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arXiv:2406.08546 · Nature Communications

Parafermions in moiré minibands

Hui Liu, Raül Perea‐Causín, Emil J. Bergholtz

Published Feb 19, 2025• 5 citations
arXivHTMLPDF

Abstract

Abstract Moiré materials provide a remarkably tunable platform for topological and strongly correlated quantum phases of matter. Very recently, the first Abelian fractional Chern insulators (FCIs) at zero magnetic field have been experimentally demonstrated, and it has been theoretically predicted that non-Abelian states with Majorana fermion excitations may be realized in the nearly dispersionless minibands of these systems. Here, we provide telltale evidence based on many-body exact diagonalization for the even more exotic possibility of moiré-based non-Abelian FCIs exhibiting Fibonacci parafermion excitations. In particular, we obtain low-energy quantum numbers, spectral flow, many-body Chern numbers, and entanglement spectra consistent with the $${{\mathbb{Z}}}_{3}$$ Z 3 Read–Rezayi parafermion phase in an exemplary moiré system with tunable quantum geometry. Our results hint towards the robustness of moiré-based parafermions and encourage the pursuit in moiré systems of these non-Abelian quasiparticles that are superior candidates for topological quantum computing.

DOI
10.1038/s41467-025-57035-x

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Abstract Moiré materials provide a remarkably tunable platform for topological and strongly correlated quantum phases of matter. Very recently, the first Abelian fractional Chern insulators (FCIs) at zero magnetic field have been experimentally demonstrated, and it has been theoretically predicted that non-Abelian states with Majorana fermion excitations may be realized in the nearly dispersionless minibands of these systems. Here, we provide telltale evidence based on many-body exact diagonalization for the even more exotic possibility of moiré-based non-Abelian FCIs exhibiting Fibonacci parafermion excitations. In particular, we obtain low-energy quantum numbers, spectral flow, many-body Chern numbers, and entanglement spectra consistent with the Z3{{\mathbb{Z}}}_{3}Z3​ Z 3 Read–Rezayi parafermion phase in an exemplary moiré system with tunable quantum geometry. Our results hint towards the robustness of moiré-based parafermions and encourage the pursuit in moiré systems of these non-Abelian quasiparticles that are superior candidates for topological quantum computing.
Breakthrough experiments have recently realized fractional Chern insulators (FCIs) in moiré materials. However, all states observed are Abelian; the possible existence of more exotic non-Abelian FCIs remains controversial both experimentally and theoretically. Here, we investigate the competition between charge density wave (CDW) order, gapless composite fermion liquid (CFL), and non-Abelian Moore-Read states at half filling of a moiré band. Although ground-state (quasi)degeneracies and spectral flow are not sufficient for distinguishing between charge order and Moore-Read states, we find evidence using entanglement spectroscopy that both these states of matter can be realized with Coulomb interactions. By further analyzing the graviton excitations of Moore-Read states, we unveil that the ground states exhibit a mixed behavior of Pfaffian and anti-Pfaffian, despite the weak breaking of particle-hole symmetry. In a double twisted bilayer graphene model, transitions between these phases can be driven by the coupling strength between the layers: at weak coupling there is a CFL phase and at strong coupling a CDW order emerges. Remarkably, however, there is compelling evidence for a non-Abelian Moore-Read FCI phase at intermediate coupling.
Higher vortexability is often viewed as a route to topological flat bands with higher-Landau-level-like quantum geometry. Here we emphasize a complementary perspective: it provides a tunable multiband structure in which wave function geometry can be varied continuously while the band dispersion, degeneracy, and topology remain fixed. We perform systematic exact-diagonalization studies of many-body phases in fractionally filled higher vortexable moiré systems, retaining the full flat-band Hilbert space rather than projecting onto a single band. The multiband treatment reveals a cascade of Abelian and non-Abelian phases at zero magnetic field, including integer and fractional exciton insulators, Abelian fractional Chern insulators, Moore-Read and Read-Rezayi states. At fixed filling, different phases are connected through transitions or crossovers driven solely by changes in wave function geometry, highlighting quantum geometry itself as a direct tuning parameter between competing topological states. At fillings associated with Moore-Read and Read-Rezayi states, our calculations show that interband mixing shifts the optimal quantum geometry regime without suppressing non-Abelian topological order under screened Coulomb interaction. Our results establish higher vortexable moiré bands as a tunable platform for exploring geometry-driven multiband topological phases at zero magnetic field.
