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arXiv:2512.01217 · Nature Communications

Experimental Witness of Quantum Jump Induced High-Order Liouvillian Exceptional Points

Zhuo-Zhu Wu, Pei-Dong Li, Tai-Hao Cui, Jia-Wei Wang, Yuan-Zhang Dong, Shuang-Qing Dai, Ji Li, Ya-Qi Wei, Quan Yuan, Xiao-Ming Cai, Liang Chen, Jian-Qi Zhang, Hui Jing, Mang Feng

quant-phSubmitted Dec 1, 2025• Announced Dec 2, 2025• 8 citations
arXivHTMLPDF

Abstract

The exceptional point has presented considerably interesting and counterintuitive phenomena associated with nonreciprocity, precision measurement, and topological dynamics. The Liouvillian exceptional point (LEP), involving the interplay of energy loss and decoherence inherently relevant to quantum jumps, has recently drawn much attention due to capability to fully capture quantum system dynamics and naturally facilitate non-Hermitian quantum investigations. It was also predicted that quantum jumps could give rise to third-order LEPs in two-level quantum systems for its high dimensional Liouvillian superoperator, which, however, has never been experimentally confirmed until now. Here we report the first observation of the third-order LEPs emerging from quantum jumps in an ultracold two-level trapped-ion system. Moreover, by combining decay with dephasing processes, we present the first experimental exploration of LEPs involving combinatorial effect of decay and dephasing. In particular, due to non-commutativity between the Lindblad superoperators governing LEPs for decay and dephasing, we witness the movement of LEPs driven by the competition between decay and dephasing occurring in an open quantum system. This unique feature of non-Hermitian quantum systems paves a new avenue for modifying nonreciprocity, enhancing precision measurement, and manipulating topological dynamics by tuning the LEPs.

Comments
24 pages, 5 figures. Supplymentary material is inclosed in the TeX Source. Accepted by Nature Communications

