There have been impressive breakthroughs in semiconductor quantum dots in recent years, with single- and two-qubit gate fidelities matching other leading platforms and scalability still remaining a relative strength; however, due to qubit wiring considerations, mobile electron architectures have been proposed to facilitate upward scaling, and this opens the possibility of enlarging the motional amplitude for electric-dipole spin resonance (EDSR)-based qubit manipulation. In this work, we examine and demonstrate the possibility of significantly outperforming static-EDSR-type single-qubit pulsing by taking advantage of greater spatial mobility to achieve higher Rabi frequencies and reduce the effect of charge noise. Our theoretical results indicate that fidelities are ultimately bottlenecked by spin-valley physics, which can be suppressed through the use of quantum optimal control. We demonstrate that, across different potential regimes and competing physical models, shuttling-based single-qubit gates retain significant advantages over existing alternatives.
There have been impressive breakthroughs in semiconductor quantum dots in recent years, with single- and two-qubit gate fidelities matching other leading platforms and scalability still remaining a relative strength; however, due to qubit wiring considerations, mobile electron architectures have been proposed to facilitate upward scaling, and this opens the possibility of enlarging the motional amplitude for electric-dipole spin resonance (EDSR)-based qubit manipulation. In this work, we examine and demonstrate the possibility of significantly outperforming static-EDSR-type single-qubit pulsing by taking advantage of greater spatial mobility to achieve higher Rabi frequencies and reduce the effect of charge noise. Our theoretical results indicate that fidelities are ultimately bottlenecked by spin-valley physics, which can be suppressed through the use of quantum optimal control. We demonstrate that, across different potential regimes and competing physical models, shuttling-based single-qubit gates retain significant advantages over existing alternatives.
Semiconductor quantum dots have shown impressive breakthroughs in the last years, with single and two qubit gate fidelities matching other leading platforms and scalability still remaining a relative strength. However, due to qubit wiring considerations, mobile electron architectures have been proposed to facilitate upward scaling. In this work, we examine and demonstrate the possibility of significantly outperforming static EDSR-type single-qubit pulsing by taking advantage of the larger spatial mobility to achieve larger Rabi frequencies and reduce the effect of charge noise. Our theoretical results indicate that fidelities are ultimately bottlenecked by spin-valley physics, which can be suppressed through the use of quantum optimal control, and we demonstrate that, across different potential regimes and competing physical models, shuttling based single-qubit gates retain significant advantage over existing alternatives.
Dynamic qubit routing is emerging as a promising architectural path for semiconductor quantum processors. Charge carriers can be rapidly moved around on a chip using traveling-wave potentials known as conveyors, preserving the spin state with high fidelity. Originally developed for spin transport, conveyor-mode shuttling may also offer opportunities for performing qubit operations directly controlled by the motion itself. Here, we demonstrate coherent single- and two-qubit control by conveyor-mode electron shuttling, using two conceptually different approaches. First, conveyor electric-dipole spin resonance (conveyor EDSR) achieves high-fidelity rotations by resonantly shuttling spins through transverse magnetic-field gradients at their mean Larmor frequency. Second, conveyor diabatic gates exploit quantization-axis tilts for tunable bang-bang control. Combining diabatic conveyor transport with exchange activation controlled by the motion directly yields a variety of effective two-qubit interactions selectable via the shuttling speed and distance. These experimental results motivate an architectural paradigm of reconfigurable and transport-driven spin qubits.
Hole spin qubits in semiconductor quantum dots (QDs) enable high-fidelity all-electric control, but conventional electric dipole spin resonance (EDSR) can require substantial rf drive power at the low magnetic fields that are favorable for qubit coherence and readout. In planar Ge hole spin qubits, this can reach -27 dBm at the device, posing challenges for scalable architectures due to heating and crosstalk. Here, we demonstrate a flopping-mode (FM) qubit in Ge, where a single spin is delocalized in a double QD, combining first-order protection against charge noise with exceptionally efficient electric driving. By mapping out coherence sweet-spots as a function of magnetic field orientation we achieve T2∗=1.4μs, T2Hahn=11.5μs, T2φ,CPMG32=130μs, and T1=226μs, and a single-qubit gate fidelity of up to 99.76% for a gate time tXπ=88 ns. Importantly, these results are obtained at a nearly in-plane magnetic field of 5 mT using only -52 dBm drive power at the device. We further find that qubit relaxation in this regime is consistent with a two-photon Orbach process, providing a route for further optimization. Our results demonstrate that FM-EDSR supports ultra-low-power, high-fidelity single-qubit operations, improvements that could benefit scalable hole-spin-based architectures and hybrid spin-photon interfaces.
