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arXiv:1901.00414 · Physical Review A

Two-photon resonance fluorescence of a ladder-type atomic system

Simone Gasparinetti, Jean-Claude Besse, Marek Pechal, Robin D. Buijs, Christopher Eichler, H. J. Carmichael, Andreas J. Wallraff

Published Sep 3, 2019• 15 citations
arXivHTMLPDF

Abstract

Multiphoton emitters are a sought-after resource in quantum photonics. Nonlinear interactions between a multilevel atomic system and a coherent drive can lead to resonant two-photon emission, but harvesting light from this process has remained a challenge due to the small oscillator strengths involved. Here we present a study of two-photon resonance fluorescence at microwave frequencies, using a superconducting, ladder-type artificial atom, a transmon, strongly coupled to a waveguide. We drive the two-photon transition between the ground and second-excited states at increasingly high powers and observe a resonance fluorescence peak whose intensity becomes comparable to single-photon emission until it splits into a Mollow-like triplet. We measure photon correlations of frequency-filtered spectral lines and find that while emission at the fundamental frequency stays antibunched, the resonance fluorescence peak at the two-photon transition is superbunched. Our results provide a route towards the realization of multiphoton sources in the microwave domain.

DOI
10.1103/physreva.100.033802

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Multiphoton emitters are a sought-after resource in quantum photonics. Nonlinear interactions between a multilevel atomic system and a coherent drive can lead to resonant two-photon emission, but harvesting light from this process has remained a challenge due to the small oscillator strengths involved. Here we present a study of two-photon resonance fluorescence at microwave frequencies, using a superconducting, ladder-type artificial atom, a transmon, strongly coupled to a waveguide. We drive the two-photon transition between the ground and second-excited states at increasingly high powers and observe a resonance fluorescence peak whose intensity becomes comparable to single-photon emission until it splits into a Mollow-like triplet. We measure photon correlations of frequency-filtered spectral lines and find that while emission at the fundamental frequency stays antibunched, the resonance fluorescence peak at the two-photon transition is superbunched. Our results provide a route towards the realization of multiphoton sources in the microwave domain.
We use a three-level artificial atom in the ladder configuration as a source of correlated, single microwave photons of different frequency. The artificial atom, a transmon-type superconducting circuit, is driven at the two-photon transition between ground and second-excited state, and embedded into an on-chip switch that selectively routes different-frequency photons into different spatial modes. Under continuous driving, we measure power cross-correlations between the two modes and observe a crossover between strong antibunching and superbunching, typical of cascade decay, and an oscillatory pattern as the drive strength becomes comparable to the radiative decay rate. By preparing the source in a superposition state using an excitation pulse, we achieve deterministic generation of entangled photon pairs, as demonstrated by nonvanishing phase correlations and more generally by joint quantum state tomography of the two itinerant photonic modes.
The coherent interaction between a two-level system and electromagnetic fields serves as a foundation for fundamental quantum physics and modern photonic quantum technology. A profound example is resonance fluorescence, where the non-classical photon emission appears in the form of a Mollow-triplet when a two-level system is continuously driven by a resonant laser. Pushing resonance fluorescence from a static to dynamic regime by using short optical pulses generates on-demand emissions of highly coherent single photons. Further increasing the driving strength in the dynamical regime enables the pursuit of exotic non-classical light emission in photon number superposition, photon number entanglement, and photon bundle states. However, the long-sought-after spectrum beyond the Mollow-triplet, a characteristic of dynamic resonance fluorescence under strong driving strength, has not been observed yet. Here we report the direct observation and systematic investigations of dynamic resonance fluorescence spectra beyond the Mollow-triplet in a solid-state cavity quantum electrodynamic system. The dynamic resonance fluorescence spectra with up to five pairs of side peaks, excitation detuning induced spectral asymmetry, and cavity filtering effect are observed and quantitatively modeled by a full quantum model with phonon scattering included. Time-resolved measurements further reveal that the multiple side peaks originate from interference of the emission associated with different temporal positions of the excitation pulses. Our work facilitates the generation of a variety of exotic quantum states of light with dynamic driving of two-level systems.
