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arXiv:2403.13582 · Physical Review A

Bosonic functional determinant approach and its application to polaron spectra

Moritz Drescher, Manfred Salmhofer B, Tilman Enss

Published Dec 2, 2024• 5 citations
arXivHTMLPDF

Abstract

The functional determinant approach (FDA) is a simple method to compute exactly certain observables for ideal quantum systems and has been successfully applied to the Fermi polaron problem to obtain the dynamical overlap and spectral function. Unfortunately, its application to bosonic ultracold gases is prohibited by the failure of the grand canonical ensemble for these systems. In this paper we show how to circumvent this problem and develop a bosonic FDA. This yields exact injection and ejection spectra for ideal Bose polarons at arbitrary temperatures. While coherent features visible at absolute zero quickly smear out with rising temperature as expected, the linewidth of the main peak is, counterintuitively, found to decrease near unitarity. Furthermore, we provide explicit formulas for the overlap operator, which allow us to compute the necessary determinants for both Bose and Fermi polarons more efficiently than previously possible.

DOI
10.1103/physreva.110.063303

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The functional determinant approach (FDA) is a simple method to compute exactly certain observables for ideal quantum systems and has been successfully applied to the Fermi polaron problem to obtain the dynamical overlap and spectral function. Unfortunately, its application to bosonic ultracold gases is prohibited by the failure of the grand canonical ensemble for these systems. In this paper we show how to circumvent this problem and develop a bosonic FDA. This yields exact injection and ejection spectra for ideal Bose polarons at arbitrary temperatures. While coherent features visible at absolute zero quickly smear out with rising temperature as expected, the linewidth of the main peak is, counterintuitively, found to decrease near unitarity. Furthermore, we provide explicit formulas for the overlap operator, which allow us to compute the necessary determinants for both Bose and Fermi polarons more efficiently than previously possible.
Abstract In this brief review, we report some new development in the functional determinant approach (FDA), an exact numerical method, in the studies of a heavy quantum impurity immersed in Fermi gases and manipulated with radio-frequency pulses. FDA has been successfully applied to investigate the universal dynamical responses of a heavy impurity in an ultracold ideal Fermi gas in both the time and frequency domain, which allows the exploration of the renowned Anderson’s orthogonality catastrophe (OC). In such a system, OC is induced by the multiple particle-hole excitations of the Fermi sea, which is beyond a simple perturbation picture and manifests itself as the absence of quasiparticles named polarons. More recently, two new directions for studying heavy impurity with FDA have been developed. One is to extend FDA to a strongly correlated background superfluid background, a Bardeen–Cooper–Schrieffer (BCS) superfluid. In this system, Anderson’s orthogonality catastrophe is prohibited due to the suppression of multiple particle-hole excitations by the superfluid gap, which leads to the existence of genuine polaron. The other direction is to generalize the FDA to the case of multiple RF pulses scheme, which extends the well-established 1D Ramsey spectroscopy in ultracold atoms into multidimensional, in the same spirit as the well-known multidimensional nuclear magnetic resonance and optical multidimensional coherent spectroscopy. Multidimensional Ramsey spectroscopy allows us to investigate correlations between spectral peaks of an impurity-medium system that is not accessible in the conventional one-dimensional spectrum.
We investigate the system of a heavy impurity embedded in a paired two-component Fermi gas at the crossover from a Bose-Einstein condensate (BEC) to a Bardeen-Cooper-Schrieffer (BCS) superfluid via an extension of the functional determinant approach (FDA). FDA is an exact numerical approach applied to study manifestations of Anderson's orthogonality catastrophe (OC) in the system of a static impurity immersed in an ideal Fermi gas. Here, we extend the FDA to a strongly correlated superfluid background described by a BCS mean-field wave function. In contrast to the ideal Fermi gas case, the pairing gap in the BCS superfluid prevents the OC and leads to genuine polaron signals in the spectrum. Thus our exactly solvable model can provide a deeper understanding of polaron physics. In addition, we find that the polaron spectrum can be used to measure the superfluid pairing gap, and in the case of a magnetic impurity, the energy of the subgap Yu-Shiba-Rusinov (YSR) bound state. Our theoretical predictions can be examined with state-of-art cold-atom experiments.
