Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Log inSign up
Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Blog
Job Board
Q3AS

© 2026 Aqora Quantum S.A.S.

TermsPrivacyLegal Notice

arXiv:2211.01765 · AAPPS bulletin

Functional determinant approach investigations of heavy impurity physics

Jia Wang

Published Sep 26, 2023• 12 citations
arXivHTMLPDF

Abstract

Abstract In this brief review, we report some new development in the functional determinant approach (FDA), an exact numerical method, in the studies of a heavy quantum impurity immersed in Fermi gases and manipulated with radio-frequency pulses. FDA has been successfully applied to investigate the universal dynamical responses of a heavy impurity in an ultracold ideal Fermi gas in both the time and frequency domain, which allows the exploration of the renowned Anderson’s orthogonality catastrophe (OC). In such a system, OC is induced by the multiple particle-hole excitations of the Fermi sea, which is beyond a simple perturbation picture and manifests itself as the absence of quasiparticles named polarons. More recently, two new directions for studying heavy impurity with FDA have been developed. One is to extend FDA to a strongly correlated background superfluid background, a Bardeen–Cooper–Schrieffer (BCS) superfluid. In this system, Anderson’s orthogonality catastrophe is prohibited due to the suppression of multiple particle-hole excitations by the superfluid gap, which leads to the existence of genuine polaron. The other direction is to generalize the FDA to the case of multiple RF pulses scheme, which extends the well-established 1D Ramsey spectroscopy in ultracold atoms into multidimensional, in the same spirit as the well-known multidimensional nuclear magnetic resonance and optical multidimensional coherent spectroscopy. Multidimensional Ramsey spectroscopy allows us to investigate correlations between spectral peaks of an impurity-medium system that is not accessible in the conventional one-dimensional spectrum.

DOI
10.1007/s43673-023-00092-5

Related papers

Heavy polarons in ultracold atomic Fermi superfluids at the BEC-BCS crossover: Formalism and applications

Jia Wang, Xia-Ji Liu, Hui Hu

We investigate the system of a heavy impurity embedded in a paired two-component Fermi gas at the crossover from a Bose-Einstein condensate (BEC) to a Bardeen-Cooper-Schrieffer (BCS) superfluid via an extension of the functional determinant approach (FDA). FDA is an exact numerical approach applied to study manifestations of Anderson's orthogonality catastrophe (OC) in the system of a static impurity immersed in an ideal Fermi gas. Here, we extend the FDA to a strongly correlated superfluid background described by a BCS mean-field wave function. In contrast to the ideal Fermi gas case, the pairing gap in the BCS superfluid prevents the OC and leads to genuine polaron signals in the spectrum. Thus our exactly solvable model can provide a deeper understanding of polaron physics. In addition, we find that the polaron spectrum can be used to measure the superfluid pairing gap, and in the case of a magnetic impurity, the energy of the subgap Yu-Shiba-Rusinov (YSR) bound state. Our theoretical predictions can be examined with state-of-art cold-atom experiments.

arXiv:2202.05363•Physical Review A•Apr 26, 2022•32 citations

Multidimensional spectroscopy of heavy impurities in ultracold fermions

Jia Wang

We investigate the system of a heavy impurity immersed in a degenerate Fermi gas, where the impurity's internal degree of freedom (pseudospin) is manipulated by a series of radio-frequency (RF) pulses at several different times. Applying the functional determinant approach, we carry out an essentially exact calculation of the Ramsey-interference-type responses to the RF pulses. These responses can be regarded as multidimensional (MD) spectroscopy of the system in the time domain. Similar to their one-dimensional counterpart studied by Knap et al. [M. Knap et al., Phys. Rev. X 2, 041020 (2012)], these responses are universal functions. A Fourier transformation of the time intervals gives the MD spectroscopy in the frequency domain, providing insightful information on the many-body correlation and relaxation via the cross peaks, e.g., the off-diagonal peaks in a two-dimensional spectrum. These features are inaccessible for the conventional, one-dimensional absorption spectrum. Our scheme provides a different method to investigate many-body nonequilibrium physics beyond the linear response regime with accessible tools in cold atoms.

