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arXiv:2305.12745 · Physical Review Research

Accelerating relaxation through Liouvillian exceptional point

Yan‐Li Zhou, Xiao-Die Yu, Chun-Wang Wu, Xie-Qian Li, Jie Zhang, Weibin Li, Ping‐Xing Chen

Published Oct 11, 2023• 46 citations
arXivHTMLPDF

Abstract

We investigate speeding up of relaxation of Markovian open quantum systems with the Liouvillian exceptional point (LEP), where the slowest decay mode degenerates with a faster decay mode. The degeneracy significantly increases the gap of the Liouvillian operator, which determines the time scale of such systems in converging to stationarity and thus accelerates the relaxation process. We explore an experimentally relevant three-level atomic system whose eigenmatrices and eigenspectra are obtained completely analytically. This allows us to gain insights into the LEP and examine the respective dynamics with details. We illustrate that the gap can be further widened by Floquet engineering, which further accelerates the relaxation process. Finally, we extend this approach to analyze laser cooling of trapped ions, where vibrations (phonons) couple to the electronic states. An optimal cooling condition is obtained analytically, which agrees with both existing experiments and numerical simulations. In this paper, we provide analytical insights into understanding LEP as well as controlling and optimizing the dissipative dynamics of atoms and trapped ions.

DOI
10.1103/physrevresearch.5.043036

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We investigate speeding up of relaxation of Markovian open quantum systems with the Liouvillian exceptional point (LEP), where the slowest decay mode degenerates with a faster decay mode. The degeneracy significantly increases the gap of the Liouvillian operator, which determines the time scale of such systems in converging to stationarity and thus accelerates the relaxation process. We explore an experimentally relevant three-level atomic system whose eigenmatrices and eigenspectra are obtained completely analytically. This allows us to gain insights into the LEP and examine the respective dynamics with details. We illustrate that the gap can be further widened by Floquet engineering, which further accelerates the relaxation process. Finally, we extend this approach to analyze laser cooling of trapped ions, where vibrations (phonons) couple to the electronic states. An optimal cooling condition is obtained analytically, which agrees with both existing experiments and numerical simulations. In this paper, we provide analytical insights into understanding LEP as well as controlling and optimizing the dissipative dynamics of atoms and trapped ions.
An ancient and counterintuitive phenomenon known as the Mpemba effect (water can cool faster when initially heated up) showcases the critical role of initial conditions in relaxation processes. How to realize and utilize this effect for speeding up relaxation is an important but challenging task in purely quantum system till now. Here, we experimentally study the strong Mpemba effect in a single trapped ion system in which an exponentially accelerated relaxation in time is observed by preparing an optimal quantum initial state with no excitation of the slowest decaying mode. Also, we demonstrate that the condition of realizing such effect coincides with the Liouvillian exceptional point, featuring the coalescence of both the eigenvalues and the eigenmodes of the systems. Our work provides an efficient strategy to engineer the dynamics of open quantum system, and suggests a link unexplored yet between the Mpemba effect and the non-Hermitian physics. The Mpemba effect is an archetype for various anomalous relaxation phenomena. Here, the authors experimentally study a quantum version of the Mpemba effect in a single trapped ion system, where relaxation is exponentially accelerated by removing the excitation of the slowest decaying mode. This phenomenon, seen in Markovian open quantum systems containing Liouvillian exceptional points, indicates a link between the Mpemba effect and non-Hermitian physics.
The exceptional point has presented considerably interesting and counterintuitive phenomena associated with nonreciprocity, precision measurement, and topological dynamics. The Liouvillian exceptional point (LEP), involving the interplay of energy loss and decoherence inherently relevant to quantum jumps, has recently drawn much attention due to capability to fully capture quantum system dynamics and naturally facilitate non-Hermitian quantum investigations. It was also predicted that quantum jumps could give rise to third-order LEPs in two-level quantum systems for its high dimensional Liouvillian superoperator, which, however, has never been experimentally confirmed until now. Here we report the first observation of the third-order LEPs emerging from quantum jumps in an ultracold two-level trapped-ion system. Moreover, by combining decay with dephasing processes, we present the first experimental exploration of LEPs involving combinatorial effect of decay and dephasing. In particular, due to non-commutativity between the Lindblad superoperators governing LEPs for decay and dephasing, we witness the movement of LEPs driven by the competition between decay and dephasing occurring in an open quantum system. This unique feature of non-Hermitian quantum systems paves a new avenue for modifying nonreciprocity, enhancing precision measurement, and manipulating topological dynamics by tuning the LEPs.
