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arXiv:2206.11197 · Physical Review A

Visualizing the breakdown of quantum multimodality in coherently driven light-matter interaction

Th. K. Mavrogordatos

Published Jul 14, 2022• 5 citations
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Abstract

We show that the saturation of a multiphoton transition is accompanied by a gradual collapse of quantum multimodality in the strong-coupling limit of the weakly driven Jaynes-Cummings (JC) model. By means of a perturbative method, we illustrate the prominent role of quantum fluctuations by focusing on the two- and three-photon resonance operation in a regime where the steady-state average photon number is below or marginally above unity. We also reveal two coexistent quantum beats in the intensity correlation function of the forwards scattered photons. These beats, originating from the states mediating the cascaded decay, arise as a direct consequence of the distinct JC spectrum. Their interference coordinates with the alternation of positive and negative values of the Wigner function around the phase-space origin in the transient conditioned on a photodetection.

DOI
10.1103/physreva.106.013711

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We show that the saturation of a multiphoton transition is accompanied by a gradual collapse of quantum multimodality in the strong-coupling limit of the weakly driven Jaynes-Cummings (JC) model. By means of a perturbative method, we illustrate the prominent role of quantum fluctuations by focusing on the two- and three-photon resonance operation in a regime where the steady-state average photon number is below or marginally above unity. We also reveal two coexistent quantum beats in the intensity correlation function of the forwards scattered photons. These beats, originating from the states mediating the cascaded decay, arise as a direct consequence of the distinct JC spectrum. Their interference coordinates with the alternation of positive and negative values of the Wigner function around the phase-space origin in the transient conditioned on a photodetection.
We calculate the cavity-field distribution in the Wigner representation for the two-photon resonance of the weakly driven Jaynes-Cummings (JC) oscillator in its strong-coupling limit. Using an effective four-level system, we analytically demonstrate the presence of steady-state and transient bimodality which breaks azimuthal symmetry in phase space. The two steady-state peaks are located at opposite positions and do not correspond to the two-photon amplitude of the driven transition. The developing bimodality is portrayed in parallel with the evolution of the intensity correlation function for the forward-scattered photons, before being finally contrasted to the few-photon steady-state and transient phase-space profiles for the cavity mode in the JC model driven on resonance.
We discuss the conditional measurement of field amplitudes by a nonclassical photon sequence in the Jaynes-Cummings (JC) model under multiphoton operation. We do so by employing a correlator of immediate experimental relevance to reveal a distinct nonclassical evolution in the spirit of Foster []. The correlator relies on the complementary nature of the pictures obtained from different unravelings of a JC source master equation. We demonstrate that direct photodetection entails a conditioned separation of timescales, a quantum beat, and a semiclassical oscillation, produced by the coherent light-matter interaction in its strong-coupling limit. We single out the quantum beat in the analytical expression for the waiting-time distribution, pertaining to the particle nature of the scattered light, and find a negative spectrum of quadrature amplitude squeezing, characteristic of its wave nature for certain operation settings. Finally, we jointly detect the dual aspects through the wave-particle correlator, showing an asymmetric regression of fluctuations to the steady state which depends on the quadrature amplitude being measured. Published by the American Physical Society 2024
We approach the strong-coupling thermodynamic limit in the response of the open driven Jaynes-Cummings (JC) oscillator. We do so by highlighting the role of quantum fluctuations against the semiclassical response in three distinct regimes of operation. We begin by demonstrating the persistence of photon blockade, predicted in Carmichael [Phys. Rev. X 5, 031028 (2015)], as a manifestation of the inherently quantum and nonlinear JC spectrum revealed for vanishing dissipation. We then proceed to discuss the importance of bistability, which, despite being present in photon blockades, is able to provide an alignment between the semiclassical nonlinearity and quantum dynamics only for a driving amplitude having the same order of magnitude as the light-matter coupling strength. This resolution brings us to the critical point of the well-known quantum-phase transition of second order on resonance, where the quantum and semiclassical pictures are once more contrasted for a varying participation of the two coherent interactions when going through the collapse of the quasienergy spectrum.
We explore the statistical behavior of the light emanating from a coherently driven Jaynes–Cummings (JC) oscillator operating in the regime of multiphoton blockade with two monitored output channels causing the loss of coherence at equal rates. We do so by adopting an operational approach that draws the particle and wave aspects of the forward-scattered radiation together, building upon the relationship between quantum optical correlation functions and conditional measurements. We first derive an analytical expression of the intensity cross-correlation function at the peak of the two-photon JC resonance to demonstrate the breakdown of detailed balance. The application of the quantum trajectory theory in parallel with the quantum regression formula subsequently uncovers various aspects of temporal asymmetry in the quantum fluctuations characterizing the cascaded process through which a multiphoton resonance is established and read out. We find that monitoring different quadratures of the cavity field in conditional homodyne detection affects the times waited between successive photon counter “clicks,” which in turn trigger the sampling of the homodyne current. Despite the fact that the steady-state cavity occupation is of the order of a photon, monitoring of the developing bimodality also impacts the ratio between the emissions directed along the two decoherence channels.
We explore the role of quantum fluctuations in the strong-coupling limit of the dissipative Jaynes–Cummings oscillator driven on resonance. For weak excitation, we derive analytical expressions for the spectrum and the intensity correlation function for the photons scattered by the two-state atom coupled to the coherently driven cavity mode. We do so by writing down a birth–death process adding the higher orders in the excitation strength needed to go beyond the pure-state factorization, following the method introduced in Carmichael (2008). Our results for the first and second-order correlation functions are complemented by the numerical investigation of the waiting-time distribution for the photon emissions directed sideways, and the comparison with ordinary resonance fluorescence. To close out our discussion, we increase the driving field amplitude and approach the critical point organizing a second-order dissipative quantum phase transition by depicting the excitation pathways in the intracavity field distribution for a finite system size.
Abstract We find that the phase-space representation of the electromagnetic field inside a driven cavity strongly coupled to a two-level atom can be employed to distinguish photon emissions along a ladder of dressed states sustaining a two-photon resonance. The emissions are told apart by means of the different quantum beats generated by the conditional states they prepare. Sample quantum trajectories explicitly reveal the difference in the transient due to the initial condition, in a background set by the Jaynes–Cummings spectrum and revealed by the strong-coupling limit. Their ensemble-averaged evolution is tracked for a time period similar to that waited for the loss of a next photon as the maximum non-exclusive probability, indicated by the peak of the intensity correlation function.