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arXiv:2208.10085 · Optics Express

Entanglement mediated by DC current induced nonreciprocal graphene plasmonics

Jay A. Berres, S. Ali Hassani Gangaraj, George W. Hanson

Published Dec 1, 2022• 3 citations
arXivHTMLPDF

Abstract

We investigate entanglement mediated by DC current induced nonreciprocal graphene plasmon polaritons. Nonreciprocal systems are ideal for the enhancement, control, and preservation of entanglement due to the potential for unidirectional beam-like wave propagation, i.e., efficiently transporting photons from one emitter to another. Using a quantum master equation and three-dimensional Green's function analysis, we investigate a system consisting of two two-level emitters dominantly interacting via electric current induced nonreciprocal plasmonic modes of a graphene waveguide. We use concurrence as a measure of entanglement. We show that nonreciprocal graphene plasmon polaritons are a promising candidate to generate and mediate concurrence, where it is shown that there is good enhancement and control of entanglement over vacuum, which is beneficial for the broad applications of entanglement as a quantum resource. We believe our findings contribute to the development of quantum devices, enabling efficient and tunable entanglement between two-level systems, which is a central goal in quantum technologies.

DOI
10.1364/oe.473847

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We investigate entanglement mediated by DC current induced nonreciprocal graphene plasmon polaritons. Nonreciprocal systems are ideal for the enhancement, control, and preservation of entanglement due to the potential for unidirectional beam-like wave propagation, i.e., efficiently transporting photons from one emitter to another. Using a quantum master equation and three-dimensional Green's function analysis, we investigate a system consisting of two two-level emitters dominantly interacting via electric current induced nonreciprocal plasmonic modes of a graphene waveguide. We use concurrence as a measure of entanglement. We show that nonreciprocal graphene plasmon polaritons are a promising candidate to generate and mediate concurrence, where it is shown that there is good enhancement and control of entanglement over vacuum, which is beneficial for the broad applications of entanglement as a quantum resource. We believe our findings contribute to the development of quantum devices, enabling efficient and tunable entanglement between two-level systems, which is a central goal in quantum technologies.
Enhanced interaction between two two-level emitters (e.g., atoms) by nonreciprocal photonic media can be of benefit to broad areas, from quantum information science to biological detection. Here we provide a detailed analysis on why nonreciprocal photon-mediated interaction enhances interatomic excitation transport efficiency. We investigate a system consisting of two two-level emitters embedded in a generic photonic environment. By comparing symmetric and asymmetric photon exchange, we analytically show that breaking electromagnetic reciprocity makes it possible for the cooperative decay rate to exceed the spontaneous decay rate, even in a translation-invariant homogeneous system. This means that the excitation of an emitter must decay mostly into the other emitter rather than leaking and dissipating into the reservoir photonic modes. We also provide an example where a chain of two-level emitters dominantly interacts via the reciprocal modes of a plasmonic waveguide. We then show that breaking reciprocity in such a system via driving a dc current through the plasmonic material can drastically increase the probability of photon emission from one emitter to another, leading to an order-of-magnitude enhancement in quantum energy-transport efficiency.
We propose a novel approach for microwave and optical fields entanglement using an electrical capacitor loaded with graphene plasmonic waveguide. In the proposed scheme, a quantum microwave signal of frequency ωmdrives the electrical capacitor, while an intensive optical field (optical pump) of frequency ω1is launched to the graphene waveguide as a surface plasmon polariton (i.e., SPP) mode. The two fields interact by the means of electrically modulating the graphene optical conductivity. It then follows that an upper and lower SPP sideband modes (of ω2= ω1+ ωmand ω3= ω1- ωmfrequencies, respectively) are generated. We show that the microwave signal and the lower sideband SPP mode are entangled, for a proper optical intensity. A quantum mechanics model is carried out to describe the fields evolution. Furthermore, novel iterative approach (based on combining the Duan criterion with the quantum regression theorem) is developed to assess the fields entanglement. Consequently, the entanglement of the two fields is evaluated versus several parameters including the waveguide length, the pump intensity, and the microwave frequency. We find that the two fields are entangled over a vast microwave frequency range. Moreover, our calculations show that a significant number of entangled photons are generated at the lower SPP sideband. The proposed scheme attains tunable mechanism for microwave-optical entanglement which paves the way for efficient quantum systems.
