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arXiv:2402.09308 · Physical Review Research

Wave-particle correlations in multiphoton resonances of coherent light-matter interaction

Th. K. Mavrogordatos

Published Mar 7, 2024• 4 citations
arXivHTMLPDF

Abstract

We discuss the conditional measurement of field amplitudes by a nonclassical photon sequence in the Jaynes-Cummings (JC) model under multiphoton operation. We do so by employing a correlator of immediate experimental relevance to reveal a distinct nonclassical evolution in the spirit of Foster []. The correlator relies on the complementary nature of the pictures obtained from different unravelings of a JC source master equation. We demonstrate that direct photodetection entails a conditioned separation of timescales, a quantum beat, and a semiclassical oscillation, produced by the coherent light-matter interaction in its strong-coupling limit. We single out the quantum beat in the analytical expression for the waiting-time distribution, pertaining to the particle nature of the scattered light, and find a negative spectrum of quadrature amplitude squeezing, characteristic of its wave nature for certain operation settings. Finally, we jointly detect the dual aspects through the wave-particle correlator, showing an asymmetric regression of fluctuations to the steady state which depends on the quadrature amplitude being measured. Published by the American Physical Society 2024

DOI
10.1103/physrevresearch.6.013250

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We explore the statistical behavior of the light emanating from a coherently driven Jaynes–Cummings (JC) oscillator operating in the regime of multiphoton blockade with two monitored output channels causing the loss of coherence at equal rates. We do so by adopting an operational approach that draws the particle and wave aspects of the forward-scattered radiation together, building upon the relationship between quantum optical correlation functions and conditional measurements. We first derive an analytical expression of the intensity cross-correlation function at the peak of the two-photon JC resonance to demonstrate the breakdown of detailed balance. The application of the quantum trajectory theory in parallel with the quantum regression formula subsequently uncovers various aspects of temporal asymmetry in the quantum fluctuations characterizing the cascaded process through which a multiphoton resonance is established and read out. We find that monitoring different quadratures of the cavity field in conditional homodyne detection affects the times waited between successive photon counter “clicks,” which in turn trigger the sampling of the homodyne current. Despite the fact that the steady-state cavity occupation is of the order of a photon, monitoring of the developing bimodality also impacts the ratio between the emissions directed along the two decoherence channels.
We show that the saturation of a multiphoton transition is accompanied by a gradual collapse of quantum multimodality in the strong-coupling limit of the weakly driven Jaynes-Cummings (JC) model. By means of a perturbative method, we illustrate the prominent role of quantum fluctuations by focusing on the two- and three-photon resonance operation in a regime where the steady-state average photon number is below or marginally above unity. We also reveal two coexistent quantum beats in the intensity correlation function of the forwards scattered photons. These beats, originating from the states mediating the cascaded decay, arise as a direct consequence of the distinct JC spectrum. Their interference coordinates with the alternation of positive and negative values of the Wigner function around the phase-space origin in the transient conditioned on a photodetection.
Abstract We operationally uncover aspects of wave/particle duality for the open driven Jaynes–Cummings (JC) model in its strong-coupling limit. We lay special emphasis on the vacuum Rabi resonance, and determine the corresponding normalized intensity-field correlation function via mapping to ordinary resonance fluorescence. We demonstrate that temporal wave–particle fluctuations of light emanating from an established vacuum Rabi resonance are explicitly non-classical, while the limit of vanishing spontaneous emission restores detailed balance. When photon blockade sets in, individual realizations show a rapidly increasing frequency of fluctuations towards the two-photon resonance, arising as a direct consequence of a resolved JC spectrum. About the two-photon resonance peak, spontaneous emissions are more likely to revive a high-frequency quantum beat in the conditioned electromagnetic field amplitude than photons escaping out of the cavity mode. The beat originates from a coherent superposition of the first excited JC couplet states, and sets the background against which nonclassical phase shifts are observed in the conditioned quadrature amplitudes. We also find that the onset of steady-state bimodality reduces the variation of the normalized intensity-field correlation, at the expense of its temporal symmetry.
Abstract We find that the phase-space representation of the electromagnetic field inside a driven cavity strongly coupled to a two-level atom can be employed to distinguish photon emissions along a ladder of dressed states sustaining a two-photon resonance. The emissions are told apart by means of the different quantum beats generated by the conditional states they prepare. Sample quantum trajectories explicitly reveal the difference in the transient due to the initial condition, in a background set by the Jaynes–Cummings spectrum and revealed by the strong-coupling limit. Their ensemble-averaged evolution is tracked for a time period similar to that waited for the loss of a next photon as the maximum non-exclusive probability, indicated by the peak of the intensity correlation function.
In the representation of dressed states, which diagonalizes the Hamiltonian in the Jaynes-Cummings model, the Bose operator for excitation annihilation Â, the spin operator Σ^_\hat \Sigma \_Σ^_ , and the corresponding Hermitian-conjugate operators are found. Using these operators, correlated coherent states were constructed and statistical properties of a field mode and an atom in these states are studied. Nonclassical field properties, such as the deviation of the probability distribution for the number of photons from the Poissonian distribution, its time dependence, and the squeezing of quadrature field components are found. For small interaction coefficients k, all these characteristics of the model vary weakly in time in the resonance case.
We explore the role of quantum fluctuations in the strong-coupling limit of the dissipative Jaynes–Cummings oscillator driven on resonance. For weak excitation, we derive analytical expressions for the spectrum and the intensity correlation function for the photons scattered by the two-state atom coupled to the coherently driven cavity mode. We do so by writing down a birth–death process adding the higher orders in the excitation strength needed to go beyond the pure-state factorization, following the method introduced in Carmichael (2008). Our results for the first and second-order correlation functions are complemented by the numerical investigation of the waiting-time distribution for the photon emissions directed sideways, and the comparison with ordinary resonance fluorescence. To close out our discussion, we increase the driving field amplitude and approach the critical point organizing a second-order dissipative quantum phase transition by depicting the excitation pathways in the intracavity field distribution for a finite system size.