arXiv:2207.10501•Physical Review A•Jan 12, 2023•11 citations

Exact Quasiparticle Properties of a Heavy Polaron in BCS Fermi Superfluids

Jia Wang, Xia-Ji Liu, Hui Hu

We present the Ramsey response and radio-frequency spectroscopy of a heavy impurity immersed in an interacting Fermi superfluid, using the exact functional determinant approach. We describe the Fermi superfluid through the conventional Bardeen-Cooper-Schrieffer theory and investigate the role of the pairing gap on quasiparticle properties revealed by the two spectroscopies. The energy cost for pair breaking prevents Anderson's orthogonality catastrophe that occurs in a noninteracting Fermi gas and allows the existence of polaron quasiparticles in the exactly solvable heavy impurity limit. Hence, we rigorously confirm the remarkable features such as dark continuum, molecule-hole continuum, and repulsive polaron. For a magnetic impurity scattering at finite temperature, we predict additional resonances related to the subgap Yu-Shiba-Rusinov bound state, whose positions can be used to measure the superfluid pairing gap. For a nonmagnetic scattering at zero temperature, we surprisingly find undamped repulsive polarons. These exact results might be readily observed in quantum gas experiments with Bose-Fermi mixtures that have a large-mass ratio.

arXiv:2202.05366•Physical Review Letters•Apr 26, 2022•28 citations

Universal many-body response of heavy impurities coupled to a Fermi sea: a review of recent progress

Richard Schmidt, Michael Knap, Dmitri A. Ivanov +3 more

In this report we discuss the dynamical response of heavy quantum impurities immersed in a Fermi gas at zero and at finite temperature. Studying both the frequency and the time domain allows one to identify interaction regimes that are characterized by distinct many-body dynamics. From this theoretical study a picture emerges in which impurity dynamics is universal on essentially all time scales, and where the high-frequency few-body response is related to the long-time dynamics of the Anderson orthogonality catastrophe by Tan relations. Our theoretical description relies on different and complementary approaches: functional determinants give an exact numerical solution for time- and frequency-resolved responses, bosonization provides accurate analytical expressions at low temperatures, and the theory of Toeplitz determinants allows one to analytically predict response up to high temperatures. Using these approaches we predict the thermal decoherence rate of the fermionic system and prove that within the considered model the fastest rate of long-time decoherence is given by [Formula: see text]. We show that Feshbach resonances in cold atomic systems give access to new interaction regimes where quantum effects can prevail even in the thermal regime of many-body dynamics. The key signature of this phenomenon is a crossover between different exponential decay rates of the real-time Ramsey signal. It is shown that the physics of the orthogonality catastrophe is experimentally observable up to temperatures [Formula: see text] where it leaves its fingerprint in a power-law temperature dependence of thermal spectral weight and we review how this phenomenon is related to the physics of heavy ions in liquid [Formula: see text]He and the formation of Fermi polarons. The presented results are in excellent agreement with recent experiments on LiK mixtures, and we predict several new phenomena that can be tested using currently available experimental technology.

arXiv:1702.08587•Reports on Progress in Physics•Jan 5, 2018•205 citations

Mass-gap functional determinant approach for mobile Fermi polarons

Emilio Ramos Rodríguez, Eugen Dizer, Xin Chen +1 more

We extend the functional determinant approach (FDA), previously restricted to static impurities, to the case of finite-mass impurities by using the mass-gap description of Fermi polarons [Phys. Rev. Lett. 135, 193401 (2025)]. The quadratic structure of the mass-gap model enables the exact evaluation of many-body spectra and Ramsey dynamics for mobile impurities. We show that this mass-gap FDA smoothly interpolates between the Fermi-edge singularity for infinitely heavy impurities and the emergence of quasiparticle weight for finite impurity mass. Our results demonstrate that the mass-gap FDA provides a transparent and computationally efficient framework to describe the quantum dynamics of mobile impurities.

cond-mat.quant-gasCross-listedarXiv:2608.30539•Sep 1, 2026•0 citations

Probing Bardeen-Cooper-Schrieffer Pairing and Quasiparticle Formation in Ultracold Gases by Rydberg Atom Spectroscopy

