Abstract Attenuated laser pulses are often employed in place for single photons in order to test the efficiency of the elements of a quantum network. In this work we analyze theoretically the dynamics of storage of an attenuated light pulse (where the pulse intensity is at the single photon level) propagating along a transmission line and impinging on the mirror of a high finesse cavity. Storage is realized by the controlled transfer of the photonic excitations into a metastable state of an atom confined inside the cavity and occurs via a Raman transition with a suitably tailored laser pulse, which drives the atom and minimizes reflection at the cavity mirror. We determine the storage efficiency of the weak coherent pulse which is reached by protocols optimized for single-photon storage. We determine the figures of merit and we identify the conditions on an arbitrary pulse for which the storage dynamics approaches the one of a single photon. Our formalism can be extended to arbitrary types of input pulses and to quantum memories composed by spin ensembles, and serves as a basis for identifying the optimal protocols for storage and readout.
Abstract Attenuated laser pulses are often employed in place for single photons in order to test the efficiency of the elements of a quantum network. In this work we analyze theoretically the dynamics of storage of an attenuated light pulse (where the pulse intensity is at the single photon level) propagating along a transmission line and impinging on the mirror of a high finesse cavity. Storage is realized by the controlled transfer of the photonic excitations into a metastable state of an atom confined inside the cavity and occurs via a Raman transition with a suitably tailored laser pulse, which drives the atom and minimizes reflection at the cavity mirror. We determine the storage efficiency of the weak coherent pulse which is reached by protocols optimized for single-photon storage. We determine the figures of merit and we identify the conditions on an arbitrary pulse for which the storage dynamics approaches the one of a single photon. Our formalism can be extended to arbitrary types of input pulses and to quantum memories composed by spin ensembles, and serves as a basis for identifying the optimal protocols for storage and readout.
We theoretically analyze the efficiency of a quantum memory for single photons. The photons propagate along a transmission line and impinge on one of the mirrors of a high-finesse cavity. The quantum memory is constituted by a single atom within the optical resonator. Photon storage is realized by the controlled transfer of the photonic excitation into a metastable state of the atom and occurs via a Raman transition with a suitably tailored laser pulse, which drives the atom. Our study is supported by numerical simulations, in which we include the modes of the transmission line and we use the experimental parameters of existing experimental setups. It reproduces the results derived using input–output theory in the corresponding regimes and can be extended to compute dynamics where the input–output formalism cannot be straightforwardly applied. Our analysis determines the maximal storage efficiency, namely, the maximal probability to store the photon in a stable atomic excitation, in the presence of spontaneous decay and cavity parasitic losses. It further delivers the form of the laser pulse that achieves the maximal efficiency by partially compensating parasitic losses. We numerically assess the conditions under which storage based on adiabatic dynamics is preferable to non-adiabatic pulses. Moreover, we systematically determine the shortest photon pulse that can be efficiently stored as a function of the system parameters.
We show how to capture a single photon of arbitrary temporal shape with one atom coupled to an optical cavity. Our model applies to Raman transitions in three-level atoms with one branch of the transition controlled by a (classical) laser pulse, and the other coupled to the cavity. Photons impinging on the cavity normally exhibit partial reflection, transmission, and/or absorption by the atom. Only a control pulse of suitable temporal shape ensures impedance matching throughout the pulse, which is necessary for complete state mapping from photon to atom. For most possible photon shapes, we derive an unambiguous analytic expression for the shape of this control pulse, and we discuss how this relates to a quantum memory.