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The exceptional point has presented considerably interesting and counterintuitive phenomena associated with nonreciprocity, precision measurement, and topological dynamics. The Liouvillian exceptional point (LEP), involving the interplay of energy loss and decoherence inherently relevant to quantum jumps, has recently drawn much attention due to capability to fully capture quantum system dynamics and naturally facilitate non-Hermitian quantum investigations. It was also predicted that quantum jumps could give rise to third-order LEPs in two-level quantum systems for its high dimensional Liouvillian superoperator, which, however, has never been experimentally confirmed until now. Here we report the first observation of the third-order LEPs emerging from quantum jumps in an ultracold two-level trapped-ion system. Moreover, by combining decay with dephasing processes, we present the first experimental exploration of LEPs involving combinatorial effect of decay and dephasing. In particular, due to non-commutativity between the Lindblad superoperators governing LEPs for decay and dephasing, we witness the movement of LEPs driven by the competition between decay and dephasing occurring in an open quantum system. This unique feature of non-Hermitian quantum systems paves a new avenue for modifying nonreciprocity, enhancing precision measurement, and manipulating topological dynamics by tuning the LEPs.
Non-Hermitian (NH) systems can display exotic topological phenomena without Hermitian counterparts, enabled by exceptional points (EPs). So far, investigations of NH topology have been restricted to EPs of the NH Hamiltonian, which governs the system dynamics conditional upon no quantum jumps occurring. The Liouvillian superoperator, which combines the effects of quantum jumps with NH Hamiltonian dynamics, possesses EPs (LEPs) that are significantly different from those of the corresponding NH Hamiltonian. We here study the topological features of the LEPs in the system consisting of a qubit coupled to a non-Markovian reservoir. We find that two distinct winding numbers can be simultaneously produced by executing a single closed path encircling the twofold LEP2, formed by two coinciding LEP2s, each involving a pair of coalescing eigenvectors of the extended Liouvillian superoperator. We experimentally demonstrate this purely non-Markovian phenomenon with a circuit, where a superconducting qubit is coupled to a decaying resonator which acts as a reservoir with memory effects. The results push the exploration of exceptional topology from the Markovian to non-Markovian regime.
Abstract Hamiltonian exceptional points (HEPs) are spectral degeneracies of non-Hermitian Hamiltonians describing classical and semiclassical open systems with losses and/or gain. However, this definition overlooks the occurrence of quantum jumps in the evolution of open quantum systems. These quantum effects are properly accounted for by considering quantum Liouvillians and their exceptional points (LEPs). Specifically, an LEP corresponds to the coalescence of two or more eigenvalues and the corresponding eigenmatrices of a given Liouvillian at critical values of external parameters (Minganti et al 2019 Phys. Rev. A 100 062131). Here, we explicitly describe how standard quantum process tomography, which reveals the dynamics of a quantum system, can be readily applied to detect and characterize quantum LEPs of quantum non-Hermitian systems. We conducted experiments on an IBM quantum processor to implement a prototype model with one-, two-, and three qubits simulating the decay of a single qubit through competing channels, resulting in LEPs but not HEPs. Subsequently, we performed tomographic reconstruction of the corresponding experimental Liouvillian and its LEPs using both single- and two-qubit operations. This example underscores the efficacy of process tomography in tuning and observing LEPs even in the absence of HEPs.
The intriguing physical phenomena associated with exceptional points have established non-Hermitian physics as a frontier of modern research. Recent investigations have extended non-Hermitian physics into the fully quantum domain. However, existing studies predominantly concentrate on discrete-variable quantum systems, while non-Hermitian quantum effects in continuous-variable encoded systems remain largely unexplored. In this work, we investigate the exceptional structure for a driven-dissipative Kerr-cat qubit, realized with a Kerr nonlinear resonator. We find that the dissipation leads to a bidirectional jump between the two basis states of the cat qubit, which is in distinct contrast with the unidirectional jump associated with normal two-level systems. The competition between this jump and a single-photon drive gives arise to the emergence of third-order Liouvillian exceptional points (LEP3s), each corresponds to a crossing point of two lines of LEP2s. We further show that the LEP3 can exhibit the topological character of the Hamiltonian EP3s, which cannot be realized with a single qubit. Our work opens the possibility of realizing non-Hermitian phenomena with continuous-variable quantum systems.
Hermiticity in quantum mechanics ensures the reality of energies, while parity-time symmetry offers an alternative route. Interestingly, in a three-level system, parity-time symmetry-breaking can lead to third-order exceptional points with distinctive topological properties. Experimentally implementing this in open quantum systems requires two well-controlled loss channels, resulting in dynamics that challenges a pure non-Hermitian description. Here we address the challenge by employing two approaches to eliminate the effects of quantum jump terms, ensuring pure non-Hermitian dynamics in a dissipative trapped ion. Based on this, we experimentally observe a parity-time symmetry-breaking-induced third-order exceptional point through non-Hermitian absorption spectroscopy. Quantum state tomography further demonstrates the coalescence of three eigenstates into a single eigenstate at the exceptional point. Finally, we identify an intrinsic third-order Liouvillian exceptional point via quench dynamics. Our experiments can be extended to observe other non-Hermitian phenomena involving multiple dissipative levels and potentially find applications in quantum information technology. Parity-time symmetry breaking and related non-Hermitian phenomena, such as high-order exceptional points, have attracted significant interest across various experimental platforms. Here the authors demonstrate a third-order exceptional point induced by parity-time symmetry breaking in a dissipative trapped ion.
Abstract Exceptional points are the branch-point singularities of non-Hermitian Hamiltonians and have rich consequences in open-system dynamics. While the exceptional points and their critical phenomena are widely studied in the non-Hermitian settings without quantum jumps, they also emerge in open quantum systems depicted by the Lindblad master equations, wherein they are identified as the degeneracies in the Liouvillian eigenspectrum. These Liouvillian exceptional points often have distinct properties compared to their counterparts in non-Hermitian Hamiltonians, leading to fundamental modifications of the steady states or the steady-state-approaching dynamics. Since the Liouvillian exceptional points widely exist in quantum systems such as the atomic vapors, superconducting qubits, and ultracold ions and atoms, they have received increasing amount of attention of late. Here, we present a brief review on an important aspect of the dynamic consequence of Liouvillian exceptional points, namely the chiral state transfer induced by the parametric encircling the Liouvillian exceptional points. Our review focuses on the theoretical description and experimental observation of the phenomena in atomic systems that are experimentally accessible. We also discuss the ongoing effort to unveil the collective dynamic phenomena close to the Liouvillian exceptional points, as a consequence of the many-body effects therein. Formally, these phenomena are the quantum-many-body counterparts to those in classical open systems with nonlinearity, but hold intriguing new potentials for quantum applications.
Open quantum systems interacting with an environment exhibit dynamics described by the combination of dissipation and coherent Hamiltonian evolution. Taken together, these effects are captured by a Liouvillian superoperator. The degeneracies of the (generically non-Hermitian) Liouvillian are exceptional points, which are associated with critical dynamics as the system approaches steady state. We use a superconducting transmon circuit coupled to an engineered environment to observe two different types of Liouvillian exceptional points that arise either from the interplay of energy loss and decoherence or purely due to decoherence. By dynamically tuning the Liouvillian superoperators in real time we observe a non-Hermiticity-induced chiral state transfer. Our study motivates a new look at open quantum system dynamics from the vantage of Liouvillian exceptional points, enabling applications of non-Hermitian dynamics in the understanding and control of open quantum systems.