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arXiv:2408.17015 · SciPost Physics

When does a Fermi puddle become a Fermi sea? Emergence of pairing in two-dimensional trapped mesoscopic Fermi gases

Emma Laird, Brendan C. Mulkerin, Jia Wang, Matthew J. Davis

Published Dec 11, 2024• 1 citation
arXivHTMLPDF

Abstract

Pairing lies at the heart of superfluidity in fermionic systems. Motivated by recent experiments in mesoscopic Fermi gases, we study up to six fermionic atoms with equal masses and equal populations in two different spin states, confined in a quasi-two-dimensional harmonic trap. We couple a stochastic variational approach with the use of an explicitly correlated Gaussian basis set, which enables us to obtain highly accurate energies and structural properties. Utilising two-dimensional two-body scattering theory with a finite-range Gaussian interaction potential, we tune the effective range to model realistic quasi-two-dimensional scattering. We calculate the excitation spectrum, pair correlation function, and number of pairs as a function of increasing attractive interaction strength. For up to six fermions in the ground state, we find that opposite spin and momentum pairing is maximised well below the Fermi surface in momentum space. By contrast, corresponding experiments on twelve fermions have found that pairing is maximal at the Fermi surface and strongly suppressed beneath [M. Holten et al., Nature 606, 287-291 (2022)]. This suggests that the Fermi sea — which acts to suppress pairing at low momenta via Pauli blocking — emerges in the transition from six to twelve particles.