We experimentally demonstrate the resonance fluorescence of a two-level artificial atom strongly coupled to a single-mode cavity field. The effect was theoretically predicted thirty years ago by Savage [Phys. Rev. Lett. 63, 1376 (1989)]. The system consists of a superconducting qubit circuit and a one-dimensional transmission line resonator. In addition, a one-dimensional transmission line strongly coupled to the atom serves as an open space. The effect takes place, when a microwave field is applied to the cavity, which in turn is resonantly coupled to the atom. The fluorescence spectrum is measured via the emission into the transmission line. We find that the central peak is determined by the atom spontaneous emission to the open space and the widths of side peaks are largely determined by the coherent interaction between the atom and the cavity, that is, the fluorescence spectrum here is very different from that of the Mollow triplet. We also derive analytical form for the spectrum. Our experimental results agree well with theoretical calculations.
We demonstrate a superconducting artificial atom with strong unidirectional coupling to a microwave photonic waveguide.Our artificial atom is realized by coupling a transmon qubit to the waveguide at two spatially separated points with time-modulated interactions.Direction-sensitive interference arising from the parametric couplings in our scheme results in a nonreciprocal response, where we measure a forward/backward ratio of spontaneous emission exceeding 100.We verify the quantum nonlinear behavior of this artificial chiral atom by measuring the resonance fluorescence spectrum under a strong resonant drive and observing well-resolved Mollow triplets.Further, we demonstrate chirality for the second transition energy of the artificial atom and control it with a pulse sequence to realize a qubit-state-dependent nonreciprocal phase on itinerant photons.Our demonstration puts forth a superconducting hardware platform for the scalable realization of several key functionalities pursued within the paradigm of chiral quantum optics, including quantum networks with all-to-all connectivity, driven-dissipative stabilization of many-body entanglement, and the generation of complex nonclassical states of light.
Abstract The coherent interaction between a two-level system and electromagnetic fields serves as a foundation for fundamental quantum physics and modern photonic quantum technology. A profound example is resonance fluorescence, where the non-classical photon emission appears in the form of a Mollow-triplet when a two-level system is continuously driven by a resonant laser. Pushing resonance fluorescence from a static to dynamic regime by using short optical pulses generates on-demand emissions of highly coherent single photons. Further increasing the driving strength in the dynamical regime enables the pursuit of exotic non-classical light emission in photon number superposition, photon number entanglement, and photon bundle states. However, the long-sought-after spectrum beyond the Mollow-triplet, a characteristic of dynamic resonance fluorescence under strong driving strength, has not been observed yet. Here we report the direct observation and systematic investigations of dynamic resonance fluorescence spectra beyond the Mollow-triplet in a solid-state cavity quantum electrodynamic system. The dynamic resonance fluorescence spectra with up to five pairs of side peaks, excitation detuning induced spectral asymmetry, and cavity filtering effect are observed and quantitatively modeled by a full quantum model with phonon scattering included. Time-resolved measurements further reveal that the multiple side peaks originate from interference of the emission associated with different temporal positions of the excitation pulses. Our work facilitates the generation of a variety of exotic quantum states of light with dynamic driving of two-level systems.
We present an experimental realization of resonance fluorescence in squeezed vacuum.We strongly couple microwave-frequency squeezed light to a superconducting artificial atom and detect the resulting fluorescence with high resolution enabled by a broadband traveling-wave parametric amplifier.We investigate the fluorescence spectra in the weak and strong driving regimes, observing up to 3.1 dB of reduction of the fluorescence linewidth below the ordinary vacuum level and a dramatic dependence of the Mollow triplet spectrum on the relative phase of the driving and squeezed vacuum fields.Our results are in excellent agreement with predictions for spectra produced by a two-level atom in squeezed vacuum [Phys.Rev. Lett.58, 2539 (1987)], demonstrating that resonance fluorescence offers a resource-efficient means to characterize squeezing in cryogenic environments.