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arXiv:2401.17394 · Physical Review Applied

Fast storage of photons in cavity-assisted quantum memories

Johann S. Kollath-Bönig, Luca Dellantonio, Luigi Giannelli, Tom Schmit, Giovanna Morigi, Anders Søndberg Sørensen

Published Oct 16, 2024• 6 citations
arXivHTMLPDF

Abstract

Ideal photonic quantum memories can store arbitrary pulses of light with unit efficiency. This requires operating in the adiabatic regime, where pulses have a duration much longer than the bandwidth of the memory. In the nonadiabatic regime of short pulses, memories are therefore imperfect, and information is always lost. We theoretically investigate the bandwidth limitations for setups based on individual atoms, or ensembles thereof, confined inside optical cavities. We identify an effective strategy for optimizing the efficiencies of the storage and retrieval process regardless of the duration or the shape of the pulses. Our protocol is derived almost completely analytically and attains efficiencies that are comparable to those obtained by numerical optimization. Furthermore, our results provide an improved understanding of the performance of quantum memories in several regimes. When considering pulses defined on an infinite time interval, the shapes can be divided into two categories, depending on their asymptotic behaviors. If the intensity of the pulse increases with time slower than or as an exponential function then the storage efficiency is only limited by the pulse width. For pulses defined on a finite interval, on the other hand, the efficiency is determined by the shape at the beginning of the storage or, correspondingly, at the end of the retrieval process.

