Abstract Exceptional points are the branch-point singularities of non-Hermitian Hamiltonians and have rich consequences in open-system dynamics. While the exceptional points and their critical phenomena are widely studied in the non-Hermitian settings without quantum jumps, they also emerge in open quantum systems depicted by the Lindblad master equations, wherein they are identified as the degeneracies in the Liouvillian eigenspectrum. These Liouvillian exceptional points often have distinct properties compared to their counterparts in non-Hermitian Hamiltonians, leading to fundamental modifications of the steady states or the steady-state-approaching dynamics. Since the Liouvillian exceptional points widely exist in quantum systems such as the atomic vapors, superconducting qubits, and ultracold ions and atoms, they have received increasing amount of attention of late. Here, we present a brief review on an important aspect of the dynamic consequence of Liouvillian exceptional points, namely the chiral state transfer induced by the parametric encircling the Liouvillian exceptional points. Our review focuses on the theoretical description and experimental observation of the phenomena in atomic systems that are experimentally accessible. We also discuss the ongoing effort to unveil the collective dynamic phenomena close to the Liouvillian exceptional points, as a consequence of the many-body effects therein. Formally, these phenomena are the quantum-many-body counterparts to those in classical open systems with nonlinearity, but hold intriguing new potentials for quantum applications.
Abstract Exceptional points are the branch-point singularities of non-Hermitian Hamiltonians and have rich consequences in open-system dynamics. While the exceptional points and their critical phenomena are widely studied in the non-Hermitian settings without quantum jumps, they also emerge in open quantum systems depicted by the Lindblad master equations, wherein they are identified as the degeneracies in the Liouvillian eigenspectrum. These Liouvillian exceptional points often have distinct properties compared to their counterparts in non-Hermitian Hamiltonians, leading to fundamental modifications of the steady states or the steady-state-approaching dynamics. Since the Liouvillian exceptional points widely exist in quantum systems such as the atomic vapors, superconducting qubits, and ultracold ions and atoms, they have received increasing amount of attention of late. Here, we present a brief review on an important aspect of the dynamic consequence of Liouvillian exceptional points, namely the chiral state transfer induced by the parametric encircling the Liouvillian exceptional points. Our review focuses on the theoretical description and experimental observation of the phenomena in atomic systems that are experimentally accessible. We also discuss the ongoing effort to unveil the collective dynamic phenomena close to the Liouvillian exceptional points, as a consequence of the many-body effects therein. Formally, these phenomena are the quantum-many-body counterparts to those in classical open systems with nonlinearity, but hold intriguing new potentials for quantum applications.
Exceptional points emerge in the complex eigenspectra of non-Hermitian systems, and give rise to rich critical behaviors. An outstanding example is the chiral state transfer, where states can swap under an adiabatic encircling around the exceptional point, but only along one direction. In dissipative quantum systems, such exceptional-point encirclings are often accompanied by decoherence, whose impact is beyond the description of non-Hermitian Hamiltonians. In this paper, we study in detail the effects of dephasing on the encircling dynamics, adopting the full Lindblad master equation. Introducing experimentally relevant quantum-jump processes that account for dephasing, we show that gaps emerge in the eigenspectra landscape of the corresponding Liouvillian superoperator. It follows that the chiral state transfer does not take place in the adiabatic limit, since the system always adiabatically follows the quasisteady state of the Liouvillian regardless of the encircling direction. Nevertheless, the chirality is restored at intermediate encircling times, where the dynamics is nonadiabatic in both encircling directions, distinct from the typical chiral state transfer in non-Hermitian systems. While our results are applicable to several recent experiments, we examine a recent cold-atom experiment in particular, and show that the observed long-time chirality is limited to the special encircling path therein. Our paper provides further insight into the chiral state transfer under experimental conditions, and is helpful for controlling open-system dynamics from the perspective of non-Hermitian physics.
As branch-point singularities of non-Hermitian matrices, the exceptional points (EPs) exhibit unique spectral topology and criticality, with intriguing dynamic consequences in non-Hermitian settings. In quantum open systems, EPs also emerge in the Liouvillian spectrum, but their dynamic impact often pertains to the transient dynamics and is challenging to demonstrate. Here, using the flexible control afforded by single-photon interferometry, we study the chiral state transfer when the Liouvillian EP is parametrically encircled. Reconstructing the density-matrix evolution by experimentally simulating the quantum Langevin equation, we show that the chirality of the dynamics is only present within an intermediate encircling timescale and dictated by the landscape of the Liouvillian spectrum near the EP. However, the chirality disappears at long times as the system always relaxes to the steady state. We then demonstrate the power-law decay of the chirality in regard to the encircling time with a parameter-dependent exponent. Our experiment confirms the transient nature of chiral state transfer near a Liouvillian EP in quantum open systems, while our scheme paves the way for simulating general open-system dynamics using single photons.
