This thesis reports on experiments investigating the emergence of many-body physics in mesoscopic two-dimensional (2D) few-fermion systems. \nThe starting point are low-entropy samples of ultracold 6Li atoms in a quasi-2D geometry. When scanning the depth of the trapping potential, we observe an enhanced stability of closed-shell configurations of the 2D harmonic oscillator. This enables us to deterministically initialize closed-shell configurations of 2, 6 and 12 atoms in the ground state. \nBy modulating the interaction strength we probe the excitation spectrum arising from the interplay of the finite single-particle gap in closed-shell configurations with the tunable attractive interactions. The full atom-counting statistics reveal pair excitations with a non-monotonous interaction dependence. These modes can be identified as the few-body precursors of a Higgs mode associated with a normal to superfluid phase transition in the thermodynamic limit. \nAdditionally, we can access the momentum distribution with single-particle resolution. This is demonstrated by measuring the momentum distribution of up to six non-interacting fermions in the ground state of the 2D trap. We observe strong density correlations that arise from fermionic quantum statistics. In the future, extending the imaging scheme to interacting systems will allow us to observe the emergence of fermionic many-body paring directly in momentum space.
This thesis reports on experiments investigating the emergence of many-body physics in mesoscopic two-dimensional (2D) few-fermion systems. \nThe starting point are low-entropy samples of ultracold 6Li atoms in a quasi-2D geometry. When scanning the depth of the trapping potential, we observe an enhanced stability of closed-shell configurations of the 2D harmonic oscillator. This enables us to deterministically initialize closed-shell configurations of 2, 6 and 12 atoms in the ground state. \nBy modulating the interaction strength we probe the excitation spectrum arising from the interplay of the finite single-particle gap in closed-shell configurations with the tunable attractive interactions. The full atom-counting statistics reveal pair excitations with a non-monotonous interaction dependence. These modes can be identified as the few-body precursors of a Higgs mode associated with a normal to superfluid phase transition in the thermodynamic limit. \nAdditionally, we can access the momentum distribution with single-particle resolution. This is demonstrated by measuring the momentum distribution of up to six non-interacting fermions in the ground state of the 2D trap. We observe strong density correlations that arise from fermionic quantum statistics. In the future, extending the imaging scheme to interacting systems will allow us to observe the emergence of fermionic many-body paring directly in momentum space.
Many-body physics describes phenomena that cannot be understood by looking only at the constituents of a system1. Striking examples are broken symmetry, phase transitions and collective excitations2. To understand how such collective behaviour emerges as a system is gradually assembled from individual particles has been a goal in atomic, nuclear and solid-state physics for decades3–6. Here we observe the few-body precursor of a quantum phase transition from a normal to a superfluid phase. The transition is signalled by the softening of the mode associated with amplitude vibrations of the order parameter, usually referred to as a Higgs mode7. We achieve fine control over ultracold fermions confined to two-dimensional harmonic potentials and prepare closed-shell configurations of 2, 6 and 12 fermionic atoms in the ground state with high fidelity. Spectroscopy is then performed on our mesoscopic system while tuning the pair energy from zero to a value larger than the shell spacing. Using full atom counting statistics, we find the lowest resonance to consist of coherently excited pairs only. The distinct non-monotonic interaction dependence of this many-body excitation, combined with comparison with numerical calculations allows us to identify it as the precursor of the Higgs mode. Our atomic simulator provides a way to study the emergence of collective phenomena and the thermodynamic limit, particle by particle. An atomic simulator formed of a few ultracold fermionic atoms trapped in a two-dimensional harmonic potential exhibits precursors of a quantum phase transition, revealing the onset of collective quantum many-body phenomena in a few-body system.
Interacting Fermi systems in two dimensions display intriguing phenomena such as high temperature superfluidity and pseudogap physics. These features emerge from the collective behavior of the constituent particles but are extremely hard to predict from microscopic theory. I will report on experiments that realize microscopic two-dimensional systems with ultracold fermionic lithium atoms. With the ability to deterministically prepare few-body ground states and to observe individual particles in momentum space, they enable a microscopic view of strongly interacting two-dimensional Fermi systems. Surprisingly, we find that characteristic features of many-body Fermi gases can already be found in systems of no more than a dozen particles: In spectroscopy, we observe collective excitations that are the few-body precursor of the Higgs amplitude mode of a superfluid. Moreover, in spin-resolved momentum space probes, we can directly image individual ‘Cooper pairs’ and show the presence of fermionic pairing even in a microscopic setting. These findings may broaden our understanding of finite-size Fermi systems, such as atomic nuclei and superconducting grains.
