons are a promising candidate to generate and mediate concurrence, where it is shown that there is good enhancement and control of entanglement over vacuum, which is beneficial for the broad applications of entanglement as a quantum resource. We believe our findings contribute to the development of quantum devices, enabling efficient and tunable entanglement between two-level systems, which is a central goal in quantum technologies.
Stimulated emission and absorption are two fundamental processes of light–matter interaction, and the coefficients of the two processes should be equal. However, we will describe a generic method to realize the significant difference between the stimulated emission and absorption coefficients of two nondegenerate energy levels, which we refer to as a nonreciprocal transition. As a simple implementation, a cyclic three-level atom system, comprising two nondegenerate energy levels and one auxiliary energy level, is employed to show a nonreciprocal transition via a combination of synthetic magnetism and reservoir engineering. Moreover, a single-photon nonreciprocal transporter is proposed using two one-dimensional semi-infinite coupled-resonator waveguides connected by an atom with nonreciprocal transition effect. Our work opens up a route to design atom-mediated nonreciprocal devices in a wide range of physical systems.
Quantum squeezing, a cornerstone of quantum optics and photonics, has played a key role in achieving ultra-precision sensing and realizing nonreciprocal engineering. However, the nonreciprocal multiquanta emission has remained largely unexplored by using directional quantum squeezing. Here, the one-way photon-photon bundle emission in a compound system consisted of two coupled optical resonators and a two-level atom is investigated. It is found that the directional quantum squeezing induces the asymmetric frequency detuning and photon hopping interaction between the two resonators, leading to the directional excitation of the two-photon super-Rabi oscillation. In particular, by harnessing intrinsic dissipation of the system, two types of two-photon bundle emission can be selectively induced for the probe field input from one direction while it is prohibited with the probe from the other direction. This finding bridges the broad fields ranging from nonreciprocal physics to quantum squeezing optics and multiquanta emission control through an all-optical approach, which can enable potential applications in chiral quantum emitters and backscattering-immune photonic communications.
We present results of our theoretical research on collective emission of photons (super- and subradiance) and photon propagation in photonic environments.Just like the single-atom emission, collective emission depends on the photonic environment. For quantum emitters in layered media, we study whether surface plasmons can enhance collective emission, especially for emitters at distances smaller than an optical wavelength.A common approximation in quantum optics is the rotating-wave approximation in the light-matter interaction. We show that in general multi-atom emission rates depend on the approximation, but exceptions exist. Interatomic interactions induced by the electromagnetic field are given by the classical Green tensor, but only when not making the rotating-wave approximation.As a final example of quantum electromagnetics, we describe photons propagating through a layered medium with alternating loss and gain, so-called loss-compensated media. There is no analogous compensation of the quantum noise associated with loss and gain media.