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arXiv:2201.07872 · Physical Review A

Fermi polarons at finite temperature: Spectral function and rf spectroscopy

Hui Hu, Xia-Ji Liu

Published Apr 8, 2022• 20 citations
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Abstract

We present a systematic study of a mobile impurity immersed in a three-dimensional Fermi sea of fermions at finite temperature, by using the standard non-self-consistent many-body $T$-matrix theory that is equivalent to a finite-temperature variational approach with the inclusion of one-particle-hole excitation. The impurity spectral function is determined in the real-frequency domain, avoiding any potential errors due to the numerical analytic continuation in previous $T$-matrix calculations and the small spectral broadening parameter used in variational calculations. In the weak-coupling limit, we find that the quasiparticle decay rate of both attractive and repulsive polarons does not increase significantly with increasing temperature, and therefore Fermi polarons may remain well defined far above Fermi degeneracy. In contrast, near the unitary limit with strong coupling, the decay rate of Fermi polarons rapidly increases and the quasiparticle picture breaks down close to the Fermi temperature. We analyze in detail the recent ejection and injection radio-frequency (rf) spectroscopy measurements, performed at Massachusetts Institute of Technology (MIT) and at the European Laboratory for Non-Linear Spectroscopy (LENS), respectively. We show that the momentum average of the spectral function, which is necessary to account for the observed rf spectroscopy, has a sizable contribution to the width of the quasiparticle peak in spectroscopy. As a result, the measured decay rate of Fermi polarons could be significantly larger than the calculated quasiparticle decay rate at zero momentum. By taking this crucial contribution into account, we find that there is a reasonable agreement between theory and experiment for the lifetime of Fermi polarons in the strong-coupling regime, as long as they remain well defined.