Single spin quantum dot qubits in silicon are a promising candidate for a scalable quantum processor due to their long coherence times, compact size, and ease of integration into existing fabrication technologies. Realizing a large quantum processor composed of thousands or more logical qubits requires the integration of conventional transistor circuitry \nand wiring interconnects to control each individual dot in the processor. The high density of control wiring required for these processors presents many engineering challenges. In this thesis, we propose a surface code quantum processor for silicon quantum dot qubits based on a node/network architecture. Local nodes consisting of just seven quantum dots are \nspatially separated on the order of microns to facilitate space for the necessary high density wiring. Entanglement is distributed between individual nodes via shuttling of entangled electron pairs throughout the network. X or Z stabilizer operations, necessary for operating the surface code, are realized by distributing three electron spin singlet pairs across four local nodes followed by local gate operations and ancilla measurements. Simulations of electron shuttling indicate that adiabatic transport is possible on timescales that do not bottleneck the processor speed. Phase rotation of the shuttled spin, induced by the Stark shift, can lower the overall shuttling fi delity; however, the error can be mitigated by proper electrostatic tuning of the stationary electron's g-factor. Using realistic noise models, we estimate error thresholds with respect to single and two-qubit gate fidelities as well as \nsinglet dephasing errors during shuttling. Electron shuttling is a key resource of the proposed network architecture. We continue the shuttling simulations by presenting an algorithm for finding constant-adiabatic shuttling control pulses, which enables a more rigorous study of how different conditions impact the shuttling speed and fidelity. These constant adiabatic pulses are used to optimize the physical device geometry to maximize charge shuttling speeds up to 300 nm/ns in the single-valley case. We then switch to an effective Hamiltonian representation where spin and valley degrees of freedom are accounted for during shuttling. Using realistic device and material parameters, shuttle speeds in the range 10-100 nm/ns with high spin entanglement \n fidelities are obtained when the tunneling energy exceeds the Zeeman energy. High fidelity shuttling also requires the inter-dot valley phase difference to be below a threshold determined by the ratio of tunneling and Zeeman energies, so that spin-valley-orbit mixing is weak. In this regime, we find that the primary source of infi delity is a coherent spin rotation that is correctable, in principle, using single spin rotations. Two-qubit gates in the network architecture are mediated by the exchange interaction, \nan interaction that stems from the Coulomb interaction but manifests as a rotation between the |0,1> and |1,0> two qubit states. Realizing fault tolerant two-qubit gates has proven difficult in silicon quantum dots due to charge noise which perturbs the electron orbitals states, causing decoherence. Quantitatively accurate modelling of exchange in general quantum dot networks is important towards realizing fault tolerant gates. Traditional modelling methods, such as a full con figuration interaction approach, are cumbersome due to significant computational overhead required when accounting for the electron-electron interactions in the calculation. We present a modi ed linear combination of harmonic orbitals con figuration interaction (LCHO-CI) approach which signifi cantly reduces the computational time for obtaining quantitatively accurate estimations of exchange. The method works by approximating the single electron orbitals of the quantum dot network using an orthogonal basis of harmonic orbitals. This choice of orthogonal basis allows a precalculated library of matrix elements to be used in evaluating the Coulomb interactions, which speeds up the LCHO-CI calculation. The modi ed LCHO-CI approach is then used to study how the physical device geometry impacts the charge noise sensitivity of a double quantum dot system. We fi nd that, in general, geometries which increase the dot charging energy and decrease the gate lever arms improve the system's sensitivity to charge noise. We conclude this thesis by pivoting away from theoretical studies of silicon quantum dots and towards experimental studies of electron transport in dopant-free GaAs heterostructures. In modulation doped GaAs heterostructures, a doping layer is used to induce a two-dimensional electron gas (2DEG) at the heterojunction. Dopant-free GaAs lack the doping layer which makes fabrication more difficult as local electron reservoirs