In this thesis, I report on the deterministic preparation and the observation of strongly correlated few-fermion systems in single and double-well potentials. In a first experiment, we studied a system of one impurity interacting with a number of majority atoms which we prepared in a single potential well in the one-dimensional limit. With increasing number of majority particles, we observed a decrease in the quasi-particle residue which is in agreement with expectations from the Anderson orthogonality catastrophe. In a second experiment, we prepared two fermions in a double-well potential which represents the fundamental building block of the Fermi-Hubbard model. By increasing the repulsion between the two fermions, we observed the crossover into the antiferromagnetic Mott-insulator regime. Furthermore, I describe a new imaging technique, which allows spin-resolved single-atom detection both in in-situ and in time-of-flight. We use this technique to investigate the emergence of momentum correlations of two repulsive fermions in the ground state of the double well. With the methods developed in this thesis, we have established a framework for quantum simulation of strongly correlated many-body systems in tunable potentials.
Pairing lies at the heart of superfluidity in fermionic systems. Motivated by recent experiments in mesoscopic Fermi gases, we study up to six fermionic atoms with equal masses and equal populations in two different spin states, confined in a quasi-two-dimensional harmonic trap. We couple a stochastic variational approach with the use of an explicitly correlated Gaussian basis set, which enables us to obtain highly accurate energies and structural properties. Utilising two-dimensional two-body scattering theory with a finite-range Gaussian interaction potential, we tune the effective range to model realistic quasi-two-dimensional scattering. We calculate the excitation spectrum, pair correlation function, and number of pairs as a function of increasing attractive interaction strength. For up to six fermions in the ground state, we find that opposite spin and momentum pairing is maximised well below the Fermi surface in momentum space. By contrast, corresponding experiments on twelve fermions have found that pairing is maximal at the Fermi surface and strongly suppressed beneath [M. Holten et al., Nature 606, 287-291 (2022)]. This suggests that the Fermi sea — which acts to suppress pairing at low momenta via Pauli blocking — emerges in the transition from six to twelve particles.
This thesis reports on experiments conducted in a single layer, quasi two-dimensional, two-component ultracold Fermi gas in the strongly interacting regime. Ultracold gases can be used to simulate key aspects of more complicated systems like for example cuprates which show high-Tc superconductivity. \nThe momentum distribution of a sample of bosonic dimers in a quasi-2D square lattice geometry was measured to obtain the coherence properties. For shallow lattices, sharp peaks in the momentum distribution, indicating coherence, were observed at zero momentum as well as at positive and negative lattice momenta along each axis. For deeper \nlattices, heating impeded the ability to prepare a Mott-insulator. \nA spatially resolved radio-frequency spectroscopy was employed for a quasi-2D Fermi gas in the normal phase throughout the BEC-BCS crossover. The interaction induced \nenergy shifts were measured in the strongly interacting region where they can be on the order of the Fermi energy and thus the local resolution is crucial. Furthermore, the onset of pairing in the strongly interacting region was measured as a function of temperature and it was shown that the fraction of free atoms decreases faster than expected from thermal non-interacting theory. At last, the pairing gap was measured using an imbalanced sample. On the BEC side it was found to be in very good agreement with two-body physics as expected. In the strongly interacting regime, however, a deviation from two-body physics indicates that here many-body effects play a role and thus further studies are required.
Fermion pairing underlies collective quantum phenomena across widely different forms of matter. In extended systems such as ultracold Fermi gases, pairing is commonly understood through the BCS--BEC crossover, where the pair size evolves from large, overlapping Cooper pairs to tightly bound dimers. In finite systems such as atomic nuclei, superconducting grains and quantum dots, however, the same pairing tendency competes with confinement, shell filling and spatial inhomogeneity, making the microscopic structure of pairs much harder to access. Here, we image pair correlations in a finite, tunable system of few fermionic atoms with single-particle resolution and full counting statistics. We observe that confinement and shell structure re-organize pairing in real space: In the weakly interacting, confinement-dominated regime, closed-shell configurations suppress correlations in the high-density trap center. Pairing is mainly observed toward the low-density surface. Open-shell systems, however, support substantially stronger central pairing. Already for surprisingly small systems, increasing either interaction strength or particle number restores a locally bulk-like Cooper-pair profile in the trap center, whereas the edge retains dimer-like correlations. By resolving where pairs form and how their character changes from localized dimers to overlapping Cooper pairs, our measurements provide a microscopic view of pairing in finite fermionic matter and connect the physics of mesoscopic cold atoms to pairing phenomena in nuclei and superconducting nanostructures.