Elizabeth Rodríguez, Marcel Gievers, Richard Schmidt

Locally probing pairing in fermionic superfluids, ranging from micro- to macroscopic scales, has been a long-standing challenge. Here, we investigate a new approach that uses Rydberg impurities as a spectroscopic sensor of the surrounding strongly correlated state of ultracold paired fermions. The extended wave function of the Rydberg electron induces a finite-range potential that can bind atoms from the BCS medium, forming molecular states. As a consequence, the optical absorption spectrum of the impurity encodes key many-body properties. Using the functional determinant approach, we provide a direct measure of the superfluid gap through frequency shifts of dimer and trimer peaks. The spectra also reveal whether the Cooper pairs are broken or trapped intact. For static Rydberg atoms, we relate this signature of pairing to the suppression of the orthogonality catastrophe due to the superconducting gap resulting in the formation of well-defined polaron quasiparticles. Our Letter establishes Rydberg atom spectroscopy as a powerful local probe of strongly correlated matter.

arXiv:2511.19191•Physical Review Letters•Apr 28, 2026•1 citation
Abstract In this brief review, we report some new development in the functional determinant approach (FDA), an exact numerical method, in the studies of a heavy quantum impurity immersed in Fermi gases and manipulated with radio-frequency pulses. FDA has been successfully applied to investigate the universal dynamical responses of a heavy impurity in an ultracold ideal Fermi gas in both the time and frequency domain, which allows the exploration of the renowned Anderson’s orthogonality catastrophe (OC). In such a system, OC is induced by the multiple particle-hole excitations of the Fermi sea, which is beyond a simple perturbation picture and manifests itself as the absence of quasiparticles named polarons. More recently, two new directions for studying heavy impurity with FDA have been developed. One is to extend FDA to a strongly correlated background superfluid background, a Bardeen–Cooper–Schrieffer (BCS) superfluid. In this system, Anderson’s orthogonality catastrophe is prohibited due to the suppression of multiple particle-hole excitations by the superfluid gap, which leads to the existence of genuine polaron. The other direction is to generalize the FDA to the case of multiple RF pulses scheme, which extends the well-established 1D Ramsey spectroscopy in ultracold atoms into multidimensional, in the same spirit as the well-known multidimensional nuclear magnetic resonance and optical multidimensional coherent spectroscopy. Multidimensional Ramsey spectroscopy allows us to investigate correlations between spectral peaks of an impurity-medium system that is not accessible in the conventional one-dimensional spectrum.
We investigate the system of a heavy impurity embedded in a paired two-component Fermi gas at the crossover from a Bose-Einstein condensate (BEC) to a Bardeen-Cooper-Schrieffer (BCS) superfluid via an extension of the functional determinant approach (FDA). FDA is an exact numerical approach applied to study manifestations of Anderson's orthogonality catastrophe (OC) in the system of a static impurity immersed in an ideal Fermi gas. Here, we extend the FDA to a strongly correlated superfluid background described by a BCS mean-field wave function. In contrast to the ideal Fermi gas case, the pairing gap in the BCS superfluid prevents the OC and leads to genuine polaron signals in the spectrum. Thus our exactly solvable model can provide a deeper understanding of polaron physics. In addition, we find that the polaron spectrum can be used to measure the superfluid pairing gap, and in the case of a magnetic impurity, the energy of the subgap Yu-Shiba-Rusinov (YSR) bound state. Our theoretical predictions can be examined with state-of-art cold-atom experiments.
We investigate the system of a heavy impurity immersed in a degenerate Fermi gas, where the impurity's internal degree of freedom (pseudospin) is manipulated by a series of radio-frequency (RF) pulses at several different times. Applying the functional determinant approach, we carry out an essentially exact calculation of the Ramsey-interference-type responses to the RF pulses. These responses can be regarded as multidimensional (MD) spectroscopy of the system in the time domain. Similar to their one-dimensional counterpart studied by Knap et al. [M. Knap et al., Phys. Rev. X 2, 041020 (2012)], these responses are universal functions. A Fourier transformation of the time intervals gives the MD spectroscopy in the frequency domain, providing insightful information on the many-body correlation and relaxation via the cross peaks, e.g., the off-diagonal peaks in a two-dimensional spectrum. These features are inaccessible for the conventional, one-dimensional absorption spectrum. Our scheme provides a different method to investigate many-body nonequilibrium physics beyond the linear response regime with accessible tools in cold atoms.
