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arXiv:1804.10558 · New Journal of Physics

Optimal storage of a single photon by a single intra-cavity atom

Luigi Giannelli, Tom Schmit, Tommaso Calarco, Christiane P. Koch, Stephan Ritter, Giovanna Morigi

Published Oct 10, 2018• 41 citations
arXivHTMLPDF

Abstract

We theoretically analyze the efficiency of a quantum memory for single photons. The photons propagate along a transmission line and impinge on one of the mirrors of a high-finesse cavity. The quantum memory is constituted by a single atom within the optical resonator. Photon storage is realized by the controlled transfer of the photonic excitation into a metastable state of the atom and occurs via a Raman transition with a suitably tailored laser pulse, which drives the atom. Our study is supported by numerical simulations, in which we include the modes of the transmission line and we use the experimental parameters of existing experimental setups. It reproduces the results derived using input–output theory in the corresponding regimes and can be extended to compute dynamics where the input–output formalism cannot be straightforwardly applied. Our analysis determines the maximal storage efficiency, namely, the maximal probability to store the photon in a stable atomic excitation, in the presence of spontaneous decay and cavity parasitic losses. It further delivers the form of the laser pulse that achieves the maximal efficiency by partially compensating parasitic losses. We numerically assess the conditions under which storage based on adiabatic dynamics is preferable to non-adiabatic pulses. Moreover, we systematically determine the shortest photon pulse that can be efficiently stored as a function of the system parameters.