Quantum batteries, which use quantum systems to store and deliver energy, are promising for next-generation energy storage. However, optimizing charging strategies and understanding the interplay between dissipation and quantum coherence remain open challenges. Here, we investigate steady-state charging in an open quantum battery and demonstrate that the charging timescale depends on the spectral gap of the Liouvillian operator governing dissipative dynamics. As a minimal example, we examine a three-level quantum battery realized in a single trapped 40Ca+{}^{40}\mathrm{Ca}^{+}40Ca+ ion, where energy from an engineered thermal photon reservoir is coherently transferred to a long-lived metastable storage state. We find that long-term dynamics are confined to a low-dimensional manifold of slow Liouvillian modes, with their spectral structure determining the relaxation rate to the charged steady state. By adjusting experimentally accessible parameters, such as reservoir occupation and coherent coupling strength, the non-Hermitian Liouvillian spectrum can approach an exceptional point. This increases the spectral gap and accelerates the approach to steady state. As a result, this mechanism significantly enhances asymptotic charging power without relying on many-body collectivity or steady coherence. Our findings offer fundamental insights into open quantum thermodynamics and provide a path to efficient energy storage and fast-charging solutions in emerging quantum technologies.
Abstract Hamiltonian exceptional points (HEPs) are spectral degeneracies of non-Hermitian Hamiltonians describing classical and semiclassical open systems with losses and/or gain. However, this definition overlooks the occurrence of quantum jumps in the evolution of open quantum systems. These quantum effects are properly accounted for by considering quantum Liouvillians and their exceptional points (LEPs). Specifically, an LEP corresponds to the coalescence of two or more eigenvalues and the corresponding eigenmatrices of a given Liouvillian at critical values of external parameters (Minganti et al 2019 Phys. Rev. A 100 062131). Here, we explicitly describe how standard quantum process tomography, which reveals the dynamics of a quantum system, can be readily applied to detect and characterize quantum LEPs of quantum non-Hermitian systems. We conducted experiments on an IBM quantum processor to implement a prototype model with one-, two-, and three qubits simulating the decay of a single qubit through competing channels, resulting in LEPs but not HEPs. Subsequently, we performed tomographic reconstruction of the corresponding experimental Liouvillian and its LEPs using both single- and two-qubit operations. This example underscores the efficacy of process tomography in tuning and observing LEPs even in the absence of HEPs.
We study the applicability of the Liouvillian exceptional points (LEPs) approach to nanoscale open quantum systems. A generic model of the driven two-level system in a thermal environment is analyzed within the nonequilibrium Green's function (NEGF) and Bloch quantum master equation formulations. We derive the latter starting from the exact NEGF Dyson equations and highlight the qualitative limitations of the LEP treatment by examining the approximations employed in its derivation. We find that the non-Markov character of evolution in open quantum systems does not allow for the introduction of the concept of exceptional points for a description of their dynamics. Theoretical analysis is illustrated with numerical simulations.
Usually, when investigating exceptional points (EPs) of an open Markovian bosonic system, one deals with spectral degeneracies of a non-Hermitian Hamiltonian (NHH), which can correctly describe the system dynamics only in the semiclassical regime. A recently proposed quantum Liouvillian framework [Minganti et al., Phys. Rev. A 100, 062131 (2019)] enables the complete determination of the dynamical properties of such systems and their EPs (referred to as Liouvillian EPs, or LEPs) in the quantum regime by taking into account the effects of quantum jumps, which are ignored in the NHH formalism. Moreover, the symmetry and eigenfrequency spectrum of the NHH become a part of much larger Liouvillian eigenspace. As such, the EPs of an NHH form a subspace of the LEPs. Here we show that once an NHH of a dissipative linear bosonic system exhibits an EP of a certain finite order nnn, it immediately implies that the corresponding LEP can become of any higher order $m\ensuremath{\ge}n$ defined in the infinite Hilbert space. These higher-order LEPs can be identified by the coherence and spectral functions at the steady state. The coherence functions can offer a convenient tool to probe extreme system sensitivity to external perturbations in the vicinity of higher-order LEPs. As an example, we study a linear bosonic system of a bimodal cavity with incoherent mode coupling to reveal its higher-order LEPs; particularly, of second and third order via first- and second-order coherence functions, respectively. Accordingly, these LEPs can be additionally revealed by squared and cubic Lorentzian spectral lineshapes in the power and intensity-fluctuation spectra. Moreover, we demonstrate that these EPs can also be associated with spontaneous parity-time (PT\mathcal{PT}PT) and anti-PT\mathcal{PT}PT-symmetry breaking in the system studied. These symmetries can be switched in the output fields (the so-called supermodes) of an additional linear coupler with a properly chosen coupling strength. Thus, we show that the initial loss-loss dynamics for the supermodes can be equivalent to the balanced gain-loss evolution.