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Journal of Modern Optics

Virtual Photons, Causality and Atomic Dynamics in Spontaneous Emission

G. Compagno, Roberto Passante, Franco Persico

Published Aug 1, 1990• 23 citations
Publisher

Abstract

The time-dependent electric energy density surrounding a two-level atom fixed at r = 0 is studied, the atom being taken in its excited state at t = 0 and the field being initially in the vacuum state. The atom-field coupling includes both rotating and counter-rotating terms. The energy density of the spontaneously emitted field in the rotating wave approximation is shown to behave non-causally, while in the presence of the complete coupling it is shown to vanish outside a sphere of radius r = ct centred on the atom. The deviations of atomic dynamics from the exponential Wigner-Weisskopf behaviour during spontaneous decay are shown to be deeply influenced by the counter-rotating terms. It is concluded that the virtual photons induced by the counter-rotating terms in the atom-field coupling are essential in order to ensure causality and cannot be neglected in any accurate treatment of spontaneous emission.

DOI
10.1080/09500349014551511

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The time-dependent electric energy density surrounding a two-level atom fixed at r = 0 is studied, the atom being taken in its excited state at t = 0 and the field being initially in the vacuum state. The atom-field coupling includes both rotating and counter-rotating terms. The energy density of the spontaneously emitted field in the rotating wave approximation is shown to behave non-causally, while in the presence of the complete coupling it is shown to vanish outside a sphere of radius r = ct centred on the atom. The deviations of atomic dynamics from the exponential Wigner-Weisskopf behaviour during spontaneous decay are shown to be deeply influenced by the counter-rotating terms. It is concluded that the virtual photons induced by the counter-rotating terms in the atom-field coupling are essential in order to ensure causality and cannot be neglected in any accurate treatment of spontaneous emission.
The time-dependent electric-energy density surrounding a two-level atom fixed at r = 0 is studied, the atom being taken in its ground state at t = 0 and the field having initially only one photon in a delocalized mode. The atom-field coupling includes both rotating and counterrotating terms. The energy density in the rotating wave approximation is shown to behave noncausally, while in the presence of the complete coupling it is shown to be affected only within a sphere of radius r = ct centred on the atom. It is concluded that the counterrotating terms in the atom-field coupling are essential in order to ensure causality and cannot be neglected in any accurate treatment of photon absorption. Some consequences of this conclusion on the operation of photodetectors in one-photon absorption are discussed.
Spontaneous emission in dipole approximation is studied theoretically using both source-field theory and a Schrodinger picture approach. Using source-field theory we obtain formal equations for the Poynting vector and energy density without making the rotating wave approximation (RWA) and Weisskopf-Wigner approximation (WWA). The initial condition at t=0 is one in which the atom is in an excited state and the field in the vacuum state. The source-field expressions are evaluated within the the RWA and WWA and are found to satisfy Poynting's theorem. To explore the consequences of not making the RWA and WWA, the Poynting vector and energy density are calculated using perturbation theory. We use a Schrodinger picture approach and essentially reproduce and complement the results of Compagno, Passante, and Persico [J. Mod. Optics 37:8, 1377 (2007)] and those of Power and Thirunamachandran [Phys. Rev. A 45, 54 (1992)] obtained using a Heisenberg picture approach. The theory involves a sum over field mode frequencies and both finite cutoffs and convergence factors are used to carry out the sums. It is shown that the perturbation theory calculation leads to unphysical values for atomic state populations for all times when a sum over all field frequencies is taken, even if a convergence factor is used. It is also proved that the fields calculated using source-field theory always satisfy Poynting's theorem for ct not equal to R, where R is the distance from the atom.
The dynamics of an initially bare pair of two-level atoms at distance R is investigated. The pair is coupled to the vacuum radiation field in the multipolar scheme and in the dipole approximation. The Heisenberg equations of motion for various atomic operators are obtained neglecting terms O(e3{\mathit{e}}^{3}e3) and for t smaller than the spontaneous relaxation time. A rigorous proof of causality in the atom-atom interaction is given. Interatomic correlations, however, are shown to develop for tR/c. This early development is shown to be compatible with the principle of relativistic causality, and to be related to the peculiar form of the vacuum zero-point fluctuations. The techniques adopted are applied to study dynamics and correlations of a superradiant state.
Quantum interference in spontaneous emission from a four-level atom is investigated with the counter-rotating terms and the energy shifts included. The atom has two upper levels which are coupled to a common lower level by the same vacuum modes and are driven by a coherent field to an auxiliary level. The effect of the counter-rotating terms in the coupling through the vacuum modes is taken into account by a unitary transformation method. We show how the quantum interference due to the energy shifts affects the spontaneous emission.
The collective spontaneous emission of NNN multilevel atoms is studied in optical vector theory and without applying the rotating-wave approximation. The counter-rotating terms are included using a unitary transformation method. We analyze the decay dynamics starting from two initial conditions, the standard Dicke and timed Dicke states. In addition to the dependence on ensemble volume and density, we also study the effect of the ensemble geometry on cooperative emission for spheres, cubes, and quasi-two-dimensional shapes in different orientations. Finally, time-dependent cooperative spontaneous emission rates are introduced and investigated.