We study the applicability of the Liouvillian exceptional points (LEPs) approach to nanoscale open quantum systems. A generic model of the driven two-level system in a thermal environment is analyzed within the nonequilibrium Green's function (NEGF) and Bloch quantum master equation formulations. We derive the latter starting from the exact NEGF Dyson equations and highlight the qualitative limitations of the LEP treatment by examining the approximations employed in its derivation. We find that the non-Markov character of evolution in open quantum systems does not allow for the introduction of the concept of exceptional points for a description of their dynamics. Theoretical analysis is illustrated with numerical simulations.
We study the applicability of the Liouvillian exceptional points (LEPs) approach to nanoscale open quantum systems. A generic model of the driven two-level system in a thermal environment is analyzed within the nonequilibrium Green's function (NEGF) and Bloch quantum master equation formulations. We derive the latter starting from the exact NEGF Dyson equations and highlight the qualitative limitations of the LEP treatment by examining the approximations employed in its derivation. We find that the non-Markov character of evolution in open quantum systems does not allow for the introduction of the concept of exceptional points for a description of their dynamics. Theoretical analysis is illustrated with numerical simulations.
Recent years have seen a surge of interest in exceptional points in open quantum systems. The natural approach in this area has been the use of Markovian master equations. While the resulting Liouvillian EPs have been seen in a variety of systems and have been associated to numerous exotic effects, it is an open question whether such degeneracies and their peculiarities can persist beyond the validity of master equations. In this work, taking the example of a dissipative double-quantum-dot system, we show that exact Heisenberg equations governing system and bath dynamics exhibit the same EPs as the corresponding master equations. To highlight the importance of this finding, we prove that the paradigmatic property associated to EPs – critical damping, persists well beyond the validity of master equations. Our results demonstrate that Liouvillian EPs can arise from underlying fundamental exact principles, rather than merely as a consequence of approximations involved in deriving master equations.
Abstract Hamiltonian exceptional points (HEPs) are spectral degeneracies of non-Hermitian Hamiltonians describing classical and semiclassical open systems with losses and/or gain. However, this definition overlooks the occurrence of quantum jumps in the evolution of open quantum systems. These quantum effects are properly accounted for by considering quantum Liouvillians and their exceptional points (LEPs). Specifically, an LEP corresponds to the coalescence of two or more eigenvalues and the corresponding eigenmatrices of a given Liouvillian at critical values of external parameters (Minganti et al 2019 Phys. Rev. A 100 062131). Here, we explicitly describe how standard quantum process tomography, which reveals the dynamics of a quantum system, can be readily applied to detect and characterize quantum LEPs of quantum non-Hermitian systems. We conducted experiments on an IBM quantum processor to implement a prototype model with one-, two-, and three qubits simulating the decay of a single qubit through competing channels, resulting in LEPs but not HEPs. Subsequently, we performed tomographic reconstruction of the corresponding experimental Liouvillian and its LEPs using both single- and two-qubit operations. This example underscores the efficacy of process tomography in tuning and observing LEPs even in the absence of HEPs.
Abstract Exceptional points are the branch-point singularities of non-Hermitian Hamiltonians and have rich consequences in open-system dynamics. While the exceptional points and their critical phenomena are widely studied in the non-Hermitian settings without quantum jumps, they also emerge in open quantum systems depicted by the Lindblad master equations, wherein they are identified as the degeneracies in the Liouvillian eigenspectrum. These Liouvillian exceptional points often have distinct properties compared to their counterparts in non-Hermitian Hamiltonians, leading to fundamental modifications of the steady states or the steady-state-approaching dynamics. Since the Liouvillian exceptional points widely exist in quantum systems such as the atomic vapors, superconducting qubits, and ultracold ions and atoms, they have received increasing amount of attention of late. Here, we present a brief review on an important aspect of the dynamic consequence of Liouvillian exceptional points, namely the chiral state transfer induced by the parametric encircling the Liouvillian exceptional points. Our review focuses on the theoretical description and experimental observation of the phenomena in atomic systems that are experimentally accessible. We also discuss the ongoing effort to unveil the collective dynamic phenomena close to the Liouvillian exceptional points, as a consequence of the many-body effects therein. Formally, these phenomena are the quantum-many-body counterparts to those in classical open systems with nonlinearity, but hold intriguing new potentials for quantum applications.
Abstract Exceptional points in non-Hermitian quantum systems give rise to genuine quantum phenomena. Recent explorations of exceptional-point-induced phase transitions have extended from discrete-variable to continuous-variable-encoded quantum systems. However, phase transitions driven by Liouvillian exceptional points (LEPs) in continuous-variable platforms remain largely unexplored. Here, we construct and investigate a Liouvillian exceptional structure based on a driven-dissipative Kerr-cat qubit. Through numerical simulations, we numerically reveal a non-Hermitian phase transition occurring at the LEP characterized by a sudden change in dynamical behavior from underdamped oscillations to overdamped relaxations as visualized via Wigner functions and Bloch sphere trajectories. The dynamical pattern of Wigner interference fringes provides a phase-space signature of the LEP-induced phase transition, while Wigner negativity certifies the genuine quantum nonclassicality of the system. Our results establish the Kerr-cat qubit as a continuous-variable setting for exploring dissipative quantum criticality and intrinsic non-Hermitian physics.
We investigate speeding up of relaxation of Markovian open quantum systems with the Liouvillian exceptional point (LEP), where the slowest decay mode degenerates with a faster decay mode. The degeneracy significantly increases the gap of the Liouvillian operator, which determines the time scale of such systems in converging to stationarity and thus accelerates the relaxation process. We explore an experimentally relevant three-level atomic system whose eigenmatrices and eigenspectra are obtained completely analytically. This allows us to gain insights into the LEP and examine the respective dynamics with details. We illustrate that the gap can be further widened by Floquet engineering, which further accelerates the relaxation process. Finally, we extend this approach to analyze laser cooling of trapped ions, where vibrations (phonons) couple to the electronic states. An optimal cooling condition is obtained analytically, which agrees with both existing experiments and numerical simulations. In this paper, we provide analytical insights into understanding LEP as well as controlling and optimizing the dissipative dynamics of atoms and trapped ions.
Exceptional points in non-Hermitian quantum systems give rise to novel genuine quantum phenomena. Recent explorations of exceptional-point-induced quantum phase transitions have extended from discrete-variable to continuous-variable-encoded quantum systems. However, quantum phase transitions driven by Liouvillian exceptional points (LEPs) in continuous-variable platforms remain largely unexplored. Here, we construct and investigate a Liouvillian exceptional structure based on a driven-dissipative Kerr-cat qubit. Through numerical simulations, we reveal a quantum phase transition occurring at the LEP characterized by a sudden change in dynamical behavior from underdamped oscillations to overdamped relaxations as visualized via Wigner functions and Bloch sphere trajectories. Notably the negativity of the Wigner function serves as a direct signature of genuine quantum coherence unattainable in conventional single-qubit non-Hermitian systems. Furthermore, we introduce the phase difference between the off-diagonal elements of the Liouvillian eigenmatrices as a novel parameter to quantify the transition. Our results establish the Kerr-cat qubit as a novel continuous-variable setting for exploring dissipative quantum criticality and intrinsic non-Hermitian physics.