Open quantum systems interacting with an environment exhibit dynamics described by the combination of dissipation and coherent Hamiltonian evolution. Taken together, these effects are captured by a Liouvillian superoperator. The degeneracies of the (generically non-Hermitian) Liouvillian are exceptional points, which are associated with critical dynamics as the system approaches steady state. We use a superconducting transmon circuit coupled to an engineered environment to observe two different types of Liouvillian exceptional points that arise either from the interplay of energy loss and decoherence or purely due to decoherence. By dynamically tuning the Liouvillian superoperators in real time we observe a non-Hermiticity-induced chiral state transfer. Our study motivates a new look at open quantum system dynamics from the vantage of Liouvillian exceptional points, enabling applications of non-Hermitian dynamics in the understanding and control of open quantum systems.
Abstract Hamiltonian exceptional points (HEPs) are spectral degeneracies of non-Hermitian Hamiltonians describing classical and semiclassical open systems with losses and/or gain. However, this definition overlooks the occurrence of quantum jumps in the evolution of open quantum systems. These quantum effects are properly accounted for by considering quantum Liouvillians and their exceptional points (LEPs). Specifically, an LEP corresponds to the coalescence of two or more eigenvalues and the corresponding eigenmatrices of a given Liouvillian at critical values of external parameters (Minganti et al 2019 Phys. Rev. A 100 062131). Here, we explicitly describe how standard quantum process tomography, which reveals the dynamics of a quantum system, can be readily applied to detect and characterize quantum LEPs of quantum non-Hermitian systems. We conducted experiments on an IBM quantum processor to implement a prototype model with one-, two-, and three qubits simulating the decay of a single qubit through competing channels, resulting in LEPs but not HEPs. Subsequently, we performed tomographic reconstruction of the corresponding experimental Liouvillian and its LEPs using both single- and two-qubit operations. This example underscores the efficacy of process tomography in tuning and observing LEPs even in the absence of HEPs.
The exceptional point has presented considerably interesting and counterintuitive phenomena associated with nonreciprocity, precision measurement, and topological dynamics. The Liouvillian exceptional point (LEP), involving the interplay of energy loss and decoherence inherently relevant to quantum jumps, has recently drawn much attention due to capability to fully capture quantum system dynamics and naturally facilitate non-Hermitian quantum investigations. It was also predicted that quantum jumps could give rise to third-order LEPs in two-level quantum systems for its high dimensional Liouvillian superoperator, which, however, has never been experimentally confirmed until now. Here we report the first observation of the third-order LEPs emerging from quantum jumps in an ultracold two-level trapped-ion system. Moreover, by combining decay with dephasing processes, we present the first experimental exploration of LEPs involving combinatorial effect of decay and dephasing. In particular, due to non-commutativity between the Lindblad superoperators governing LEPs for decay and dephasing, we witness the movement of LEPs driven by the competition between decay and dephasing occurring in an open quantum system. This unique feature of non-Hermitian quantum systems paves a new avenue for modifying nonreciprocity, enhancing precision measurement, and manipulating topological dynamics by tuning the LEPs.
Open photonic systems provide a versatile platform for non-Hermitian physics, enabling control over complex spectra, transport, and light-matter interactions. Exceptional points (EPs), at which eigenvalues and eigenvectors coalesce and the governing operator becomes defective, play a central role because they combine branch-point spectral topology, nonanalytic perturbative response, and controllable eigenstate conversion. This Review provides a unified framework for EP photonics by systematically distinguishing exceptional degeneracies according to the underlying operator, spectral variable, boundary conditions, and experimentally accessible observables. We discuss Hamiltonian EPs, absorbing EPs associated with scattering zeros, real-frequency scattering-matrix and Jones-matrix EPs, Bloch and Floquet EPs, and Liouvillian EPs in open quantum systems. We review their spectral topology, static and dynamical encircling, higher-order exceptional structures, and coexistence with bound states in the continuum, together with applications in sensing, lasing, coherent absorption, directional scattering, polarization and wavefront control, nonlinear optics, optical storage, nonreciprocal photonics, and quantum photonics. We also critically assess the current limitations, practical challenges, and future perspectives of EP-based photonic technologies, with particular attention to robustness, noise, scalability, and experimentally measurable performance.