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arXiv:2401.17368 · Physical review. B./Physical review. B

Floquet-Bloch theory for nonperturbative response to a static drive

Christophe De Beule, Steven Gassner, Spenser Talkington, E. J. Melé

Published Jun 17, 2024• 6 citations
arXivHTMLPDF

Abstract

We develop the Floquet-Bloch theory of noninteracting fermions on a periodic lattice in the presence of a constant electric field. As long as the field lies along a reciprocal-lattice vector, time periodicity of the Bloch Hamiltonian is inherited from the evolution of momentum in the Brillouin zone. The corresponding Floquet quasienergies yield the Wannier-Stark ladder with interband couplings included to all orders. These results are compared to perturbative results where the lowest-order interband correction gives the field-induced polarization shift in terms of the electric susceptibility. Additionally, we investigate electronic transport by coupling the system to a bath within the Floquet-Keldysh formalism. We then study the breakdown of the band-projected theory from the onset of interband contributions and Landau-Zener resonances in the band-resolved currents. In particular, we consider the transverse quantum-geometric response in two spatial dimensions due to the Berry curvature. In the strong-field regime, the semiclassical theory predicts a plateau of the geometric response as a function of field strength. Here, we scrutinize the conditions under which the semiclassical results continue to hold in the quantum theory.

DOI
10.1103/physrevb.109.235421

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We develop the Floquet-Bloch theory of noninteracting fermions on a periodic lattice in the presence of a constant electric field. As long as the field lies along a reciprocal-lattice vector, time periodicity of the Bloch Hamiltonian is inherited from the evolution of momentum in the Brillouin zone. The corresponding Floquet quasienergies yield the Wannier-Stark ladder with interband couplings included to all orders. These results are compared to perturbative results where the lowest-order interband correction gives the field-induced polarization shift in terms of the electric susceptibility. Additionally, we investigate electronic transport by coupling the system to a bath within the Floquet-Keldysh formalism. We then study the breakdown of the band-projected theory from the onset of interband contributions and Landau-Zener resonances in the band-resolved currents. In particular, we consider the transverse quantum-geometric response in two spatial dimensions due to the Berry curvature. In the strong-field regime, the semiclassical theory predicts a plateau of the geometric response as a function of field strength. Here, we scrutinize the conditions under which the semiclassical results continue to hold in the quantum theory.
We study a periodically driven Bloch system connected to a heat bath by introducing a formalism that combines the Floquet analysis and the quantum Liouville equation. We first obtain the density matrix for such a system without electron-electron interactions, and find that by turning off the thermal contact, the system goes into a diagonal ensemble where the density matrix is diagonal under the Floquet-Bloch eigenbasis. We then calculate the current response that consists of a dissipationless intrinsic part and a dissipative extrinsic correction to the first order in damping. The correction originates from a shift in polarization between the diagonal ensemble and a Bloch thermal equilibrium. We further apply the result to a two-band model with broken time-reversal and inversion symmetries revealing the role of the external driven field strength.
Nonequilibrium quantum physics greatly simplifies in the case of time-periodic Hamiltonians, since Floquet theory provides an analog to Bloch's theorem in the time domain. Still, the formal properties of Floquet many-body theory remain underexplored. Here, we study what happens to the uniform electron gas when a space-time periodic potential of arbitrary strength is applied, which leads to band splitting. The case of a potential traveling at constant speed is special, since the problem can be made time independent by transforming to a comoving frame. We perform linear-response theory, in the sense that we apply an additional perturbatively small but nonperiodic probing field, for which we illustrate the analogy of Fermi's golden rule and the photoemission spectrum of a many-electron system. As in the equilibrium case, the latter is related to the spectral function which is positive definite. We also analyze the parameter dependence of the controllable photoemission spectra by virtue of Floquet-Bloch engineering.
We consider an infinite one dimensional array of alternating charges embedded in a two-dimensional configuration space and subjected to a weak static electric field transverse to the lattice axis. Expansion of the Coulomb interaction about a lattice site gives a transverse restoring stiffness κ∝ζ(3)/L3κ\propto ζ(3)/L^3κ∝ζ(3)/L3, defining the oscillator length aya_yay​, while Bloch periodicity is retained along the lattice direction and the transverse motion is represented in a harmonic basis. The Coulomb matrix elements are governed by the dimensionless scale ηr−sη_{r-s}ηr−s​, which couples the reciprocal-lattice transfer to the transverse oscillator length. A regularized one dimensional extension is also introduced through Coulomb regularization, yielding a finite diagonal offset and an exponentially decaying even-transfer coupling in reciprocal space. Small ηr−sη_{r-s}ηr−s​ yields logarithmic, parity-dependent transverse-state coupling, while large ηr−sη_{r-s}ηr−s​ approaches the one-dimensional Coulomb limit. In the finite-order spectrum, the latter approaches the Kronig Penney reference toward the band edge while retaining distinct Brillouin zone curvature. The formulation therefore identifies two characteristic quantities of the alternating lattice: the transverse restoring stiffness and the one-dimensional Madelung form, while retaining the two dimensional structure required to describe the response to a transverse electric field. Keywords: alternating charge lattice; Bloch states; Coulomb interaction; transverse electric field; regularization; reciprocal space coupling; Brillouin zone spectrum.
We construct a systematic high-frequency expansion for periodically driven quantum systems based on the Brillouin-Wigner (BW) perturbation theory, which generates an effective Hamiltonian on the projected zero-photon subspace in the Floquet theory, reproducing the quasienergies and eigenstates of the original Floquet Hamiltonian up to desired order in $1/\ensuremath{\omega}$, with $\ensuremath{\omega}$ being the frequency of the drive. The advantage of the BW method is that it is not only efficient in deriving higher-order terms, but even enables us to write down the whole infinite series expansion, as compared to the van Vleck degenerate perturbation theory. The expansion is also free from a spurious dependence on the driving phase, which has been an obstacle in the Floquet-Magnus expansion. We apply the BW expansion to various models of noninteracting electrons driven by circularly polarized light. As the amplitude of the light is increased, the system undergoes a series of Floquet topological-to-topological phase transitions, whose phase boundary in the high-frequency regime is well explained by the BW expansion. As the frequency is lowered, the high-frequency expansion breaks down at some point due to band touching with nonzero-photon sectors, where we find numerically even more intricate and richer Floquet topological phases spring out. We have then analyzed, with the Floquet dynamical mean-field theory, the effects of electron-electron interaction and energy dissipation. We have specifically revealed that phase transitions from Floquet-topological to Mott insulators emerge, where the phase boundaries can again be captured with the high-frequency expansion.
We develop a geometric perturbation theory of Bloch states for perturbations coupling via the interband Berry connection. The gauge-invariant Bargmann trace builds the dressed dispersion and connection order by order as a hierarchy Q(N)Q^{(N)}Q(N), starting with the quantum geometric tensor. Higher members encode multiband geometry beyond the quantum metric and Berry curvature. Connected amplitudes control vertex-order corrections, while strict-order corrections reduce to disconnected products. For a uniform electric field we find the fully coherent, purely geometric sector of the third-order response.
Topological properties lie at the heart of many fascinating phenomena in solid-state systems such as quantum Hall systems or Chern insulators. The topology of the bands can be captured by the distribution of Berry curvature, which describes the geometry of the eigenstates across the Brillouin zone. Using fermionic ultracold atoms in a hexagonal optical lattice, we engineered the Berry curvature of the Bloch bands using resonant driving and show a full momentum-resolved measurement of the ensuing Berry curvature. Our results pave the way to explore intriguing phases of matter with interactions in topological band structures.