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arXiv:2402.15114

Cavity based non-destructive detection of photoassociation in a dark MOT

V. I. Gokul, Arun Bahuleyan, S. P. Dinesh, V. R. Thakar, S. A. Rangwala

Published Feb 23, 2024• 0 citations
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Abstract

The photoassociation (PA) of rubidium dimer (Rb2) in a dark magneto-optic trap (MOT) is studied using atom-cavity collective strong coupling. This allows non-destructive detection of the molecule formation process as well as rapid and repeated interrogation of the atom-molecule system. The vacuum Rabi splitting (VRS) measurements from the bright MOT are carefully calibrated against equivalent measurements with fluorescence. Further loading rates in dark MOT are determined using VRS. This method provides a reliable, fast, and non-destructive detection scheme for ultracold molecules when the atoms are non-fluorescing using the free atoms coupled to a cavity.

DOI
10.48550/arxiv.2402.15114

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The photoassociation (PA) of rubidium dimer (Rb2) in a dark magneto-optic trap (MOT) is studied using atom-cavity collective strong coupling. This allows non-destructive detection of the molecule formation process as well as rapid and repeated interrogation of the atom-molecule system. The vacuum Rabi splitting (VRS) measurements from the bright MOT are carefully calibrated against equivalent measurements with fluorescence. Further loading rates in dark MOT are determined using VRS. This method provides a reliable, fast, and non-destructive detection scheme for ultracold molecules when the atoms are non-fluorescing using the free atoms coupled to a cavity.
The photoassociation (PA) of a rubidium dimer in a dark magneto-optical trap (MOT) is studied using atom-cavity collective strong coupling. This allows nondestructive detection of the molecule formation process as well as rapid and repeated interrogation of the atom-molecule system. The vacuum Rabi splitting (VRS) measurements from the bright MOT are carefully calibrated against equivalent measurements with fluorescence. Further loading rates in the dark MOT are determined using VRS. This method provides a reliable, fast, and nondestructive detection scheme for detecting the PA using the free atoms coupled to a cavity when the atoms are in a nonfluorescing state.
The collective strong coupling of rubidium atoms in a magneto-optical trap (MOT) to the Laguerre-Gaussian (LG) modes of a Fabry-P\'erot cavity is investigated. Bright and dark 85Rb^{85}\mathrm{Rb}85Rb MOT atoms are prepared at the geometric center of the cavity, and the vacuum Rabi splitting (VRS) of the collectively coupled atom-cavity system is measured for LGl0{\mathrm{LG}}_{l0}LGl0​ (l=0,1,2,3l=0,1,2,3l=0,1,2,3) modes. The atom number coupled to the cavity mode depends on the overlap of the atomic density distribution and the specific spatial mode function, which is reflected in the measured VRS spectrum. The known mode function and the measured VRS can then be used to test whether the atomic density distribution in the experiment is Gaussian or uniform. A simple theoretical model for this process is described, and the experimental measurements are found to be in close agreement with the model.
We present a technique, based on atoms coupled to an optical cavity, for nondestructive detection of trapped ions. We demonstrate the vacuum-Rabi splitting (VRS), arising from collective strong coupling of ultracold Rb atoms and a cavity, to change in the presence of trapped Rb+\mathrm{R}{\mathrm{b}}^{+}Rb+ ions. The Rb+\mathrm{R}{\mathrm{b}}^{+}Rb+ ions are optically dark and the Rb atoms are prepared in a dark magneto-optical trap. The VRS is measured on an optically open transition of the initially dark Rb atoms. The measurement itself is fast, nondestructive, and has sufficient fidelity to permit the measurement of the atomic-state-selective ion-atom collision rate. This demonstration illustrates a method based on atom-cavity coupling to measure two-particle interactions generically and nondestructively.
This thesis focuses on the construction and development of an experiment to study cold potassium atoms in an optical ring cavity. Firstly we load a potassium-39 magneto optical trap (MOT) inside the ring cavity. To achieve this a laser system, rectangular magnetic coils system and vacuum system are designed and constructed. To stabilise the laser system, a detailed study of various potassium spectroscopy techniques is undertaken and the reference laser is suitably locked to the magnetically induced spectroscopy. We load an ensemble of 10\\(^5\\) potassium atoms inside the ring cavity mode and study their collective strong coupling with the cavity field. In the collective strong coupling regime, the photons are coherently exchanged between the atomic ensemble and cavity field. This rate of exchange is determined by the singlephoton Rabi frequency `2\\(g\\)' which must be larger than the cavity field decay rate `2\\(k\\)' and atomic spontaneous emission rate `2\\(ᵧ\\)'. As a result of this coupling, the peak in the cavity transmission signal undergoes a splitting known as `vacuum Rabi splitting' (or `normal mode splitting'). The vacuum Rabi splitting has been realised and measured to be ~ 2\\(π\\). 18 MHz in our system.
In this paper, we report the measurement of molecular formation rate constant of Rb2{\mathrm{Rb}}_{2}Rb2​ directly in a magneto-optical trap (MOT). The ground state molecules are detected by two-photon ionization, resonantly enhanced through the intermediate ${a}^{3}{\ensuremath{\Sigma}}_{u}^{+}\ensuremath{\rightarrow}{2}^{3}{\ensuremath{\Pi}}_{g}$ molecular band. We have measured the rate constant as a function of atomic density to conclude that the molecules Rb2{\mathrm{Rb}}_{2}Rb2​ are formed in the MOT by a photoassociation process caused by the trapping laser beams. We also measured the rate constant as a function of the trapping laser intensity. The results here presented are of importance to future experiments involving trapping of cold molecules.
This paper presents a setup capable of producing a high-flux continuous beam of cold rubidium atoms for cavity quantum electrodynamics experiments in the region of strong coupling. A 2D + magneto-optical trap (MOT), loaded with rubidium getters in a dry-film-coated vapor cell, fed a secondary moving-molasses MOT (MM-MOT) at a rate greater than 2 × 10 10 atoms/s. The MMMOT provided a continuous beam with a tunable velocity. This beam was then directed through the waist of a cavity with a length of 280 µm, resulting in a vacuum Rabi splitting of more than ±10 MHz. The presence of a sufficient number of atoms in the cavity mode also enabled splitting in the polarization perpendicular to the input. The cavity was in the strong coupling region, with an atom-photon dipole coupling coefficient g of 7 MHz, a cavity mode decay rate κ of 3 MHz, and a spontaneous emission decay rate γ of 6 MHz.