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arXiv:1204.0239 · Physical Review Letters

Spin Dynamics in the Kapitza-Dirac Effect

Sven Ahrens, Heiko Bauke, Christoph H. Keitel, Carsten Müller

Published Jul 23, 2012• 68 citations
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Abstract

Electron spin dynamics in Kapitza-Dirac scattering from a standing laser wave of high frequency and high intensity is studied. We develop a fully relativistic quantum theory of the electron motion based on the time-dependent Dirac equation. Distinct spin dynamics, with Rabi oscillations and complete spin-flip transitions, is demonstrated for Kapitza-Dirac scattering involving three photons in a parameter regime accessible to future high-power x-ray laser sources. The Rabi frequency and, thus, the diffraction pattern is shown to depend crucially on the spin degree of freedom.

DOI
10.1103/physrevlett.109.043601

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Electron spin dynamics in Kapitza-Dirac scattering from a standing laser wave of high frequency and high intensity is studied. We develop a fully relativistic quantum theory of the electron motion based on the time-dependent Dirac equation. Distinct spin dynamics, with Rabi oscillations and complete spin-flip transitions, is demonstrated for Kapitza-Dirac scattering involving three photons in a parameter regime accessible to future high-power x-ray laser sources. The Rabi frequency and, thus, the diffraction pattern is shown to depend crucially on the spin degree of freedom.
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Kapitza-Dirac scattering of nonrelativistic electrons from counterpropagating bichromatic laser waves of linear polarization is studied. The focus lies on the electronic spin dynamics in the Bragg regime when the laser fields possess a frequency ratio of 2. To this end, the time-dependent Pauli equation is solved numerically, both in coordinate space and momentum space. Our numerical results are corroborated by analytical derivations. We demonstrate that, for certain incident electron momenta, the scattering crucially relies on the electron spin which undergoes characteristic Rabi-like oscillations. A parameter regime is identified where the Rabi oscillations reach maximum amplitude. We also briefly discuss spin-dependent Kapitza-Dirac scattering of protons.
We discuss electron diffraction from two standing waves with two different frequencies. The effects of increasing the frequency of the second laser beam and changing the laser amplitudes on the form and period of the Rabi oscillation are studied theoretically. The corresponding scattering probabilities for certain incident electron momenta are obtained by an analytical Rabi matrix and numerical solution of the Dirac equation. We show that at high intensities, $\ensuremath{\ge}{10}^{20}$ W ${\mathrm{cm}}^{\ensuremath{-}2}$, the process with an even number of photons involved in the Kapitza-Dirac effect can be used as a spin filter for free electrons. On the other hand, the process with an odd number photons and an electron with momentum along the laser polarization preserves the initial spin of the electron.
A relativistic description of the Kapitza-Dirac effect in the so-called Bragg regime with two and three interacting photons is presented by investigating both numerical and perturbative solutions of the Dirac equation in momentum space. We demonstrate that spin flips can be observed in the two-photon and the three-photon Kapitza-Dirac effects for certain parameters. During the interaction with the laser field the electron's spin is rotated, and we give explicit expressions for the rotation axis and the rotation angle. The off-resonant Kapitza-Dirac effect, that is, when the Bragg condition is not exactly fulfilled, is described by a generalized Rabi theory. We also analyze the in-field quantum dynamics as obtained from the numerical solution of the Dirac equation.
The Kapitza-Dirac effect, which refers to electron scattering at standing light waves, is studied in the Bragg regime with counterpropagating elliptically polarized electromagnetic waves with the same intensity, wavelength, and degree of polarization for two different setups. In the first setup, where the electric-field components of the counterpropagating waves have the same sense of rotation, we find distinct spin effects. The spins of the scattered electrons and of the nonscattered electrons, respectively, precess with a frequency that is of the order of the Bragg-reflection Rabi frequency. When the electric-field components of the counterpropagating waves have an opposite sense of rotation, which is the second considered setup, the standing wave has linear polarization, and no spin effects can be observed. Our results are based on numerical solutions of the time-dependent Dirac equation and the analytical solution of a relativistic Pauli equation, which accounts for the leading relativistic effects.
We theoretically demonstrate the feasibility of producing an electron spin beam splitter using Kapitza-Dirac diffraction on bichromatic standing waves which are created by the fundamental frequency and its third harmonic. The relativistic electron in the Bragg regime absorbs three photons with a frequency of $\ensuremath{\omega}$ and emits a photon with a frequency of $3\ensuremath{\omega}$; we introduce this as the four-photon Kapitza-Dirac effect. In this four-photon Kapitza-Dirac effect distinct spin effects arise in different polarizations of the third harmonic laser beam. It is shown that the shape of the Rabi oscillation between the initial and scattered states is changed and finds two unequal peaks for all polarizations of laser beams. For the case of circular polarization of the fundamental and third harmonic, despite Rabi oscillation, the spin down electron beam in 0.23 fs intervals maintains its momentum and spin. Also we find that if a suitable combination of a linearly polarized fundamental laser beam and a third harmonic with circular polarization in the condition $\stackrel{P\vec}{p}\ifmmode\cdot\else\textperiodcentered\fi{}\stackrel{P\vec}{A}$ term is involved, it results in a spin-dependent oscillation that preserves the spin state of the initial electron.