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arXiv:2212.00182 · Physical Review A

Raman spectroscopy of Fermi polarons

Hui Hu, Xia-Ji Liu

Published Dec 12, 2022• 6 citations
arXivHTMLPDF

Abstract

By using a non-self-consistent many-body $T$-matrix theory, we calculate the finite-temperature Raman spectroscopy of a mobile impurity immersed in a Fermi bath in three dimensions. The dependencies of the Raman spectrum on the transferred momentum, temperature, and impurity-bath interaction are discussed in detail. We confirm that the peak in the Raman spectrum shows a weaker dependence on the impurity concentration than that in the radio-frequency spectroscopy due to the nonzero transferred momentum, as anticipated. We compare our theoretical prediction with the recent measurement by Gal Ness et al. [G. Ness, C. Shkedrov, Y. Florshaim, O. K. Diessel, J. von Milczewski, R. Schmidt, and Y. Sagi, Phys. Rev. X 10, 041019 (2020)] without any adjustable parameters. At weak coupling, we find a good quantitative agreement. However, close to the Feshbach resonance the agreement becomes worse. At strong coupling, we find that an unrealistic Fermi bath temperature might be needed to account for the experimental data.

DOI
10.1103/physreva.106.063306

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By using a non-self-consistent many-body TTT-matrix theory, we calculate the finite-temperature Raman spectroscopy of a mobile impurity immersed in a Fermi bath in three dimensions. The dependencies of the Raman spectrum on the transferred momentum, temperature, and impurity-bath interaction are discussed in detail. We confirm that the peak in the Raman spectrum shows a weaker dependence on the impurity concentration than that in the radio-frequency spectroscopy due to the nonzero transferred momentum, as anticipated. We compare our theoretical prediction with the recent measurement by Gal Ness et al. [G. Ness, C. Shkedrov, Y. Florshaim, O. K. Diessel, J. von Milczewski, R. Schmidt, and Y. Sagi, Phys. Rev. X 10, 041019 (2020)] without any adjustable parameters. At weak coupling, we find a good quantitative agreement. However, close to the Feshbach resonance the agreement becomes worse. At strong coupling, we find that an unrealistic Fermi bath temperature might be needed to account for the experimental data.
We present a systematic study of a mobile impurity immersed in a three-dimensional Fermi sea of fermions at finite temperature, by using the standard non-self-consistent many-body TTT-matrix theory that is equivalent to a finite-temperature variational approach with the inclusion of one-particle-hole excitation. The impurity spectral function is determined in the real-frequency domain, avoiding any potential errors due to the numerical analytic continuation in previous TTT-matrix calculations and the small spectral broadening parameter used in variational calculations. In the weak-coupling limit, we find that the quasiparticle decay rate of both attractive and repulsive polarons does not increase significantly with increasing temperature, and therefore Fermi polarons may remain well defined far above Fermi degeneracy. In contrast, near the unitary limit with strong coupling, the decay rate of Fermi polarons rapidly increases and the quasiparticle picture breaks down close to the Fermi temperature. We analyze in detail the recent ejection and injection radio-frequency (rf) spectroscopy measurements, performed at Massachusetts Institute of Technology (MIT) and at the European Laboratory for Non-Linear Spectroscopy (LENS), respectively. We show that the momentum average of the spectral function, which is necessary to account for the observed rf spectroscopy, has a sizable contribution to the width of the quasiparticle peak in spectroscopy. As a result, the measured decay rate of Fermi polarons could be significantly larger than the calculated quasiparticle decay rate at zero momentum. By taking this crucial contribution into account, we find that there is a reasonable agreement between theory and experiment for the lifetime of Fermi polarons in the strong-coupling regime, as long as they remain well defined.
We theoretically examine the finite-temperature spectral function of Fermi polarons in three dimensions by using a self-consistent many-body TTT-matrix theory in real frequency. In comparison with the previous results from a non-self-consistent many-body TTT-matrix approach, we show that the treatment of self-consistency in the impurity Green's function leads to notable changes in almost all the dynamical quantities, including the vertex function, impurity self-energy, and spectral function. Eventually, it gives rise to quantitatively different predictions for the measurable radio-frequency spectrum and Raman spectrum at finite temperature. Using the recent spectroscopic measurements as a benchmark, we find that the self-consistent many-body TTT-matrix theory somehow provides a better explanation for the experimental data. The notable difference in the predictions from the non-self-consistent and self-consistent theories suggests that more accurate theoretical descriptions are needed in order to fully account for the current spectroscopic observations on Fermi polarons.