DOI
10.21468/scipostphys.17.6.163

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Pairing lies at the heart of superfluidity in fermionic systems. Motivated by recent experiments in mesoscopic Fermi gases, we study up to six fermionic atoms with equal masses and equal populations in two different spin states, confined in a quasi-two-dimensional harmonic trap. We couple a stochastic variational approach with the use of an explicitly correlated Gaussian basis set, which enables us to obtain highly accurate energies and structural properties. Utilising two-dimensional two-body scattering theory with a finite-range Gaussian interaction potential, we tune the effective range to model realistic quasi-two-dimensional scattering. We calculate the excitation spectrum, pair correlation function, and number of pairs as a function of increasing attractive interaction strength. For up to six fermions in the ground state, we find that opposite spin and momentum pairing is maximised well below the Fermi surface in momentum space. By contrast, corresponding experiments on twelve fermions have found that pairing is maximal at the Fermi surface and strongly suppressed beneath [M. Holten et al., Nature 606, 287-291 (2022)]. This suggests that the Fermi sea — which acts to suppress pairing at low momenta via Pauli blocking — emerges in the transition from six to twelve particles.
We theoretically investigate equal-mass spin-balanced two-component Fermi gases in which pairs of atoms with opposite spins interact via a short-range isotropic model potential. We probe the distinction between two-dimensional and quasi-two-dimensional harmonic confinement by tuning the effective range parameter within two-dimensional scattering theory. Our approach, which yields numerically exact energetic and structural properties, combines a correlated Gaussian basis-set expansion with the stochastic variational method. For systems containing up to six particles, we: 1) Present the ground- and excited-state energy spectra; 2) Study non-local correlations by analysing the one- and two-body density matrices, extracting from these the occupation numbers of natural orbitals, the momentum distributions of atoms and pairs, and the molecular `condensate fraction’; 3) Study local correlations by computing the radial and pair distribution functions. This paper extends current theoretical knowledge on the properties of trapped few-fermion systems as realised in state-of-the-art cold-atom experiments.
This thesis reports on experiments investigating the emergence of many-body physics in mesoscopic two-dimensional (2D) few-fermion systems. \nThe starting point are low-entropy samples of ultracold 6Li atoms in a quasi-2D geometry. When scanning the depth of the trapping potential, we observe an enhanced stability of closed-shell configurations of the 2D harmonic oscillator. This enables us to deterministically initialize closed-shell configurations of 2, 6 and 12 atoms in the ground state. \nBy modulating the interaction strength we probe the excitation spectrum arising from the interplay of the finite single-particle gap in closed-shell configurations with the tunable attractive interactions. The full atom-counting statistics reveal pair excitations with a non-monotonous interaction dependence. These modes can be identified as the few-body precursors of a Higgs mode associated with a normal to superfluid phase transition in the thermodynamic limit. \nAdditionally, we can access the momentum distribution with single-particle resolution. This is demonstrated by measuring the momentum distribution of up to six non-interacting fermions in the ground state of the 2D trap. We observe strong density correlations that arise from fermionic quantum statistics. In the future, extending the imaging scheme to interacting systems will allow us to observe the emergence of fermionic many-body paring directly in momentum space.
Relation between the binding energy of a pair of electrons in Cooper's configuration and the magnitude of the attractive interaction between them is investigated theoretically for a two-dimensional electron gas when the electron pair has (a) zero and (b) finite center of mass momentum (CMM) first (i) in the background of a passive Fermi sea and (ii) with inclusion of the effect of Pauli exclusion principle in the presence of an active Fermi sea, at zero temperature. In the Cooper's approach (Cooper 1956 Phys. Rev. 104 1189) two pairing electrons are considered above the Fermi sea. Due to Pauli exclusion principle, these two electrons are forbidden to go into the states whose energies are less than the Fermi energy. Consequently, the role of the electrons which form the Fermi sea is passive in formation of electron pair (Fujita and Godoy 2001 Theory of High Temperature Superconductivity (Kluwer Academic Publishers)). However, in the case of an active Fermi sea, implying possible presence of multiple pairs of electrons coming out of the Fermi sea, the two electrons will have less available region in the momentum space for pair formation due to the Pauli blocking effect. In both the situations, threshold values of attractive interaction are found to exist to bind the electrons having finite CMM even with respect to the Fermi energy while with arbitrarily small value of attractive interaction they can be bound only in the case of zero CMM and that too in the presence of a passive Fermi sea. However, the presence of an active Fermi sea strongly opposes the pair formation having lower CMM. Furthermore, raising the range of the attractive interaction below and above the Fermi surface makes the pair formation more difficult due to enhanced Pauli blocking in this case. In the case of a passive Fermi sea however, with the increase in the range of the attractive interaction it becomes easier for the electron pairs to be in both Cooper pair state (CP) and true bound state (TB). These results are totally distinct from those obtained by Randeria et al (1989 Phys. Rev. Lett. 62 981, 1990 Phys. Rev. B 41 327) that a fermionic bound state in true vacuum is a necessary and sufficient condition for the Cooper pairing instability in the presence of a passive Fermi sea, independent of attractive interaction strength implying that for a potential which is attractive everywhere in two dimension, a two-body bound state exists for an arbitrarily weak attraction. Our calculations show, in the mean field approximation, that co-existence of TB state and CP state with various CMMs can occur only beyond a critical attractive interaction strength. This could lead to the formation of incoherent pairs even under strong coupling situation, which may hint onto the pseudo gap formation leading to some of the exotic features in the anomalous normal state seen in some of the exotic superconductors.
This work deals with the key constituent behind the existence of superfluid states in ultracold fermionic gases confined in a harmonic trap in 2D, namely, the formation of Cooper pairs in the presence of a Fermi sea in inhomogeneous confinement. For a set of finite-range models representing particle–particle interaction, we first ascertain the simultaneity of the emergence of bound states and the divergence of the s-wave scattering length in 2D as a function of the interaction potential parameters in free space. Then, through the analysis of two particles interacting in 2D harmonic confinement, we evaluate the energy shift with respect to the discrete harmonic oscillator levels for both repulsive and attractive cases. All of these results are the basis for determining the energy gaps of Cooper pairs arising from two particles interacting in the presence of a Fermi sea consisting of particles immersed in a 2D harmonic trap.
Interacting Fermi systems in two dimensions display intriguing phenomena such as high temperature superfluidity and pseudogap physics. These features emerge from the collective behavior of the constituent particles but are extremely hard to predict from microscopic theory. I will report on experiments that realize microscopic two-dimensional systems with ultracold fermionic lithium atoms. With the ability to deterministically prepare few-body ground states and to observe individual particles in momentum space, they enable a microscopic view of strongly interacting two-dimensional Fermi systems. Surprisingly, we find that characteristic features of many-body Fermi gases can already be found in systems of no more than a dozen particles: In spectroscopy, we observe collective excitations that are the few-body precursor of the Higgs amplitude mode of a superfluid. Moreover, in spin-resolved momentum space probes, we can directly image individual ‘Cooper pairs’ and show the presence of fermionic pairing even in a microscopic setting. These findings may broaden our understanding of finite-size Fermi systems, such as atomic nuclei and superconducting grains.
We present a coupled-pair approach for studying few-body physics in harmonically trapped ultracold gases. The method is applied to a two-component Fermi system of NNN particles. A stochastically variational Gaussian expansion method is applied, focusing on optimization of the two-body correlations present in the strongly interacting, or unitary, limit. The ground-state energy of the four-, six- and eight-body problem with equal spin populations is calculated with high accuracy and minimal computational effort. We also calculate the structural properties of these systems and discuss their implication for the many-body ultracold gas and other few-body calculations.