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arXiv:2212.11400 · Physical Review X

Resonance Fluorescence of a Chiral Artificial Atom

Chaitali Joshi, Frank Yang, Mohammad Mirhosseini

Published Jun 26, 2023• 100 citations
arXivHTMLPDF

Abstract

We demonstrate a superconducting artificial atom with strong unidirectional coupling to a microwave photonic waveguide.Our artificial atom is realized by coupling a transmon qubit to the waveguide at two spatially separated points with time-modulated interactions.Direction-sensitive interference arising from the parametric couplings in our scheme results in a nonreciprocal response, where we measure a forward/backward ratio of spontaneous emission exceeding 100.We verify the quantum nonlinear behavior of this artificial chiral atom by measuring the resonance fluorescence spectrum under a strong resonant drive and observing well-resolved Mollow triplets.Further, we demonstrate chirality for the second transition energy of the artificial atom and control it with a pulse sequence to realize a qubit-state-dependent nonreciprocal phase on itinerant photons.Our demonstration puts forth a superconducting hardware platform for the scalable realization of several key functionalities pursued within the paradigm of chiral quantum optics, including quantum networks with all-to-all connectivity, driven-dissipative stabilization of many-body entanglement, and the generation of complex nonclassical states of light.

DOI
10.1103/physrevx.13.021039

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We demonstrate a superconducting artificial atom with strong unidirectional coupling to a microwave photonic waveguide.Our artificial atom is realized by coupling a transmon qubit to the waveguide at two spatially separated points with time-modulated interactions.Direction-sensitive interference arising from the parametric couplings in our scheme results in a nonreciprocal response, where we measure a forward/backward ratio of spontaneous emission exceeding 100.We verify the quantum nonlinear behavior of this artificial chiral atom by measuring the resonance fluorescence spectrum under a strong resonant drive and observing well-resolved Mollow triplets.Further, we demonstrate chirality for the second transition energy of the artificial atom and control it with a pulse sequence to realize a qubit-state-dependent nonreciprocal phase on itinerant photons.Our demonstration puts forth a superconducting hardware platform for the scalable realization of several key functionalities pursued within the paradigm of chiral quantum optics, including quantum networks with all-to-all connectivity, driven-dissipative stabilization of many-body entanglement, and the generation of complex nonclassical states of light.
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We present an experimental realization of resonance fluorescence in squeezed vacuum.We strongly couple microwave-frequency squeezed light to a superconducting artificial atom and detect the resulting fluorescence with high resolution enabled by a broadband traveling-wave parametric amplifier.We investigate the fluorescence spectra in the weak and strong driving regimes, observing up to 3.1 dB of reduction of the fluorescence linewidth below the ordinary vacuum level and a dramatic dependence of the Mollow triplet spectrum on the relative phase of the driving and squeezed vacuum fields.Our results are in excellent agreement with predictions for spectra produced by a two-level atom in squeezed vacuum [Phys.Rev. Lett.58, 2539 (1987)], demonstrating that resonance fluorescence offers a resource-efficient means to characterize squeezing in cryogenic environments.
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We address recent advances in quantum optics with propagating microwaves\nin superconducting circuits. This research field exploits on the fact that the coupling between a superconducting artificial atom and propagating microwave photons in a one-dimensional (1D) open transmission line can be made strong enough to observe quantum effects, without using any cavity to confine the microwave photons.\nWe embed an artificial atom, a superconducting transmon qubit, in a 1D open\ntransmission line and investigate the scattering properties of coherent microwaves. When an input coherent state, with an average photon number much less than 1, is on resonance with the artificial atom, we observe extinction of up to 99% in the forward propagating field. We observe the strong nonlinearity of the artificial atom and under strong driving we observe the Mollow triplet. We also study the statistics of the reflected and transmitted beams, which are predicted to be nonclassical states. In particular, we demonstrate photon antibunching in the reflected beam by measuring the second-order correlation function. By applying a second control tone, we observe the Autler-Townes splitting and a giant cross-Kerr effect.\nFurthermore, we demonstrate fast operation of a single-photon router using\nthe Autler-Townes splitting. This device provides important steps towards the realization of a quantum network. This thesis describes the motivation, theoretical background, design, implementation and measurement results.
Experiments utilizing quantum optics have progressed rapidly in last few decades, particularly in the context of quantum computation, simulation, and communication. Early work in this field focused on implementations of cavity quantum electrodynamics (QED), where atoms, either natural or artificial, are strongly coupled to the confined photonic modes of cavities. However, in recent years, achieving strong coupling between atoms and itinerant photons has also gained significant interest for its applications in quantum networking. To this end, many atomic platforms are attempting to realize the waveguide QED architecture: atoms that interact with the continua of propagating photonic modes within a waveguide. In this thesis, we realize the strong-coupling regime of a waveguide QED architecture by coupling superconducting artificial atoms, typically operated as qubits, to one-dimensional transmission lines. We first demonstrate that superconducting qubits in a waveguide QED system can be used as high-quality quantum emitters. We then leverage the quantum interference between the simultaneous emission from multiple qubits in order to generate non-classical, spatially entangled, and directional itinerant microwave photons. These types of photons are particularly useful for remote entanglement and quantum communication protocols. Finally, we demonstrate that superconducting qubits can be engineered to enter novel regimes of light-matter interactions that are difficult, or even impossible, to achieve in other atomic platforms. In particular, we realize the giant-atom regime of waveguide QED, where the atom can no longer be treated as a point-like object. We use our giant atoms to implement tunable atom-waveguide couplings, as well as decoherence-free waveguide-mediated interactions between multiple atoms.