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arXiv:2410.07805 · Physical Review Letters

Experimental Realization of Self-Contained Quantum Refrigeration

Keyi Huang, Xi Cheng, Xinyue Long, Hongfeng Liu, Yu-ang Fan, Xiangyu Wang, Yuxuan Zheng, Yufang Feng, Xinfang Nie, Dawei Lu

Published May 23, 2024• 16 citations
arXivHTMLPDF

Abstract

A fundamental challenge in quantum thermodynamics is the exploration of inherent dimensional constraints in thermodynamic machines. In the context of two-level systems, the most compact refrigerator necessitates the involvement of three entities, operating under self-contained conditions that preclude the use of external work sources. Here, we build such a smallest refrigerator using a nuclear spin system, where three distinct two-level carbon-13 nuclei in the same molecule are involved to facilitate the refrigeration process. The self-contained feature enables it to operate without relying on net external work, and the unique mechanism sets this refrigerator apart from its classical counterparts. We evaluate its performance under varying conditions and systematically scrutinize the cooling constraints across a spectrum of scenarios, which sheds light on the interplay between quantum information and thermodynamics.

DOI
10.1103/physrevlett.132.210403

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A fundamental challenge in quantum thermodynamics is the exploration of inherent dimensional constraints in thermodynamic machines. In the context of two-level systems, the most compact refrigerator necessitates the involvement of three entities, operating under self-contained conditions that preclude the use of external work sources. Here, we build such a smallest refrigerator using a nuclear spin system, where three distinct two-level carbon-13 nuclei in the same molecule are involved to facilitate the refrigeration process. The self-contained feature enables it to operate without relying on net external work, and the unique mechanism sets this refrigerator apart from its classical counterparts. We evaluate its performance under varying conditions and systematically scrutinize the cooling constraints across a spectrum of scenarios, which sheds light on the interplay between quantum information and thermodynamics.
We investigate the fundamental dimensional limits to thermodynamic machines. In particular, we show that it is possible to construct self-contained refrigerators (i.e., not requiring external sources of work) consisting of only a small number of qubits and/or qutrits. We present three different models, consisting of two qubits, a qubit and a qutrit with nearest-neighbor interactions, and a single qutrit, respectively. We then investigate the fundamental limits to their performance; in particular, we show that it is possible to cool towards absolute zero.
Understanding the thermodynamics of quantum systems is of fundamental importance, from both theoretical and experimental perspectives. A growing interest has been recently given to small self-contained quantum thermal machines, the functioning of which requires no external source of work or control, but only incoherent interactions with thermal baths. The simplicity of such machines makes them and ideal test-bed for exploring quantum thermodynamics. So far, however, the importance of quantum effects in these machines has remained elusive. Here we show that entanglement, the paradigmatical quantum effect, plays a fundamental role in small self-contained quantum refrigerators, as it can enhance cooling and energy transport -- except notably when the efficiency is close to the Carnot limit. Hence a truly quantum refrigerator can outperform a classical one. Furthermore, the amount of entanglement alone quantifies the enhancement in cooling. More generally, our work shows that entanglement opens new possibilities in thermodynamics.
Quantum mechanics has given us a new playground in which to experiment that boasts several unique features. In this thesis, we explore it in the context of thermodynamics: looking at what kind of thermal devices can be constructed and how quantum behaviour affects them. We consider three research strands. In the first part we formulate a selection of heat engines with two-qubit systems, utilising environments that induce quantum correlations into the system. We see that these correlations can have some effects on the work of the engine, but this effect is system dependent. Describing the dynamics of a quantum system in contact with an external environment is often achieved with a master equation. When considering systems comprised of multiple subsystems, the description becomes more complicated and some of the master equations that have been used previously produce unphysical results. In the second part of this thesis we show that if one does the proper analysis of the microscopic derivation of these master equations, then no thermodynamical inconsistencies occur. When one considers a system connected to three or more environments, a whole new set of possible thermodynamical machines becomes available. One notable case of these is the absorption refrigerator, which performs refrigeration without the need for an external work source. For the third part, we show how one can construct an absorption refrigerator using a three-qubit system with two-body interactions and describe its operation. We also show some thermal control properties of the three-qubit system.
Brunner et al. [Phys. Rev. E 85 (2012) 05111] have claimed that, "essentially only the smallest machines can approach Carnot efficiency". We have verified this claim by raising self-contained four-qubit quantum refrigerator, and we have shown that according to concepts of virtual qubit, it can reach the maximum efficiency in other words Carnot efficiency. But its efficiency, such as self-contained three-qubit quantum refrigerator is not universal. We also investigated a special case of self-contained four-qubit quantum refrigerator, in other words self-contained four-qubit quantum refrigerator with two hot baths in the same temperature. We demonstrated that its efficiency has the form as efficiency of a self-contained three-qubit quantum refrigerator. In other words, from the perspective of efficiency, this particular model is equivalent to self-contained three-qubit quantum refrigerator. We also demonstrated the efficiency of this particular model in the Carnot limit that is independent from details of system model, but only depends on the environmental temperatures. Also, we raised a system that consists of n-qubit which acts as a refrigerator. According to self-contained four-qubit quantum refrigerator, we also investigated a special case of self-contained n-qubit quantum refrigerator — a self-contained n-qubit quantum refrigerator with (n - 2) baths in the same temperature. We considered the three different special situations of the n-qubit refrigerator and demonstrated their efficiency in three different situations which has the form as efficiency of self-contained three-qubit quantum refrigerator. In this special situations, (n - 2) qubits are in thermal contact with isothermal heat baths.
Abstract We propose a model of two identical autonomous quantum refrigerators that interact through their qubits coupled to cold thermal baths. We consider the same specific disposition for each refrigerator related to a three-level system coupled to different thermal baths and, in turn, to a qubit as the object to be cooled. By coupling the two systems, we show that under certain conditions on the model parameters, the devices can operate in the regime of an independent autonomous quantum refrigerator or be subject to an adjustment of the thermodynamic performances. We further investigate the correlations induced by the interaction between the two refrigerators, and illustrate their behavior with respect to their thermodynamic performances. We have found that adjusting the different interaction constants of the model can lead to an evolution of the quantum correlations of the two machines that is inversely related to the behavior of the thermodynamic quantities of both refrigerators. However, this is not necessarily the case when the temperatures of the model are considered as the reference parameters.