Parafermion modes are non-Abelian anyons which were introduced as ZN{\mathbb{Z}}_{N}ZN​ generalizations of Z2{\mathbb{Z}}_{2}Z2​ Majorana states. In particular, Z3{\mathbb{Z}}_{3}Z3​ parafermions can be used to produce Fibonacci anyons, laying a path towards universal topological quantum computation. Due to their fractional nature, much of the theoretical work on Z3{\mathbb{Z}}_{3}Z3​ parafermions has relied on bosonization methods or parafermionic quasiparticles. In this paper, we introduce a representation of Z3{\mathbb{Z}}_{3}Z3​ parafermions in terms of purely fermionic models. We establish the equivalency of a family of lattice fermionic models written in the basis of the $t\ensuremath{-}J$ model with a Kitaev-like chain supporting free Z3{\mathbb{Z}}_{3}Z3​ parafermionic modes at its ends. By using density matrix renormalization group calculations, we are able to characterize the topological phase transition and study the effect of local operators (doping and magnetic fields) on the spatial localization of the parafermionic modes and their stability. Moreover, we discuss the necessary ingredients towards realizing Z3{\mathbb{Z}}_{3}Z3​ parafermions in strongly interacting electronic systems.
The possibility of realizing non-Abelian excitations (non-Abelions) in two-dimensional (2D) Abelian states of matter has generated a lot of interest recently. A well-known example of such non-Abelions are parafermion zeros modes (PFZMs) which can be realized at the endpoints of the so called genons in fractional quantum Hall (FQH) states or fractional Chern insulators (FCIs). In this letter, we discuss some known signatures of PFZMs and also introduce some novel ones. In particular, we show that the topological entanglement entropy (TEE) shifts by a quantized value after crossing PFZMs. Utilizing those signatures, we present the first large scale numerical study of PFZMs and their stability against perturbations in both FQH states and FCIs within the density-Matrix-Renormalization-Group (DMRG) framework. Our results can help build a closer connection with future experiments on FQH states with genons.
Twisted bilayer materials provide a versatile platform for realizing correlated topological states. Motivated by the recent experimental realization of atomic Bose-Einstein condensates in twisted bilayer optical lattices, we investigate the emergence of fractional topological phases in such systems. For experimentally realistic parameters, the single-particle spectrum hosts a pair of quasi-degenerate nearly flat moiré bands. We show using self-consistent Hartree-Fock calculations that atomic interactions spontaneously break time-reversal symmetry, lift the quasi-degeneracy, and generate an isolated nearly flat band with a nonzero Chern number. At fractional filling, exact diagonalization of the Hamiltonian projected to this band reveals a threefold degenerate ground-state manifold and a characteristic particle entanglement spectrum, providing strong evidence for a fractional Chern insulator. The resulting many-body gap is of order 10−3ER10^{-3}E_R10−3ER​, corresponding to a nanokelvin energy scale accessible to state-of-the-art cold-atom experiments. Our scheme requires neither spin-orbit coupling, as in transition metal dichalcogenides, nor a finite magnetic field, as in existing twisted-bilayer-graphene experiments, providing a highly tunable route to strongly correlated topological phases in twisted bilayer optical lattices.
Experimental realizations of Abelian fractional Chern insulators (FCIs) have demonstrated the potentials of moiré systems in synthesizing exotic quantum phases. Remarkably, twisted multilayer graphene system may also host non-Abelian states competing with charge density wave under Coulomb interaction. Here, through larger scale exact diagonalization simulations, we map out the quantum phase diagram for ν=1/2ν=1/2ν=1/2 system with electrons occupying the lowest moirè band of the double twisted bilayer graphene. By increasing the system size, we find the ground state has six-fold near degeneracy and with a finite spectral gap separating the ground states from excited states across a broad range of parameters. Further computation of many-body Chern number establish the topological order of the state, and we rule out possibility of charge density wave orders based on featureless density structure factor. Furthermore, we inspect the particle-cut entanglement spectrum to identify the topological state as a non-Abelian Moore-Read state. Combining all the above evidences we conclude that Moore-Read ground state dominates the quantum phase diagram for the double twisted bilayer graphene system for a broad range of coupling strength with realistic Coulomb interaction.