We present the Ramsey response and radio-frequency spectroscopy of a heavy impurity immersed in an interacting Fermi superfluid, using the exact functional determinant approach. We describe the Fermi superfluid through the conventional Bardeen-Cooper-Schrieffer theory and investigate the role of the pairing gap on quasiparticle properties revealed by the two spectroscopies. The energy cost for pair breaking prevents Anderson's orthogonality catastrophe that occurs in a noninteracting Fermi gas and allows the existence of polaron quasiparticles in the exactly solvable heavy impurity limit. Hence, we rigorously confirm the remarkable features such as dark continuum, molecule-hole continuum, and repulsive polaron. For a magnetic impurity scattering at finite temperature, we predict additional resonances related to the subgap Yu-Shiba-Rusinov bound state, whose positions can be used to measure the superfluid pairing gap. For a nonmagnetic scattering at zero temperature, we surprisingly find undamped repulsive polarons. These exact results might be readily observed in quantum gas experiments with Bose-Fermi mixtures that have a large-mass ratio.
In this report we discuss the dynamical response of heavy quantum impurities immersed in a Fermi gas at zero and at finite temperature. Studying both the frequency and the time domain allows one to identify interaction regimes that are characterized by distinct many-body dynamics. From this theoretical study a picture emerges in which impurity dynamics is universal on essentially all time scales, and where the high-frequency few-body response is related to the long-time dynamics of the Anderson orthogonality catastrophe by Tan relations. Our theoretical description relies on different and complementary approaches: functional determinants give an exact numerical solution for time- and frequency-resolved responses, bosonization provides accurate analytical expressions at low temperatures, and the theory of Toeplitz determinants allows one to analytically predict response up to high temperatures. Using these approaches we predict the thermal decoherence rate of the fermionic system and prove that within the considered model the fastest rate of long-time decoherence is given by [Formula: see text]. We show that Feshbach resonances in cold atomic systems give access to new interaction regimes where quantum effects can prevail even in the thermal regime of many-body dynamics. The key signature of this phenomenon is a crossover between different exponential decay rates of the real-time Ramsey signal. It is shown that the physics of the orthogonality catastrophe is experimentally observable up to temperatures [Formula: see text] where it leaves its fingerprint in a power-law temperature dependence of thermal spectral weight and we review how this phenomenon is related to the physics of heavy ions in liquid [Formula: see text]He and the formation of Fermi polarons. The presented results are in excellent agreement with recent experiments on LiK mixtures, and we predict several new phenomena that can be tested using currently available experimental technology.
We extend the functional determinant approach (FDA), previously restricted to static impurities, to the case of finite-mass impurities by using the mass-gap description of Fermi polarons [Phys. Rev. Lett. 135, 193401 (2025)]. The quadratic structure of the mass-gap model enables the exact evaluation of many-body spectra and Ramsey dynamics for mobile impurities. We show that this mass-gap FDA smoothly interpolates between the Fermi-edge singularity for infinitely heavy impurities and the emergence of quasiparticle weight for finite impurity mass. Our results demonstrate that the mass-gap FDA provides a transparent and computationally efficient framework to describe the quantum dynamics of mobile impurities.
Locally probing pairing in fermionic superfluids, ranging from micro- to macroscopic scales, has been a long-standing challenge. Here, we investigate a new approach that uses Rydberg impurities as a spectroscopic sensor of the surrounding strongly correlated state of ultracold paired fermions. The extended wave function of the Rydberg electron induces a finite-range potential that can bind atoms from the BCS medium, forming molecular states. As a consequence, the optical absorption spectrum of the impurity encodes key many-body properties. Using the functional determinant approach, we provide a direct measure of the superfluid gap through frequency shifts of dimer and trimer peaks. The spectra also reveal whether the Cooper pairs are broken or trapped intact. For static Rydberg atoms, we relate this signature of pairing to the suppression of the orthogonality catastrophe due to the superconducting gap resulting in the formation of well-defined polaron quasiparticles. Our Letter establishes Rydberg atom spectroscopy as a powerful local probe of strongly correlated matter.