We extend the functional determinant approach (FDA), previously restricted to static impurities, to the case of finite-mass impurities by using the mass-gap description of Fermi polarons [Phys. Rev. Lett. 135, 193401 (2025)]. The quadratic structure of the mass-gap model enables the exact evaluation of many-body spectra and Ramsey dynamics for mobile impurities. We show that this mass-gap FDA smoothly interpolates between the Fermi-edge singularity for infinitely heavy impurities and the emergence of quasiparticle weight for finite impurity mass. Our results demonstrate that the mass-gap FDA provides a transparent and computationally efficient framework to describe the quantum dynamics of mobile impurities.
We give a detailed account of a stationary impurity in an ideal Bose-Einstein condensate, which we call the ideal Bose polaron, at both zero and nonzero temperatures and arbitrary strength of the impurity-boson coupling. The time evolution is solved exactly and it is found that, surprisingly, many of the features that have been predicted for the real BEC are already present in this simpler setting and can be understood analytically therein. We obtain explicit formulas for the time evolution of the condensate wave function at T=0T=0T=0 and of the one-particle density matrix at T>0T>0T>0. For negative scattering length, the system is found to thermalize even though the dynamics are perfectly coherent. The time evolution and thermal values of the Tan contact are derived and compared to a recent experiment. We find that contrary to the Fermi polaron, the contact is not bounded at unitarity as long as a condensate exists. An explicit formula for the dynamical overlap at T=0T=0T=0 allows us to compute the rf spectrum which can be understood in detail by relating it to the two-body problem of one boson and the impurity.
We present a systematic study of a mobile impurity immersed in a three-dimensional Fermi sea of fermions at finite temperature, by using the standard non-self-consistent many-body TTT-matrix theory that is equivalent to a finite-temperature variational approach with the inclusion of one-particle-hole excitation. The impurity spectral function is determined in the real-frequency domain, avoiding any potential errors due to the numerical analytic continuation in previous TTT-matrix calculations and the small spectral broadening parameter used in variational calculations. In the weak-coupling limit, we find that the quasiparticle decay rate of both attractive and repulsive polarons does not increase significantly with increasing temperature, and therefore Fermi polarons may remain well defined far above Fermi degeneracy. In contrast, near the unitary limit with strong coupling, the decay rate of Fermi polarons rapidly increases and the quasiparticle picture breaks down close to the Fermi temperature. We analyze in detail the recent ejection and injection radio-frequency (rf) spectroscopy measurements, performed at Massachusetts Institute of Technology (MIT) and at the European Laboratory for Non-Linear Spectroscopy (LENS), respectively. We show that the momentum average of the spectral function, which is necessary to account for the observed rf spectroscopy, has a sizable contribution to the width of the quasiparticle peak in spectroscopy. As a result, the measured decay rate of Fermi polarons could be significantly larger than the calculated quasiparticle decay rate at zero momentum. By taking this crucial contribution into account, we find that there is a reasonable agreement between theory and experiment for the lifetime of Fermi polarons in the strong-coupling regime, as long as they remain well defined.
We calculate nonperturbative self-consistent fermionic and bosonic spectral functions of ultracold Fermi gases with the spectral functional approach. This approach allows for a direct real-time computation of nonperturbative correlation functions, and in the present work we use spectral Dyson-Schwinger equations. We focus on the normal phase of the spin-balanced Fermi gas and provide numerical results for the full fermionic and bosonic spectral functions. The spectral functions are then used for the determination of the equation of state, the Tan contact, and ejection rf spectra at unitarity. These results are compared to experimental data, the self-consistent TTT-matrix approach, and lattice results. Our approach offers a wide range of applications, including the ab initio calculation of transport and spectral properties of the superfluid phase in the BCS-BEC crossover.