DOI
10.1088/1367-2630/aae725

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We theoretically analyze the efficiency of a quantum memory for single photons. The photons propagate along a transmission line and impinge on one of the mirrors of a high-finesse cavity. The quantum memory is constituted by a single atom within the optical resonator. Photon storage is realized by the controlled transfer of the photonic excitation into a metastable state of the atom and occurs via a Raman transition with a suitably tailored laser pulse, which drives the atom. Our study is supported by numerical simulations, in which we include the modes of the transmission line and we use the experimental parameters of existing experimental setups. It reproduces the results derived using input–output theory in the corresponding regimes and can be extended to compute dynamics where the input–output formalism cannot be straightforwardly applied. Our analysis determines the maximal storage efficiency, namely, the maximal probability to store the photon in a stable atomic excitation, in the presence of spontaneous decay and cavity parasitic losses. It further delivers the form of the laser pulse that achieves the maximal efficiency by partially compensating parasitic losses. We numerically assess the conditions under which storage based on adiabatic dynamics is preferable to non-adiabatic pulses. Moreover, we systematically determine the shortest photon pulse that can be efficiently stored as a function of the system parameters.
Abstract Attenuated laser pulses are often employed in place for single photons in order to test the efficiency of the elements of a quantum network. In this work we analyze theoretically the dynamics of storage of an attenuated light pulse (where the pulse intensity is at the single photon level) propagating along a transmission line and impinging on the mirror of a high finesse cavity. Storage is realized by the controlled transfer of the photonic excitations into a metastable state of an atom confined inside the cavity and occurs via a Raman transition with a suitably tailored laser pulse, which drives the atom and minimizes reflection at the cavity mirror. We determine the storage efficiency of the weak coherent pulse which is reached by protocols optimized for single-photon storage. We determine the figures of merit and we identify the conditions on an arbitrary pulse for which the storage dynamics approaches the one of a single photon. Our formalism can be extended to arbitrary types of input pulses and to quantum memories composed by spin ensembles, and serves as a basis for identifying the optimal protocols for storage and readout.
We show how to capture a single photon of arbitrary temporal shape with one atom coupled to an optical cavity. Our model applies to Raman transitions in three-level atoms with one branch of the transition controlled by a (classical) laser pulse, and the other coupled to the cavity. Photons impinging on the cavity normally exhibit partial reflection, transmission, and/or absorption by the atom. Only a control pulse of suitable temporal shape ensures impedance matching throughout the pulse, which is necessary for complete state mapping from photon to atom. For most possible photon shapes, we derive an unambiguous analytic expression for the shape of this control pulse, and we discuss how this relates to a quantum memory.
A single rubidium atom trapped within a high-finesse optical cavity is an efficient source of single photons. We theoretically and experimentally study single-photon generation using a vacuum stimulated Raman adiabatic passage. We experimentally achieve photon generation efficiencies of up to 34% and 56% on the D1{D}_{1}D1​ and D2{D}_{2}D2​ line, respectively. Output coupling with 89% results in record-high efficiencies for single photons in one spatiotemporally well-defined propagating mode. We demonstrate that the observed generation efficiencies are constant in a wide range of applied pump laser powers and virtual level detunings. This allows for independent control over the frequency and wave packet envelope of the photons without loss in efficiency. In combination with the long trapping time of the atom in the cavity, our system constitutes a significant advancement toward an on-demand, highly efficient single-photon source for quantum information processing tasks.
Ideal photonic quantum memories can store arbitrary pulses of light with unit efficiency. This requires operating in the adiabatic regime, where pulses have a duration much longer than the bandwidth of the memory. In the nonadiabatic regime of short pulses, memories are therefore imperfect, and information is always lost. We theoretically investigate the bandwidth limitations for setups based on individual atoms, or ensembles thereof, confined inside optical cavities. We identify an effective strategy for optimizing the efficiencies of the storage and retrieval process regardless of the duration or the shape of the pulses. Our protocol is derived almost completely analytically and attains efficiencies that are comparable to those obtained by numerical optimization. Furthermore, our results provide an improved understanding of the performance of quantum memories in several regimes. When considering pulses defined on an infinite time interval, the shapes can be divided into two categories, depending on their asymptotic behaviors. If the intensity of the pulse increases with time slower than or as an exponential function then the storage efficiency is only limited by the pulse width. For pulses defined on a finite interval, on the other hand, the efficiency is determined by the shape at the beginning of the storage or, correspondingly, at the end of the retrieval process.
We theoretically studied the implementation of a quantum memory and an optical transistor in a system composed by a single atom trapped inside a high finesse cavity. In order to store and map the quantum state of an input pulse onto internal states of the single atom (quantum memory) we employ the electromagnetically induced transparency (EIT) phenomenon (which can work out as an optical transistor) where the information can be transferred to the dark state of the atom modelled by a three-level system in a Λ-type configuration. In our model we consider a suitable temporal shape for the control field that ensures the adiabaticity of the storage process and retrieval of the probe pulse. The dynamic of the field inside the cavity was obtained by master equation approach, while the outside field was calculated by input-output formalism. We have analysed two different setups: i) two-sided and ii) single-sided cavities. While the first setup is the most appropriate and commonly used to observe cavity-EIT in the transmission spectrum, thus the best configuration for the optical transistor, the maximum quantum memory efficiency can not reach reasonable values, being limited to 50% for symmetric cavities. On the other hand, with single-sided cavity the quantum memory efficiency increases considerably and can reach values close to 100% in the strong atom-field coupling regime. However this specific setup is not favourable to observe the cavity-EIT effect in the transmission spectrum and then it is not appropriate to control the transmission of light pulses.
Taking the non-Markovian effect into account, we study how to store a single photon of arbitrary temporal shape in a single atom coupled to an optical cavity. Our model applies to Raman transitions in three-level atoms, with one branch of the transition controlled by a driving pulse, and the other coupled to the cavity. For any couplings of input field to the optical cavity and detunings of the atom from the driving pulse and cavity, we extend the input-output relation from Markovian to non-Markovian dynamics. For most possible photon shapes, we derive an analytic expression for the driving pulse in order to completely map the input photon into the atom. We find that the amplitude of the driving pulse depends only on the detuning of the atom from the frequency of the cavity, i.e., the detuning of the atom to the driving pulse has no effect on the strength of the driving pulse.