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arXiv:2403.11142 · Physical Review Research

Dynamics and resonance fluorescence from a superconducting artificial atom doubly driven by quantized and classical fields

Xinhui Ruan, Jia-Heng Wang, Dong He, Pengtao Song, Shengyong Li, Qianchuan Zhao, Le‐Man Kuang, Jaw-Shen Tsai, Chang‐Ling Zou, Jing Zhang, Dongning Zheng, O. V. Astafiev, Yu-xi Liu, Zhihui Peng

Published Jul 15, 2024• 4 citations
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Abstract

We report an experimental demonstration of resonance fluorescence in a two-level superconducting artificial atom under two driving fields coupled to a detuned cavity. One of the fields is classical and the other is varied from quantum (vacuum fluctuations) to classical by controlling the photon number inside the cavity. The device consists of a transmon qubit strongly coupled to a one-dimensional transmission line and a coplanar waveguide resonator. We observe a sideband anticrossing and asymmetry in the emission spectra of the system through a one-dimensional transmission line, which is fundamentally different from the weak-coupling case. By changing the photon number inside the cavity, the emission spectrum of our doubly driven system approaches the case when the atom is driven by two classical bichromatic fields. We also measure the dynamical evolution of the system through the transmission line and study the properties of the first-order correlation function, Rabi oscillations, and energy relaxation in the system. The study of resonance fluorescence from an atom driven by two fields promotes understanding decoherence in superconducting quantum circuits and may find applications in superconducting quantum computing and quantum networks. Published by the American Physical Society 2024

DOI
10.1103/physrevresearch.6.033064

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We experimentally demonstrate the resonance fluorescence of a two-level artificial atom strongly coupled to a single-mode cavity field. The effect was theoretically predicted thirty years ago by Savage [Phys. Rev. Lett. 63, 1376 (1989)]. The system consists of a superconducting qubit circuit and a one-dimensional transmission line resonator. In addition, a one-dimensional transmission line strongly coupled to the atom serves as an open space. The effect takes place, when a microwave field is applied to the cavity, which in turn is resonantly coupled to the atom. The fluorescence spectrum is measured via the emission into the transmission line. We find that the central peak is determined by the atom spontaneous emission to the open space and the widths of side peaks are largely determined by the coherent interaction between the atom and the cavity, that is, the fluorescence spectrum here is very different from that of the Mollow triplet. We also derive analytical form for the spectrum. Our experimental results agree well with theoretical calculations.
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Abstract The coherent interaction between a two-level system and electromagnetic fields serves as a foundation for fundamental quantum physics and modern photonic quantum technology. A profound example is resonance fluorescence, where the non-classical photon emission appears in the form of a Mollow-triplet when a two-level system is continuously driven by a resonant laser. Pushing resonance fluorescence from a static to dynamic regime by using short optical pulses generates on-demand emissions of highly coherent single photons. Further increasing the driving strength in the dynamical regime enables the pursuit of exotic non-classical light emission in photon number superposition, photon number entanglement, and photon bundle states. However, the long-sought-after spectrum beyond the Mollow-triplet, a characteristic of dynamic resonance fluorescence under strong driving strength, has not been observed yet. Here we report the direct observation and systematic investigations of dynamic resonance fluorescence spectra beyond the Mollow-triplet in a solid-state cavity quantum electrodynamic system. The dynamic resonance fluorescence spectra with up to five pairs of side peaks, excitation detuning induced spectral asymmetry, and cavity filtering effect are observed and quantitatively modeled by a full quantum model with phonon scattering included. Time-resolved measurements further reveal that the multiple side peaks originate from interference of the emission associated with different temporal positions of the excitation pulses. Our work facilitates the generation of a variety of exotic quantum states of light with dynamic driving of two-level systems.
Multiphoton emitters are a sought-after resource in quantum photonics. Nonlinear interactions between a multilevel atomic system and a coherent drive can lead to resonant two-photon emission, but harvesting light from this process has remained a challenge due to the small oscillator strengths involved. Here we present a study of two-photon resonance fluorescence at microwave frequencies, using a superconducting, ladder-type artificial atom, a transmon, strongly coupled to a waveguide. We drive the two-photon transition between the ground and second-excited states at increasingly high powers and observe a resonance fluorescence peak whose intensity becomes comparable to single-photon emission until it splits into a Mollow-like triplet. We measure photon correlations of frequency-filtered spectral lines and find that while emission at the fundamental frequency stays antibunched, the resonance fluorescence peak at the two-photon transition is superbunched. Our results provide a route towards the realization of multiphoton sources in the microwave domain.
An electromagnetic wave propagating through a waveguide with a strongly coupled two-level superconducting artificial atom exhibits an evolving superposition with the atom. The Rabi oscillations in the atom result from a single excitation-relaxation, corresponding to photon absorption and stimulated emission from and to the field. In this study, we experimentally investigated the time-dependent behavior of the field transmitted through a waveguide with a strongly coupled transmon. The scattered fields agree well with the predictions of the input-output theory. We demonstrate that the time evolution of the propagating fields, because of the interaction, encapsulates all information about the atom. Furthermore, we deduced the dynamics of the incoherent radiation component from the first-order correlation function of the measured field.