We consider a spin impurity with multiple energy levels moving in a noninteracting Fermi sea and theoretically solve this Fermi-spin-polaron problem at nonzero temperature by using a non-self-consistent many-body TTT-matrix theory. We focus on the simplest case with spin 12\frac{1}{2}21​, where the two energy states of the impurity are coupled by a Rabi flip term. At small Rabi coupling, the impurity exhibits damped Rabi oscillations, where the decoherence is caused by the interaction with the Fermi sea, as recently reported in Fermi-polaron experiments with ultracold atoms. We investigate the dependence of Rabi oscillations on the Rabi coupling strength and examine the additional nonlinear damping due to large Rabi coupling. At finite temperature and nonzero impurity concentration, the impurity can acquire a pronounced momentum distribution. We show that the momentum or thermal average can sizably reduce the visibility of Rabi oscillations. We compare our theoretical predictions to recent experimental data and find good agreement without any adjustable parameters.
We theoretically investigate how quasiparticle properties of an attractive Fermi polaron are affected by nonzero temperature and finite impurity concentration in three dimensions and in free space. By applying both non-self-consistent and self-consistent many-body TTT-matrix theories, we calculate the polaron energy (including decay rate), effective mass, and residue, as functions of temperature and impurity concentration. The temperature and concentration dependencies are weak on the BCS side with a negative impurity-medium scattering length. Toward the strong attraction regime across the unitary limit, we find sizable dependencies. In particular, with increasing temperature the effective mass quickly approaches the bare mass and the residue is significantly enhanced. At temperature $T\ensuremath{\sim}0.1{T}_{F}$, where TF{T}_{F}TF​ is the Fermi temperature of the background Fermi sea, the residual polaron-polaron interaction seems to become attractive. This leads to a notable down-shift in the polaron energy. We show that, by taking into account the temperature and impurity concentration effects, the measured polaron energy in the first Fermi polaron experiment [Schirotzek , Phys. Rev. Lett. 102, 230402 (2009)] could be better theoretically explained.
The Fermi polaron, formed by an impurity interacting with a surrounding Fermi sea, exemplifies the canonical quasiparticle concept as a cornerstone in our description of quantum many-body systems across a wide range of energy scales. Experiments on atomic quantum gases have provided profound insights into the universal nature of the Fermi polaron. While most previous studies have focused on the case of zero impurity momentum, finite-momentum properties have remained largely uncharted. Here, we investigate the moving Fermi polaron by combining a novel Raman acceleration scheme with high-precision radio-frequency spectroscopy, exploring the quasiparticle dispersion relation over a wide range of momenta. We compare our measurements of energy shifts and spectral linewidths with a microscopic theory and reach quantitative agreement for all momenta. For low momenta, we find the energy of the moving polaron to be fully consistent with the Fermi liquid picture of a dressed particle with a constant effective mass. At high momenta, the polaron approaches the behavior of a weakly interacting bare particle, featuring small energy shifts and weak broadening. For intermediate momenta, broadening is generally larger and, most strikingly, the behavior differs for attractive and repulsive polarons. While the repulsive polaron exhibits a smooth connection between both regimes along with a monotonic change of the energy shift, the attractive case shows a peculiar non-monotonic behavior. With increasing momentum, the attractive polaron enters a regime where its energy deviates from the constant effective mass expression and broadening suddenly increases. By comparing this observation with theory, we show that this abrupt behavior coincides with the attractive polaron entering a molecule-hole continuum, where it is no longer the ground state. We interpret this as a motion-induced polaron-molecule transition.
We theoretically analyze inverse radio-frequency (rf) spectroscopy experiments in two-component Fermi gases. We consider a small number of impurity atoms interacting strongly with a bath of majority atoms. In two-dimensional geometries we find that the main features of the rf spectrum correspond to an attractive polaron and a metastable repulsive polaron. Our results suggest that the attractive polaron has been observed in a recent experiment [B. Fr\"ohlich et al., Phys. Rev. Lett. 106, 105301 (2011)].