Paul Dyke, S. Musolino, Hadrien Kurkjian, D. J. M. Ahmed-Braun, A. Pennings, I. Herrera, Sascha Hoinka, S. J. J. M. F. Kokkelmans, V. E. Colussi, Chris J. Vale
Symmetry-breaking phase transitions are central to our understanding of states of matter. When a continuous symmetry is spontaneously broken, new excitations appear that are tied to fluctuations of the order parameter. In superconductors and fermionic superfluids, the phase and amplitude can fluctuate independently, giving rise to two distinct collective branches. However, amplitude fluctuations are difficult to both generate and measure, as they do not couple directly to the density of fermions and have only been observed indirectly to date. Here, we excite amplitude oscillations in an atomic Fermi gas with resonant interactions by an interaction quench. Exploiting the sensitivity of Bragg spectroscopy to the amplitude of the order parameter, we measure the time-resolved response of the atom cloud, directly revealing amplitude oscillations at twice the frequency of the gap. The magnitude of the oscillatory response shows a strong temperature dependence, and the oscillations appear to decay faster than predicted by time-dependent Bardeen-Cooper-Schrieffer theory applied to our experimental setup.
Symmetry-breaking phase transitions are central to our understanding of states of matter. When a continuous symmetry is spontaneously broken, new excitations appear that are tied to fluctuations of the order parameter. In superconductors and fermionic superfluids, the phase and amplitude can fluctuate independently, giving rise to two distinct collective branches. However, amplitude fluctuations are difficult to both generate and measure, as they do not couple directly to the density of fermions and have only been observed indirectly to date. Here, we excite amplitude oscillations in an atomic Fermi gas with resonant interactions by an interaction quench. Exploiting the sensitivity of Bragg spectroscopy to the amplitude of the order parameter, we measure the time-resolved response of the atom cloud, directly revealing amplitude oscillations at twice the frequency of the gap. The magnitude of the oscillatory response shows a strong temperature dependence, and the oscillations appear to decay faster than predicted by time-dependent Bardeen-Cooper-Schrieffer theory applied to our experimental setup.
Bragg spectroscopy shows the evolution of gapless Goldstone modes and single-particle-like excitations in an atomic Fermi superfluid as it crosses from a Bardeen–Cooper–Schrieffer superfluid to the Bose–Einstein condensate regime. Spontaneous symmetry breaking is a central paradigm of elementary particle physics1, magnetism2, superfluidity3 and superconductivity4. According to Goldstone’s theorem, phase transitions that break continuous symmetries lead to the existence of gapless excitations in the long-wavelength limit5. These Goldstone modes can become the dominant low-energy excitation, showing that symmetry breaking has a profound impact on the physical properties of matter. Here, we present a comprehensive study of the elementary excitations in a homogeneous strongly interacting Fermi gas through the crossover from a Bardeen–Cooper–Schrieffer (BCS) superfluid to a Bose–Einstein condensate (BEC) of molecules using two-photon Bragg spectroscopy. The spectra exhibit a discrete Goldstone mode, associated with the broken-symmetry superfluid phase, as well as pair-breaking single-particle excitations. Our techniques yield a direct determination of the superfluid pairing gap and speed of sound in close agreement with strong-coupling theories.
In quantum many-body systems with spontaneous breaking of continuous symmetries, Higgs modes emerge as collective amplitude oscillations of order parameters. Recently, Higgs mode has been observed in the ultracold Fermi gas. In the present paper, we use the time-dependent Bogoliubov-de Gennes equations to investigate Higgs amplitude oscillations of the superfluid order parameter in a Fermi gas induced by a rapid change of the s-wave scattering length. In particular, we investigate the Higgs mode with different values of the initial scattering length. We find that the energy of the Higgs mode coincides with the threshold energy of the pair-breaking excitation, and exponent of the power-low decay of the Higgs mode γ continuously changes between γ=−1/2 and γ=−3/2 through the Bardeen-Cooper-Schrieffer-Bose-Einstein condensation (BCS-BEC) crossover. Moreover, we propose the optimal ramp speed of the scattering length for observing the clearest Higgs oscillations.
In phase transitions, spontaneous symmetry breaking results in a nonzero order parameter and two collective excitations: the Goldstone and the amplitude mode. These modes, which define key properties of superconductors and fermionic superfluids, are well understood in homogeneous systems. However, their behavior under strong confinement remains largely unexplored, particularly when their excitation energy becomes comparable to the imposed discrete level spacing. In this scenario, hybridization between different collective modes is expected to take place. Here, we show how the amplitude mode hybridizes with a spatial mode in a confined fermionic superfluid. Using lattice modulation spectroscopy, we observe the evolution of the mode throughout the entire crossover from the Bardeen-Cooper-Schrieffer (BCS) state to Bose-Einstein condensation (BEC) of molecules. In the BCS regime, the excitation energy is located at twice the pairing gap, then gradually becomes an in-gap excitation in the strongly correlated regime. Further to the BEC limit, the excitation energy approaches twice the level spacing. The spectral weight of this mode vanishes when approaching the superfluid critical temperature. Our experimental results are in excellent agreement with an effective field theory, providing strong evidence that amplitude oscillations hybridize with and eventually transform into breathing oscillations of the order parameter. The strong modification of the excitation spectrum reveals how confinement and finite-size effects impact fundamental modes of symmetry-broken states.