Electrically tunable graphene plasmons are anticipated to enable strong light-matter interactions with resonant quantum emitters. However, plasmon resonances in graphene are typically limited to infrared frequencies, below those of optical excitations in robust quantum light sources and many biologically interesting molecules. Here we propose to utilize near fields generated by the plasmon-assisted nonlinear optical response of nanostructured graphene to resonantly couple with proximal quantum emitters operating in the near infrared. We show that the nonlinear near field produced by a graphene nanodisk can strongly excite and coherently control quantum states in two- and three-level atomic systems when the third harmonic of its plasmon resonance is tuned to a particular electronic transition. In the present scheme, emitter and plasmon resonances are nondegenerate, circumventing strong enhancement of spontaneous emission. We envision potential applications for the proposed nonlinear plasmonic coupling scheme in sensing and temporal quantum control.
We investigate spontaneous and pumped entanglement of two level systems in the vicinity of a photonic topological insulator interface, which supports a nonreciprocal (unidirectional), scattering-immune and topologically-protected surface plasmon polariton in the bandgap of the bulk material [1]. To this end, we derive a master equation for qubit interactions in a general three-dimensional, nonreciprocal, inhomogeneous and lossy environment. The environment is represented exactly, via the photonic Green function. The resulting entanglement is shown to be extremely robust to defects occurring in the material system, such that strong entanglement is maintained even if the interface exhibits electrically-large and geometrically sharp discontinuities. Alternatively, depending on the initial excitation state, using a non-reciprocal environment allows two qubits to remain unentangled even for very close spacing. The topological nature of the material is manifest in the insensitivity of the entanglement to variations in the material parameters that preserve the gap Chern number. Our formulation and results should be useful for both fundamental investigations of quantum dynamics in nonreciprocal environments, and technological applications related to entanglement in two-level systems.
In this paper, we review the theory of open quantum systems and macroscopic quantum electrodynamics, providing a self-contained account of many aspects of these two theories. The former is presented in the context of a qubit coupled to a electromagnetic thermal bath, the latter is presented in the context of a quantization scheme for surface-plasmon polaritons (SPPs) in graphene based on Langevin noise currents. This includes a calculation of the dyadic Green’s function (in the electrostatic limit) for a Graphene sheet between two semi-infinite linear dielectric media, and its subsequent application to the construction of SPP creation and annihilation operators. We then bring the two fields together and discuss the entanglement of two qubits in the vicinity of a graphene sheet which supports SPPs. The two qubits communicate with each other via the emission and absorption of SPPs. We find that a Schrödinger cat state involving the two qubits can be partially protected from decoherence by taking advantage of the dissipative dynamics in graphene. A comparison is also drawn between the dynamics at zero temperature, obtained via Schrödinger’s equation, and at finite temperature, obtained using the Lindblad equation.
We investigate spontaneous entanglement of two qubits mediated by nonreciprocal surface plasmon polaritons (SPPs) in a Weyl semimetal. In the absence of external magnetic fields, the topology of the Weyl semimetal even gives rise to nonreciprocal SPPs that are topologically protected and reside inside the photonic gap. We utilize this nonreciprocal SPP as a mediator of entanglement of two spatially separated qubits. Our two main findings are (1) the nonreciprocal SPP gives better quantum entanglement than the reciprocal one, and (2) the entanglement achieved in the Weyl semimetal is sufficiently long lived compared to the entanglement using SPPs in conventional metals.