Ideal photonic quantum memories can store arbitrary pulses of light with unit efficiency. This requires operating in the adiabatic regime, where pulses have a duration much longer than the bandwidth of the memory. In the nonadiabatic regime of short pulses, memories are therefore imperfect, and information is always lost. We theoretically investigate the bandwidth limitations for setups based on individual atoms, or ensembles thereof, confined inside optical cavities. We identify an effective strategy for optimizing the efficiencies of the storage and retrieval process regardless of the duration or the shape of the pulses. Our protocol is derived almost completely analytically and attains efficiencies that are comparable to those obtained by numerical optimization. Furthermore, our results provide an improved understanding of the performance of quantum memories in several regimes. When considering pulses defined on an infinite time interval, the shapes can be divided into two categories, depending on their asymptotic behaviors. If the intensity of the pulse increases with time slower than or as an exponential function then the storage efficiency is only limited by the pulse width. For pulses defined on a finite interval, on the other hand, the efficiency is determined by the shape at the beginning of the storage or, correspondingly, at the end of the retrieval process.
Optical quantum memories are important components in the long-distance quantum communication based on quantum repeater protocol. To outperform the direct transmission of light with quantum repeaters, it is crucial to develop quantum memories with high fidelity, high efficiency and long storage time. Recently, we demonstrate that it is feasible to achieve a high storage efficiency of 92% for electromagnetically-induced-transparency (EIT)-based memory with weak coherent signal pulses in cold atomic ensembles [1]. To realize the highly-efficient memory with quantum light, we have built a bright and narrowband photon-pair source which can be locked to atomic transition based on the cavity-enhanced spontaneous parametric down conversion [2]. Here, we present our results on the storage of single photons generated by such a source in EIT-based memories. A storage efficiency of 36% is obtained in initial runs. Future improvements toward a high efficiency are discussed. Such a development paves the way for the applications of photon-pair-based quantum repeater and multi-photon synchronization.
We report on the high-efficiency storage and retrieval of weak coherent optical pulses and photonic qubits in a cavity-enhanced solid-state quantum memory. By using an atomic frequency comb (AFC) memory in a Pr 3+ :Y 2 SiO 5 crystal embedded in an impedance-matched cavity, we stored weak coherent pulses at the single photon level with up to 62% efficiency for a pre-determined storage time of 2 µs. We also confirmed that the impedance-matched cavity enhances the efficiency for longer storage times up to 70 µs. Harnessing the temporal multimodality of the AFC scheme, we stored weak coherent time-bin qubits with a record (51 ± 2%) efficiency and a fidelity over (94.8 ± 1.4)%, limited by imperfections in the qubits creation and measurement.
Photonic quantum information processing has emerged as a powerful platform for realising quantum-enhanced technologies. In order to be scalable, many of these technologies depend on the availability of a suitable quantum memory for the coherent storage and on-demand retrieval of photonic quantum states. In this thesis, I investigate broadband light storage in a room-temperature Raman memory, implemented both in free space and, for the first time, inside a low-finesse optical cavity designed for low-noise operation. The ability of the Raman memory to preserve phase coherence was tested by storing coherent polarisation states in two spatially separate atomic ensembles. Polarisation storage with a fidelity of up to 97 ± 1% was demonstrated by performing full process tomography on the system. The Raman memory was then interfaced for the first time with a spontaneous parametric downconversion (SPDC) source of heralded, GHz-bandwidth single photons. The memory performance was characterised by measuring the second-order autocorrelation of the retrieved fields. While the SPDC input photon statistics showed a clear influence on the statistics of the retrieved field, four-wave mixing (FWM) noise, stimulated by spontaneous Raman scattering, prevented the preservation of non-classical photon statistics during read-out. Suppressing this source of noise represents the last remaining challenge for realising a broadband single-photon Raman memory suitable for quantum information applications. To this end, I demonstrate a novel cavity implementation of the Raman memory which reduces the FWM contribution relative to the signal field by re-distributing the density of states into which the noise photons can be scattered. Cavity-enhanced memory operation was investigated using weak coherent input states, showing a significant improvement of the signal-to-noise ratio compared to the free-space memory implementation. This proof-of-principle demonstration suggests that cavity Raman memories may offer a practical route towards low-noise, high-bandwidth quantum storage at room temperature.