Understanding how pairing correlations in superconductors evolve out of equilibrium is a central challenge in quantum many-body physics. In systems with s-wave pairing, the character of Cooper pairing evolves continuously from a BCS regime of weakly bound, overlapping pairs to a BEC regime of tightly bound molecules, each with distinct excitation spectra. Here we realize and probe pairing dynamics across these regimes using cold, non-degenerate 87Rb atoms coupled to an optical cavity with Floquet dressing. Our cavity-QED platform emulates fermionic superfluids through a mapping onto Anderson pseudospins, while optical and microwave control tunes the ratio of interactions to single-particle energies, providing a flexible approach complementary to ultracold Feshbach and ultrafast solid-state platforms. Following a quench, we observe persistent pairing and transient oscillations of the order parameter associated with a collective amplitude (Higgs) mode. We find that the decay of these oscillations sharply distinguishes weak- and strong-pairing regimes: in the weak-pairing regime, oscillations decay with a power-law exponent ∣α∣=0.65(8), whereas in the strong-pairing regime the decay is substantially faster, with ∣α∣>1. The oscillation frequency is set by the minimum quasiparticle excitation energy, directly linking nonequilibrium dynamics to the underlying excitation spectrum. Our results establish nonequilibrium dynamics as a direct probe of pairing character and collective excitations in interacting quantum systems.
A new field of research, which gained interest in the past years, is the field of non- equilibrium physics of strongly interacting fermionic systems. In this thesis we present a novel apparatus to study an ultracold strongly interacting superfluid Fermi gas driven out of equilibrium. In more detail, we study the excitation of a collective mode, the Higgs mode, and the dynamics occurring after a rapid quench of the interaction strength. Ultracold gases are ideal candidates to explore the physics of strongly interacting Fermi gases due to their purity and the possibility to continuously change many different system parameters, such as the interaction strength. The novel apparatus enabling the experiments outlined below is built from scratch. The setup is described and characterized in detail. We produce a fermionic superfluid of 4 × 10^6 6Li atoms at a temperature of T/T_F = 0.07 ± 0.02, where T_F is the Fermi temperature. This is achieved within 23 s by a combination of laser cooling, radio frequency evaporation of 23Na and simultaneous sympathetic cooling of 6Li in an optical plugged magnetic trap and subsequent evaporative cooling of 6Li in a dipole trap. In this thesis we provide the first experimental evidence of the Higgs mode in a strongly interacting Fermi gas in the crossover from a BCS superfluid to a molecular Bose-Einstein condensate. We develop a novel excitation method, which directly couples to the amplitude of the order parameter. This is achieved by continuously changing the population of one spin component by driving a radio frequency transition to a previously unoccupied third hyperfine state. This effectively modulates the interaction strength and the amplitude of the order parameter. We spectroscopically observe a resonance behavior at twice the gap frequency. For strong coupling, the peak width broadens and eventually the Higgs mode disappears when the Cooper pairs turn into tightly bound dimers signaling the instability of the Higgs mode. It has been suggested that the Higgs mode frequency is a precise measure of the superconducting gap in the BEC-BCS crossover, where the exact value of the gap is yet unknown and numerical calculations are challenging. Hence, our novel method provides a unique technique to determine the superconducting gap. Moreover, we perform rapid variations of the interaction parameter and vary both the initial interaction strength and the amplitude of the quench. The rapid quenches are performed by rapidly transferring one spin component of a two-component spin mixture into a third state with a different interaction strength by using a radio frequency transition. Using this novel method, we can perform the quenches in half the Fermi time, which is experimentally very close to a sudden change and to date faster than any other research group performing interaction quenches with ultra cold gases. In the experiment, we observe a fast relaxation to a zero order parameter for large quenches, whereas for small quenches we observe, after a sudden drop, a revival of the order parameter and equilibration to a long-term superfluid steady state. Our measurement provides the first evidence of the collapse and subsequent revival of order in a strongly interacting fermionic system.
Experimental evidence of the Higgs mode in strongly interacting superfluid Fermi gases had not been observed until recently [Behrle et al., Nat. Phys. 14, 781 (2018).]. Due to the coupling with other collective modes and quasiparticle excitations, generating stable Higgs-mode oscillations is challenging. We study how to excite long-lived Higgs-mode oscillations in a homogeneous superfluid Fermi gas in the BCS-BEC crossover. We find that the Higgs mode can be excited by time-periodically modulating the scattering length at an appropriate amplitude and frequency. However, even for a modulation frequency below twice the pairing-gap energy, quasiparticles are still excited through the generation of higher harmonics due to nonlinearity in the superfluid. More importantly, we find that persistent Higgs-mode oscillations with almost constant amplitude can be produced by removing particles at an appropriate momentum, and the oscillation amplitude can be controlled by the number of removed particles. Finally, we propose two ways to experimentally realize particle removal.