DOI
10.1103/physrevapplied.22.044038

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Ideal photonic quantum memories can store arbitrary pulses of light with unit efficiency. This requires operating in the adiabatic regime, where pulses have a duration much longer than the bandwidth of the memory. In the nonadiabatic regime of short pulses, memories are therefore imperfect, and information is always lost. We theoretically investigate the bandwidth limitations for setups based on individual atoms, or ensembles thereof, confined inside optical cavities. We identify an effective strategy for optimizing the efficiencies of the storage and retrieval process regardless of the duration or the shape of the pulses. Our protocol is derived almost completely analytically and attains efficiencies that are comparable to those obtained by numerical optimization. Furthermore, our results provide an improved understanding of the performance of quantum memories in several regimes. When considering pulses defined on an infinite time interval, the shapes can be divided into two categories, depending on their asymptotic behaviors. If the intensity of the pulse increases with time slower than or as an exponential function then the storage efficiency is only limited by the pulse width. For pulses defined on a finite interval, on the other hand, the efficiency is determined by the shape at the beginning of the storage or, correspondingly, at the end of the retrieval process.
We theoretically analyze the efficiency of a quantum memory for single photons. The photons propagate along a transmission line and impinge on one of the mirrors of a high-finesse cavity. The quantum memory is constituted by a single atom within the optical resonator. Photon storage is realized by the controlled transfer of the photonic excitation into a metastable state of the atom and occurs via a Raman transition with a suitably tailored laser pulse, which drives the atom. Our study is supported by numerical simulations, in which we include the modes of the transmission line and we use the experimental parameters of existing experimental setups. It reproduces the results derived using input–output theory in the corresponding regimes and can be extended to compute dynamics where the input–output formalism cannot be straightforwardly applied. Our analysis determines the maximal storage efficiency, namely, the maximal probability to store the photon in a stable atomic excitation, in the presence of spontaneous decay and cavity parasitic losses. It further delivers the form of the laser pulse that achieves the maximal efficiency by partially compensating parasitic losses. We numerically assess the conditions under which storage based on adiabatic dynamics is preferable to non-adiabatic pulses. Moreover, we systematically determine the shortest photon pulse that can be efficiently stored as a function of the system parameters.
Quantum efficiency is an important characteristic of quantum memory devices that are aimed at recording the quantum state of light signals and its storing and reading. In the case of memory based on an ensemble of cold atoms placed in an optical cavity, the efficiency is restricted, in particular, by relaxation processes in the system of active atomic levels. We show how the effect of the relaxation on the quantum efficiency can be determined in a regime of the memory usage in which the evolution of signals in time is not arbitrarily slow on the scale of the field lifetime in the cavity and when the frequently used approximation of the adiabatic elimination of the quantized cavity mode field cannot be applied. Taking into account the effect of the nonadiabaticity on the memory quality is of interest in view of the fact that, in order to increase the field–medium coupling parameter, a higher cavity quality factor is required, whereas storing and processing of sequences of many signals in the memory implies that their duration is reduced. We consider the applicability of the well-known efficiency estimates via the system cooperativity parameter and estimate a more general form. In connection with the theoretical description of the memory of the given type, we also discuss qualitative differences in the behavior of a random source introduced into the Heisenberg–Langevin equations for atomic variables in the cases of a large and a small number of atoms.
Abstract Attenuated laser pulses are often employed in place for single photons in order to test the efficiency of the elements of a quantum network. In this work we analyze theoretically the dynamics of storage of an attenuated light pulse (where the pulse intensity is at the single photon level) propagating along a transmission line and impinging on the mirror of a high finesse cavity. Storage is realized by the controlled transfer of the photonic excitations into a metastable state of an atom confined inside the cavity and occurs via a Raman transition with a suitably tailored laser pulse, which drives the atom and minimizes reflection at the cavity mirror. We determine the storage efficiency of the weak coherent pulse which is reached by protocols optimized for single-photon storage. We determine the figures of merit and we identify the conditions on an arbitrary pulse for which the storage dynamics approaches the one of a single photon. Our formalism can be extended to arbitrary types of input pulses and to quantum memories composed by spin ensembles, and serves as a basis for identifying the optimal protocols for storage and readout.
We demonstrate the storage of 5-ns light pulses in a single rubidium atom coupled to a fiber-based optical resonator. Our storage protocol addresses a regime beyond the conventional adiabatic limit and approaches the theoretical bandwidth limit. We extract the optimal control laser pulse properties from a numerical simulation of our system and measure storage efficiencies of $(8.1\ifmmode\pm\else\textpm\fi{}1.1)%$, in close agreement with the maximum expected efficiency. Such well-controlled and high-bandwidth atom-photon interfaces are key components for future hybrid quantum networks.
We report on the high-efficiency storage and retrieval of weak coherent optical pulses and photonic qubits in a cavity-enhanced solid-state quantum memory. By using an atomic frequency comb (AFC) memory in a Pr 3+ :Y 2 SiO 5 crystal embedded in an impedance-matched cavity, we stored weak coherent pulses at the single photon level with up to 62% efficiency for a pre-determined storage time of 2 µs. We also confirmed that the impedance-matched cavity enhances the efficiency for longer storage times up to 70 µs. Harnessing the temporal multimodality of the AFC scheme, we stored weak coherent time-bin qubits with a record (51 ± 2%) efficiency and a fidelity over (94.8 ± 1.4)%, limited by imperfections in the qubits creation and measurement.
Abstract We investigate the non-stationary and relaxation phenomena in cavity-assisted quantum memories for light. As a storage medium we consider an ensemble of cold atoms with standard Lambda-scheme of working levels. Some theoretical aspects of the problem were treated previously by many authors, and recent experiments stimulate more deep insight into the ultimate ability and limitations of the device. Since quantum memories can be used not only for the storage of quantum information, but also for a substantial manipulation of ensembles of quantum states, the speed of such manipulation and hence the ability to write and retrieve the signals of relatively short duration becomes important. In our research we do not apply the so-called bad cavity limit, and consider the memory operation of the signals whose duration is not much larger than the cavity field lifetime, accounting also for the finite lifetime of atomic coherence. In our paper we present an effective approach that makes it possible to find the non-stationary amplitude and phase behavior of strong classical control field, that matches the desirable time profile of both the envelope and the phase of the retrieved quantized signal. The phase properties of the retrieved quantized signals are of importance for the detection and manipulation of squeezing, entanglement, etc by means of optical mixing and homodyning.