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arXiv:2403.18319

Doppler-assisted quantum resonances through swappable excitation pathways in Potassium vapor

Gourab Pal, Subhasish Dutta Gupta, Saptarishi Chaudhuri

Published Mar 27, 2024• 0 citations
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Abstract

We report the observation of two additional sub-natural line width quantum interference in the $D_2$ manifold of $^{39}K$ vapor, in addition to the usual single Electromagnetically induced transparency peak. The other two features appear exclusively because $^{39}K$ ground hyperfine splitting is smaller than the Doppler broadened absorption profile. This allows probe and control beams to swap their transition pathways. The control beam detuning captures the nature of the coherence, therefore an unusual phenomenon of conversion from perfect transparency to enhanced absorption is observed and explained by utilizing adiabatic elimination of the excited state in the Master equation. Controlling such dark and bright resonances leads to new applications in quantum technologies viz. frequency offset laser stabilization and long-lived quantum memory.

DOI
10.48550/arxiv.2403.18319

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We report the observation of two additional sub-natural line width quantum interference in the D2D_2D2​ manifold of 39K^{39}K39K vapor, in addition to the usual single Electromagnetically induced transparency peak. The other two features appear exclusively because 39K^{39}K39K ground hyperfine splitting is smaller than the Doppler broadened absorption profile. This allows probe and control beams to swap their transition pathways. The control beam detuning captures the nature of the coherence, therefore an unusual phenomenon of conversion from perfect transparency to enhanced absorption is observed and explained by utilizing adiabatic elimination of the excited state in the Master equation. Controlling such dark and bright resonances leads to new applications in quantum technologies viz. frequency offset laser stabilization and long-lived quantum memory.
We report the observation of two additional sub-natural line width quantum interferences in the D2 manifold of 39K vapor, in addition to the usual single Electromagnetically induced transparency peak. The other two features appear exclusively because 39K ground hyperfine splitting is smaller than the Doppler broadened absorption profile. This allows probe and control beams to swap their transition pathways. The control beam detuning captures the nature of the coherence, therefore an unusual phenomenon of conversion from perfect transparency to enhanced absorption is observed and explained by utilizing adiabatic elimination of the excited state in the Master equation. Controlling such dark and bright resonances leads to new applications in quantum technologies viz. frequency offset laser stabilization and long-lived quantum memory.
We report the observation of two additional sub-natural line width quantum interferences in the D2 manifold of 39K vapor, in addition to the usual single Electromagnetically induced transparency peak. The other two features appear exclusively because 39K ground hyperfine splitting is smaller than the Doppler broadened absorption profile. This allows probe and control beams to swap their transition pathways. The control beam detuning captures the nature of the coherence, therefore an unusual phenomenon of conversion from perfect transparency to enhanced absorption is observed and explained by utilizing adiabatic elimination of the excited state in the Master equation. Controlling such dark and bright resonances leads to new applications in quantum technologies viz. frequency offset laser stabilization and long-lived quantum memory.
Abstract We report the observation of two additional sub-natural line width quantum interferences in the D 2 manifold of 39 K vapor, in addition to the usual single Electromagnetically Induced Transparency (EIT) peak. In a typical three level Λ-type system, only one EIT peak is observed. However, here we report observation of two additional line shapes riding on top of the absorption profile. The fact that the hyperfine splitting is smaller than the Doppler width in 39 K allows the probe and control beams to swap their transition pathways in different velocity groups of atoms even when their frequencies are kept constant. Our observations are in striking contrast to standard EIT measurements. These findings are in quantitative agreement with density matrix formalism taking into account velocity-selective two-photon resonances. Owing to the favorably low ground hyperfine splitting (Δ hf ) in 39 K, which allows a significantly large number of atoms with a Doppler shift greater than or equal to the Δ hf , the strength of these additional resonances is strong compared to that of other alkali atoms such as 87 Rb, 133 Cs where these resonances can not be observed. The control photon detuning to atomic transition captures the nature of the coherence; therefore an unusual phenomenon of conversion from perfect transparency to enhanced absorption of the probe photon is observed and explained by utilizing the adiabatic elimination of the excited state in the Master equation. Controlling such dark and bright resonances leads to new applications in quantum technologies such as frequency-offset laser stabilization and long-lived quantum memory.
The cesium D2{D}_{2}D2​ line closed hyperfine transition $F=4\ensuremath{\rightarrow}{F}^{\ensuremath{'}}=5$ was simultaneously coupled and probed in a hot atomic beam. We experimentally showed that, when the probe laser frequency approached that of the two-photon-resonance corresponding to electromagnetically induced absorption conditions, an enhanced transparency of the coupling laser appeared, combined with a further central absorption peak at zero probe laser detuning. Simultaneously, the coupling laser parametric dispersion showed a broad negative pattern together with a narrower steep positive phase shift in correspondence with the two-photon resonance, with sub-Doppler half-widths down to about 10kHz10\phantom{\rule{0.3em}{0ex}}\mathrm{kHz}10kHz.
We experimentally observe a non-linear absorption resonance in one of the two probe beams of a double Λ system which is interacting with three optical beams. This probe beam counterpropagates to the other two beams, both of which are co-propagating. The absorption resonance in this probe beam arises due to interaction between the dark states of the double Λ created by the co-propagating beams. The double Λ configuration of levels is in the D2 hyperfine manifold of 87Rb atoms, and the interaction is studied at room temperature. The non-linear absorption resonance is shown to be a three-photon process arising whenever the two co-propagating beams satisfy the two-photon Raman condition, necessary for electromagnetically induced transparency. Through a dressed state analysis, we show that the absorption feature is a result of interference between the absorption pathways to the excited states, from the ground states of the double Λ. The non-linear nature of the probe beam absorption enables it to perform like a directional optical switch. This absorption switch operates conditioned on non-absorption of a single photon of the same frequency due to a coherent process, in a beam traveling in the opposite direction.
We observed a detuned slow light phenomenon based on electromagnetically induced transparency in (87)Rb D2 line composed of multiple excited-hyperfine states within a Doppler-broadened linewidth. The results show that the maximum group delay of a probe occurs at off-detuned two-photon resonance frequency. The observed detuned group delay is analyzed with numerical calculations for a probe pulse interacting with the neighboring excited-states-modified Doppler broadening atoms for a fixed coupling field. The experimental results are in good agreement with the numerical calculations.