must be used to bring carriers and induce a 2DEG. The lack of the doping layer offers several advantages over modulation doped heterostructures, such as gate-ability of the 2DEG and ability to make ambipolar devices (both n- and p-type ohmic contacts). Realizing n- and p-type ohmic contacts requires etching a recess pit and depositing the ohmic material at an angle in order to preventing screening of the top gate when inducing a 2DEG or two-dimensional hole gas (2DHG). Magnetotransport experiments are used to characterize an induced 2DEG and 2DHG in a Hall bar fabricated on a 310 nm deep single heterojunction. The carrier mobility and density can be tuned using the top gate, and we achieve peak mobility values of 4.5E6 cm2/Vs and 0.65E6 cm2/Vs for the 2DEG and 2DHG respectively. We then move to a one-dimensional system and study electron transport through a quantum point contact. Conductance quantization is observed, and subband spectroscopy \nmeasurements indicate a 1D subband spacing of 4.5 meV. Finally, we study dynamically driven electron transport in a zero-dimensional system using a tunable-barrier quantum dot acting as a single electron pump. Single electron pumping is observed up to T = 5 K, and fi ts to the electron cascade model suggests pumping errors of 1.87 ppm when operated at a driving frequency of f = 500 MHz.
Si/SiGe quantum wells that incorporate Ge concentration oscillations, known as long-period Wiggle Wells, have been shown to enhance the Dresselhaus spin-orbit coupling of conduction-band electrons. Such intrinsic spin-orbit coupling is desirable when performing spin-qubit gate operations based on electric dipole spin resonance (EDSR) because it eliminates the need for external micromagnets. However, random-alloy disorder plays a key role in this materials system by spatially randomizing the valley splitting and the valley phase φs,s, and it has not been fully accounted for in recent EDSR analyses. Here, we show that alloy disorder affects EDSR in two main ways. First, the Rabi frequency Ω acquires a dependence on the valley phase, given by cosφs,s, which causes spatial randomization of Ω. Despite this variability, we show that fast EDSR can be achieved at most locations across a given sample. Second, a new Rabi driving mechanism emerges, enabled by valley dipoles and the hybridization of ground and excited valley states, which arise from alloy disorder and EDSR driving, respectively. This mechanism is dominant in regions of low valley splitting. Alloy disorder can therefore strengthen EDSR, but it can also cause gradients in Ω that lead to dephasing in the rotating frame. We explore this problem by first locating "sweet spots," where EDSR is relatively insensitive to electric-field fluctuations. We then show that high-fidelity Rabi oscillations can be achieved in the presence of realistic charge noise. These results suggest that Wiggle Wells are a promising platform for high-quality, micromagnet-free gate operations.
There are many successful proposals for using electron spins in quantum dots as qubits. However, a semiconductor quantum dot-based qubit that is scalable, reliable and robust enough for actual quantum information applications has not been realized yet. Common problems in semiconductor quantum dot-based spin qubits are (i) the manipulation and coupling of spin states in a scalable way and (ii) the decoherence of the qubit. While the first problem has been overcome with the so-called exchange-only qubit, the second problem is still hindering the progress towards large-scale quantum computation using quantum dot-based spin qubits.\n \n In this regard, we propose a feasible and scalable exchange-only spin qubit composed of four quantum dots that is, to leading order, intrinsically insensitive to randomly fluctuating magnetic noise, while still offering a full electric control. Motivated by our findings, we then analyze in full detail the main relaxation mechanisms in exchange-only spin qubits composed of three and four dots, and find the regimes where the coherence time of the qubit can be extended by several orders of magnitude. We then explore the possibility of implementing our proposal for an exchange-only qubit in a device composed of three quantum dots—which would offer an unprecedented degree of tunability—and in an already existing device with five quantum dots, proving that a straightforward implementation of our proposal is feasible.\n \n We conclude this project with a thorough analysis of a common electric dipole spin resonance (EDSR) experiment in a system composed of two quantum dots with intrinsic spin-mixing mechanisms. EDSR is a broadly used tool for spectroscopy of quantum dots, yet a detailed theoretical analysis of the physics of an electrically driven system of quantum dots at resonance is still lacking.