DOI
10.1103/physreva.105.043303

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We present a systematic study of a mobile impurity immersed in a three-dimensional Fermi sea of fermions at finite temperature, by using the standard non-self-consistent many-body TTT-matrix theory that is equivalent to a finite-temperature variational approach with the inclusion of one-particle-hole excitation. The impurity spectral function is determined in the real-frequency domain, avoiding any potential errors due to the numerical analytic continuation in previous TTT-matrix calculations and the small spectral broadening parameter used in variational calculations. In the weak-coupling limit, we find that the quasiparticle decay rate of both attractive and repulsive polarons does not increase significantly with increasing temperature, and therefore Fermi polarons may remain well defined far above Fermi degeneracy. In contrast, near the unitary limit with strong coupling, the decay rate of Fermi polarons rapidly increases and the quasiparticle picture breaks down close to the Fermi temperature. We analyze in detail the recent ejection and injection radio-frequency (rf) spectroscopy measurements, performed at Massachusetts Institute of Technology (MIT) and at the European Laboratory for Non-Linear Spectroscopy (LENS), respectively. We show that the momentum average of the spectral function, which is necessary to account for the observed rf spectroscopy, has a sizable contribution to the width of the quasiparticle peak in spectroscopy. As a result, the measured decay rate of Fermi polarons could be significantly larger than the calculated quasiparticle decay rate at zero momentum. By taking this crucial contribution into account, we find that there is a reasonable agreement between theory and experiment for the lifetime of Fermi polarons in the strong-coupling regime, as long as they remain well defined.
By using a non-self-consistent many-body TTT-matrix theory, we calculate the finite-temperature Raman spectroscopy of a mobile impurity immersed in a Fermi bath in three dimensions. The dependencies of the Raman spectrum on the transferred momentum, temperature, and impurity-bath interaction are discussed in detail. We confirm that the peak in the Raman spectrum shows a weaker dependence on the impurity concentration than that in the radio-frequency spectroscopy due to the nonzero transferred momentum, as anticipated. We compare our theoretical prediction with the recent measurement by Gal Ness et al. [G. Ness, C. Shkedrov, Y. Florshaim, O. K. Diessel, J. von Milczewski, R. Schmidt, and Y. Sagi, Phys. Rev. X 10, 041019 (2020)] without any adjustable parameters. At weak coupling, we find a good quantitative agreement. However, close to the Feshbach resonance the agreement becomes worse. At strong coupling, we find that an unrealistic Fermi bath temperature might be needed to account for the experimental data.
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We theoretically examine the finite-temperature spectral function of Fermi polarons in three dimensions by using a self-consistent many-body TTT-matrix theory in real frequency. In comparison with the previous results from a non-self-consistent many-body TTT-matrix approach, we show that the treatment of self-consistency in the impurity Green's function leads to notable changes in almost all the dynamical quantities, including the vertex function, impurity self-energy, and spectral function. Eventually, it gives rise to quantitatively different predictions for the measurable radio-frequency spectrum and Raman spectrum at finite temperature. Using the recent spectroscopic measurements as a benchmark, we find that the self-consistent many-body TTT-matrix theory somehow provides a better explanation for the experimental data. The notable difference in the predictions from the non-self-consistent and self-consistent theories suggests that more accurate theoretical descriptions are needed in order to fully account for the current spectroscopic observations on Fermi polarons.
We study theoretically the lifetimes of attractive and repulsive Fermi polarons, as well as the molecule at finite momentum in three dimensions. To this end, we develop a technique that allows for the computation of Green's functions in the whole complex frequency plane using exact analytical continuation within the functional renormalization group. The improved numerical stability and reduced computational cost of this method yield access to previously inaccessible momentum-dependent quasiparticle properties of low-lying excited states. While conventional approaches like the non-self-consistent T -matrix approximation method cannot determine these lifetimes, we are able to find the momentum-dependent lifetime at different interaction strengths of both the attractive and repulsive polaron as well as the molecule. At weak coupling our results confirm predictions made from effective Fermi liquid theory regarding the decay of the attractive polaron, and we demonstrate that Fermi liquidlike behavior extends far into the strong-coupling regime where the attractive polaron and molecule exhibit a p 4 momentum scaling in their decay widths. Our results offer an intriguing insight into the momentum-dependent quasiparticle properties of the Fermi polaron problem, which can be measured using techniques such as Raman transfer and Ramsey interferometry. Published by the American Physical Society 2024
We present a theory of radio-frequency spectroscopy of impurities interacting with a quantum gas at finite temperature. By working in the canonical ensemble of a single impurity, we show that the impurity spectral response is directly connected to the finite-temperature equation of state (free energy) of the impurity. We consider two different response protocols: injection, where the impurity is introduced into the medium from an initially noninteracting state, and ejection, where the impurity is ejected from an initially interacting state with the medium. We show that there is a simple mapping between injection and ejection spectra, which is connected to the detailed balance condition in thermal equilibrium. To illustrate the power of our approach, we specialize to the case of the Fermi polaron, corresponding to an impurity atom that is immersed in a noninteracting Fermi gas. For a mobile impurity with a mass equal to the fermion mass, we employ a finite-temperature variational approach to obtain the impurity spectral response. We find a striking nonmonotonic dependence on temperature in the impurity free energy, the contact, and the radio-frequency spectra. For the case of an infinitely heavy Fermi polaron, we derive exact results for the finite-temperature free energy, thus generalizing Fumi's theorem to arbitrary temperature. We also determine the exact dynamics of the contact after a quench of the impurity-fermion interactions. Finally, we show that the injection and ejection spectra obtained from the variational approach compare well with the exact spectra, thus demonstrating the accuracy of our approximation method.
The Fermi polaron, formed by an impurity interacting with a surrounding Fermi sea, exemplifies the canonical quasiparticle concept as a cornerstone in our description of quantum many-body systems across a wide range of energy scales. Experiments on atomic quantum gases have provided profound insights into the universal nature of the Fermi polaron. While most previous studies have focused on the case of zero impurity momentum, finite-momentum properties have remained largely uncharted. Here, we investigate the moving Fermi polaron by combining a novel Raman acceleration scheme with high-precision radio-frequency spectroscopy, exploring the quasiparticle dispersion relation over a wide range of momenta. We compare our measurements of energy shifts and spectral linewidths with a microscopic theory and reach quantitative agreement for all momenta. For low momenta, we find the energy of the moving polaron to be fully consistent with the Fermi liquid picture of a dressed particle with a constant effective mass. At high momenta, the polaron approaches the behavior of a weakly interacting bare particle, featuring small energy shifts and weak broadening. For intermediate momenta, broadening is generally larger and, most strikingly, the behavior differs for attractive and repulsive polarons. While the repulsive polaron exhibits a smooth connection between both regimes along with a monotonic change of the energy shift, the attractive case shows a peculiar non-monotonic behavior. With increasing momentum, the attractive polaron enters a regime where its energy deviates from the constant effective mass expression and broadening suddenly increases. By comparing this observation with theory, we show that this abrupt behavior coincides with the attractive polaron entering a molecule-hole continuum, where it is no longer the ground state. We interpret this as a motion-induced polaron-molecule transition.