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arXiv:2312.13325 · Laser & Photonics Review

Tailoring Sub‐Doppler Spectra of Thermal Atoms with a Dielectric Optical Metasurface Chip

Dengke Zhang, Chen Qing

Published Mar 7, 2024• 3 citations
arXivHTMLPDF

Abstract

Abstract Compact and robust structures to precisely control and acquire atomic spectra are increasingly important for the pursuit of widespread applications. Sub‐Doppler responses of thermal atoms are critical in constructing high‐precision devices and systems. In this study, a nanograting metasurface specifically is designed for atomic rubidium vapor and integrated it into a miniature vapor cell. Using the metasurface with built‐in multifunctional controls for light, pump‐probe atomic spectroscopy is established and sub‐Doppler responses are experimentally observed at low incident power. Moreover, the sub‐Doppler lineshape can be tailored by varying the incident polarization state. The spectrum transformation from absorption to transparency is observed. Using one of the sharp responses, laser stabilization with a stability of at 2 s can be achieved. This work reveals the effective control of atomic spectra with optical metasurface chips, which may have great potential for future developments in fundamental optics and novel optical applications.

DOI
10.1002/lpor.202301276

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Atomic spectroscopy serves as the basis for quantum precision measurements, where frequency-stabilized lasers are crucial for obtaining accurate atomic spectra.This work introduces a compact laser frequency stabilization system that employs a multifunctional metasurface to adjust the polarization, amplitude, and propagation direction of incident light.By combining with a Rb atomic vapor cell, the system achieves a tunable sub-Doppler spectrum for laser frequency stabilization.The experimental result demonstrates that a laser frequency stability of 3 × 10 -11 is attained from 1 to 200 s at 780 nm with the input power at 20 μW.The devices hold significant potential for compactness, integration, and mass production, making them highly suitable for quantum measurement applications.
We demonstrate chip-scale sub-Doppler spectroscopy in an integrated and fiber-coupled photonic-metasurface device. The device is a stack of three planar components: a photonic mode expanding grating emitter circuit with a monolithically integrated tilt-compensating dielectric metasurface, a microfabricated atomic vapor cell, and a mirror. The metasurface photonic circuit efficiently emits a 130 μm wide (1/e2 diameter) collimated surface-normal beam with only −6.3 dB loss and couples the reflected beam back into the waveguide and connecting fiber, requiring no alignment between the stacked components. We develop a simple model based on light propagation through the photonic device to interpret the atomic spectroscopy signals and explain spectral features covering the full Rb hyperfine state manifold. The demonstration of waveguide-to-waveguide coupling through the vapor cell paves the way for atomic ensembles to be used as components in complex photonic integrated circuits, allowing the unique properties of atomic systems to be available for future highly miniaturized optical devices and systems.
We report on the atomic spectroscopy and laser frequency stabilization using a new type of a miniaturized glass vapor cell with a scalable thickness varying from 500 nm up to 8 μm. The cell is fabricated by lithography and etching techniques in a Pyrex glass substrate, followed by anodic bonding. It is filled with rubidium vapor using a distillation procedure. This simple and cost-effective fabrication method provides an attractive and compact solution for atomic cells, with applications in quantum metrology, sensing, communication, and light-vapor manipulations at the subwavelength scale. Using the fabricated cell, we have performed fluorescence and transmission spectroscopy of the Rubidium D2 line and observed sub-Doppler broadened lines. As an example, for a potential application, we have used the fabricated cell to demonstrate the stabilization of a 780 nm diode laser to the level about 10−10 in fractional frequency.
The integration of nanophotonic optical phased arrays (OPA) with alkali vapor cells has the potential to enhance the performance of chip-scale atomic systems by enabling novel methods for beam shaping and active alignment in atomic spectroscopy. In this work, we present the first demonstration of an OPA used for precision saturated absorption spectroscopy with a rubidium vapor cell integrated directly on the chip. The OPA, consisting of 64 emitters, expands a sub-micron waveguide mode into a >100 µm diameter free-space beam, optimized for the D2 absorption line of rubidium. We resolved the sub-Doppler hyperfine splittings in both 85Rb and 87Rb isotopes, achieving Lorentzian linewidths ranging from 25 to 40 MHz suitable for stabilizing the cooling lasers in rubidium cold atom systems.
Abstract Emerging miniaturized atomic sensors such as optically pumped magnetometers (OPMs) have attracted widespread interest due to their application in high‐spatial‐resolution biomagnetism imaging. While optical probing systems in conventional OPMs require bulk optical devices including linear polarizers and lenses for polarization conversion and wavefront shaping, which are challenging for chip‐scale integration. In this study, an integrated optical probing scheme based on localized‐interference metasurface for chip‐scale OPM is developed. Our monolithic metasurface allows tailorable linear polarization conversion and wavefront manipulation. Two silicon‐based metasurfaces namely meta‐polarizer and meta‐polarizer‐lens are fabricated and characterized, with maximum transmission efficiency and extinction ratio (ER) of 86.29 % and 14.2 dB for the meta‐polarizer as well as focusing efficiency and ER of 72.79 % and 6.4 dB for the meta‐polarizer‐lens, respectively. A miniaturized vapor cell with 4 × 4 × 4 mm 3 dimension containing 87 Rb and N 2 is combined with the meta‐polarizer to construct a compact zero‐field resonance OPM for proof of concept. The sensitivity of this sensor reaches approximately 9 fT/Hz 1/2 with a dynamic range near zero magnetic field of about ±2.3 nT. This study provides a promising solution for chip‐scale optical probing, which holds potential for the development of chip‐integrated OPMs as well as other advanced atomic devices where the integration of optical probing system is expected.
Abstract Programmability and precise control of laser frequency are essential for quantum experiments and applications such as atomic clocks, quantum computers, and cold-atom sensors. Current systems use bulky, power-hungry modulators and frequency shifters which are difficult to integrate and limit portability and scalability. We report an electrically controllable, agile optical frequency source based on a semiconductor laser stabilized to a photonic integrated resonator cavity with a lead zirconate titanate (PZT) actuator. We demonstrate this approach with precision programmable frequency control of a 780-nm laser that can periodically reference to rubidium-87 ( 87 Rb) spectroscopy followed by fast, programmable, arbitrary frequency tuning sequences for quantum control. We use this approach to demonstrate sub-Doppler cooling of 87 Rb without any external modulators, achieving atom-cloud temperatures as low as 16 μ K. The device achieves a tuning strength up to 1 GHz/V with 11 MHz modulation bandwidth while consuming only 10 nW of electrical power. This work establishes a route toward compact, low-power, and chip-scale laser systems for next-generation quantum and atomic sensing technologies.