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arXiv:2403.13622 · Journal of Physics A Mathematical and Theoretical

Nonlocality of the energy density of a spontaneously emitted single-photon from a Hydrogen atom

Maxime Federico, Hans Rudolf Jauslin

Published Nov 27, 2024• 1 citation
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Abstract

Abstract We analyze through the expectation value of the energy density the spatial nonlocality of single photons emitted by the spontaneous decay of a Hydrogen atom. By using a minimal coupling between the quantized electromagnetic field and the atom, we compute the state of the photon under the assumption that only a single-photon is produced. The calculations are thus performed in the subspace of single-photon states which is essentially equivalent to the rotating wave approximation. We obtain a characterization of the spatial decay of the energy density. We compute the asymptotic limit of large distances from the atom at each given time, and find an algebraic behavior of 1 / r 6 . This result confirms that the energy density of single-photon states is nonlocal and the algebraic decay is far from the maximal quasiexponential localization predicted by the theory.

DOI
10.1088/1751-8121/ad97fa

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Abstract We analyze through the expectation value of the energy density the spatial nonlocality of single photons emitted by the spontaneous decay of a Hydrogen atom. By using a minimal coupling between the quantized electromagnetic field and the atom, we compute the state of the photon under the assumption that only a single-photon is produced. The calculations are thus performed in the subspace of single-photon states which is essentially equivalent to the rotating wave approximation. We obtain a characterization of the spatial decay of the energy density. We compute the asymptotic limit of large distances from the atom at each given time, and find an algebraic behavior of 1 / r 6 . This result confirms that the energy density of single-photon states is nonlocal and the algebraic decay is far from the maximal quasiexponential localization predicted by the theory.
We investigate, in the case of the $2P\text{\ensuremath{-}}1S$ transition in atomic hydrogen, the behavior of the spontaneously emitted electromagnetic field in space-time. We focus on Glauber's wave function for the emitted photon, a quantity which we find is nonzero outside the light cone at all times after the start of the emission. We identify the uncertainty on the position of the decaying electron as a source of departure from causality in the naive sense of the term. We carry out a detailed study of the emitted electric field in the mid- and far-field regions, through analytical and numerical computations as well as asymptotic arguments.
We investigate, in the case of the 2p−1s2\mathrm{p}-1\mathrm{s}2p−1s transition in atomic Hydrogen, the behaviour of the spontaneously emitted electromagnetic field in spacetime. We focus on Glauber's wave function for the emitted photon, a quantity which we find is nonzero outside the lightcone at all times after the start of the emission. We identify the uncertainty on the position of the decaying electron as a source of departure from causality in the naive sense of the term. We carry out a detailed study of the emitted electric field in the mid- and far-field regions, through analytical and numerical computations as well as asymptotic arguments.
The time-dependent electric energy density surrounding a two-level atom fixed at r = 0 is studied, the atom being taken in its excited state at t = 0 and the field being initially in the vacuum state. The atom-field coupling includes both rotating and counter-rotating terms. The energy density of the spontaneously emitted field in the rotating wave approximation is shown to behave non-causally, while in the presence of the complete coupling it is shown to vanish outside a sphere of radius r = ct centred on the atom. The deviations of atomic dynamics from the exponential Wigner-Weisskopf behaviour during spontaneous decay are shown to be deeply influenced by the counter-rotating terms. It is concluded that the virtual photons induced by the counter-rotating terms in the atom-field coupling are essential in order to ensure causality and cannot be neglected in any accurate treatment of spontaneous emission.
The nonlocality of single-photon states has been analyzed from several different but interrelated perspectives. In this article we propose a demonstration based on the electromagnetic energy density observable and on the antilocal property of the frequency operator $\mathrm{\ensuremath{\Omega}}=c{(\ensuremath{-}\mathrm{\ensuremath{\Delta}})}^{1/2}$. The present proof is based on the standard quantization of the electromagnetic field, which can be formulated equivalently in the momentum representations or in the position representations of Landau and Peierls [Z. Phys. 62, 188 (1930)] and of Bia\l{}ynicki-Birula [edited by E. Wolf (Elsevier, Amsterdam, 1996)]. Our proof extends to all single-photon states the results of Bia\l{}ynicki-Birula, which were formulated for two particular classes of states, those involving a uniform localization [Phys. Rev. Lett. 80, 5247 (1998)] or alternatively states that are electrically or magnetically localized [Phys. Rev. A 79, 032112 (2009)]. Our approach is formulated in terms of Knight's definition of strict localization [J. Math. Phys. 2, 459 (1961)], based on the comparison of expectation values of single-photon states of local observables with those of the vacuum.
We calculate spatial localization and phase properties of spontaneously emitted photons. Our model is simple yet fully quantized: the emitting atom is a two-level atom located in a one-dimensional multimode optical cavity. Although the photon state vector does not have a position-space representation, the expectation value of the square of the electric field operator (intensity) is spatially localized and this pattern shifts at the speed of light. The emitted photon exhibits classical-like phase properties in the intensity expectation value when it “interferes with itself” after reflection. The phase properties of the emitted radiation are also evident at times sufficiently long for the radiation to have returned to the emitting atom before the decay of excited atomic state is complete.