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arXiv:2308.13200 · Physical Review A

Parameter-space investigation for spin-dependent electron diffraction in the Kapitza-Dirac effect

Yang Wang, Sven Ahrens

Published Jan 16, 2024• 2 citations
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Abstract

We demonstrate that spin-dependent electron diffraction is possible for a smooth range of transverse electron momenta in a two-photon Bragg scattering scenario of the Kapitza-Dirac effect. Our analysis is rendered possible by introducing a generalized specification for quantifying spin-dependent diffraction, yielding an optimization problem which is solved by making use of a Newton gradient iteration scheme. With this procedure, we investigate the spin-dependent effect for different transverse electron momenta and different laser polarizations of the standing-light-wave Kapitza-Dirac scattering. The possibility of using arbitrarily low transverse electron momenta when setting up a spin-dependent Kapitza-Dirac experiment allows longer interaction times of the electron with the laser and therefore enables less constraining parameters for an implementation of the effect.

DOI
10.1103/physreva.109.012212

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We demonstrate that spin-dependent electron diffraction is possible for a smooth range of transverse electron momenta in a two-photon Bragg scattering scenario of the Kapitza-Dirac effect. Our analysis is rendered possible by introducing a generalized specification for quantifying spin-dependent diffraction, yielding an optimization problem which is solved by making use of a Newton gradient iteration scheme. With this procedure, we investigate the spin-dependent effect for different transverse electron momenta and different laser polarizations of the standing-light-wave Kapitza-Dirac scattering. The possibility of using arbitrarily low transverse electron momenta when setting up a spin-dependent Kapitza-Dirac experiment allows longer interaction times of the electron with the laser and therefore enables less constraining parameters for an implementation of the effect.
We present the possibility of spin-dependent Kapitza-Dirac scattering based on a two-photon interaction only. The interaction scheme is inspired from a Compton scattering process, for which we explicitly show the mathematical correspondence to the spin dynamics of an electron diffraction process in a standing light wave. The spin effect has the advantage that it already appears in a Bragg scattering setup with arbitrary low field amplitudes, for which we have estimated the diffraction count rate in a realistic experimental setup at available x-ray free-electron laser facilities.
Quantum mechanical diffraction is of particular interest, because it contradicts our everyday life experience. \nThis theoretical work considers the diffraction of electrons at standing waves of light, referred \nto as the Kapitza-Dirac effect. The work focuses on a special version of a Kapitza-Dirac effect in which \nthe electron interacts with three photons. The particular property of this 3-photon Kapitza-Dirac effect \nis, that the electron spin is rotated. \nThis work considers different relativistic and non-relativistic quantum mechanical wave equations \nwhich are described in momentum space. On one hand, the quantum dynamics of the diffracted electrons \nis solved numerically in momentum space and the properties of the 3-photon Kapitza-Dirac effect \nare investigated in detail. On the other hand, the quantum dynamics is solved via time-dependent \nperturbation theory and is compared with the numerical results. \nIn contrast to the originally proposed Kapitza-Dirac effect with two interacting photons, the number \nof absorbed and emitted photons by the electron is not equal for the 3-photon Kapitza-Dirac effect. \nTherefore, the diffraction process only appears for relativistic electron momenta in laser propagation \ndirection. Furthermore, a very high field strength of the laser beam is required for driving the Kapitza- \nDirac effect with a measurable diffraction probability. The electron spin is rotated along the axis of the \nmagnetic field of the laser beam, when it undergoes the diffraction process. The rotation angle of the \nspin rotation depends on the electron momentum component in laser polarization direction. Therefore, \nthe probability for flipping the electron spin can be tuned by choosing the electron momentum in \nthe direction of the laser polarization. An experimental investigation may by established by utilizing \nfuture X-ray laser facilities.
We demonstrate the theoretical feasibility of spin-dependent diffraction and spin polarization of an electron in two counterpropagating, circularly polarized laser beams. The spin dynamics appears in a two-photon process of the Kapitza-Dirac effect in the Bragg regime. We show the spin dependence of the diffraction process by comparison of the time evolution of spin-up and spin-down electrons in a relativistic quantum simulation. We further discuss the spin properties of the scattering by studying an analytically approximated solution of the time-evolution matrix. A classification scheme in terms of unitary or nonunitary propagation matrices is used for establishing a generalized and spin-independent description of the spin properties in the diffraction process.
Theoretical spin properties of the Kapitza-Dirac effect beyond the plane-wave description are not known in detail. We develop a method for computing electron diffraction of the two-photon Kapitza-Dirac effect in a two-dimensional Gaussian beam standing light wave within a relativistic formulation. The solutions are computed on the basis of time-dependent perturbation theory, where a momentum space formulation with the use of a Fourier transformation of the external potential allows for the solving the perturbative time-integrals. An iteration over each possible quantum state combination leads to a quadratic scaling of our method with respect to spacial grid resolution, where time-stepping does not occur in the numeric implementation. The position- and momentum space grids are adapted to the two-photon interaction geometry at low resolution, for which our study only finds partial convergence of the simulated diffraction pattern. Further, the method has the advantage of having an easy implementable parallelization layout.
Kapitza-Dirac scattering of nonrelativistic electrons from counterpropagating bichromatic laser waves of linear polarization is studied. The focus lies on the electronic spin dynamics in the Bragg regime when the laser fields possess a frequency ratio of 2. To this end, the time-dependent Pauli equation is solved numerically, both in coordinate space and momentum space. Our numerical results are corroborated by analytical derivations. We demonstrate that, for certain incident electron momenta, the scattering crucially relies on the electron spin which undergoes characteristic Rabi-like oscillations. A parameter regime is identified where the Rabi oscillations reach maximum amplitude. We also briefly discuss spin-dependent Kapitza-Dirac scattering of protons.
Electron spin dynamics in Kapitza-Dirac scattering from a standing laser wave of high frequency and high intensity is studied. We develop a fully relativistic quantum theory of the electron motion based on the time-dependent Dirac equation. Distinct spin dynamics, with Rabi oscillations and complete spin-flip transitions, is demonstrated for Kapitza-Dirac scattering involving three photons in a parameter regime accessible to future high-power x-ray laser sources. The Rabi frequency and, thus, the diffraction pattern is shown to depend crucially on the spin degree of freedom.