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arXiv:1606.04813 · Physical Review A

Spin dynamics in Kapitza-Dirac scattering of electrons from bichromatic laser fields

Matthias M. Dellweg, Hani M. Awwad, Carsten Müller

Published Aug 31, 2016• 14 citations
arXivHTMLPDF

Abstract

Kapitza-Dirac scattering of nonrelativistic electrons from counterpropagating bichromatic laser waves of linear polarization is studied. The focus lies on the electronic spin dynamics in the Bragg regime when the laser fields possess a frequency ratio of 2. To this end, the time-dependent Pauli equation is solved numerically, both in coordinate space and momentum space. Our numerical results are corroborated by analytical derivations. We demonstrate that, for certain incident electron momenta, the scattering crucially relies on the electron spin which undergoes characteristic Rabi-like oscillations. A parameter regime is identified where the Rabi oscillations reach maximum amplitude. We also briefly discuss spin-dependent Kapitza-Dirac scattering of protons.

DOI
10.1103/physreva.94.022122

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Nonrelativistic Kapitza-Dirac scattering of electrons from counterpropagating bichromatic laser waves is studied in the resonant Bragg regime, taking the electron spin into account. We show that the intrinsic field-induced detuning, which arises in the Rabi oscillation dynamics between initial and scattering state of the electron, can be compensated by a suitable adjustment of its incident momentum. Analytical formulas of the optimized electron momentum for spin-dependent three-photon and spin-independent four-photon Kapitza-Dirac scattering are obtained from simplified model systems in reduced dimensionality, which preserve the characteristic properties of the process.
The Kapitza-Dirac effect, which refers to electron scattering at standing light waves, is studied in the Bragg regime with counterpropagating elliptically polarized electromagnetic waves with the same intensity, wavelength, and degree of polarization for two different setups. In the first setup, where the electric-field components of the counterpropagating waves have the same sense of rotation, we find distinct spin effects. The spins of the scattered electrons and of the nonscattered electrons, respectively, precess with a frequency that is of the order of the Bragg-reflection Rabi frequency. When the electric-field components of the counterpropagating waves have an opposite sense of rotation, which is the second considered setup, the standing wave has linear polarization, and no spin effects can be observed. Our results are based on numerical solutions of the time-dependent Dirac equation and the analytical solution of a relativistic Pauli equation, which accounts for the leading relativistic effects.
Coherent scattering of an electron beam by the Kapitza-Dirac effect from a standing laser wave which comprises two frequency components is studied. To this end, the Schr\"odinger equation is solved numerically with a suitable ponderomotive potential. Besides, an analytical solution for electron diffraction in the asymptotic domain of large field amplitudes is obtained and a mathematical model in reduced dimensionality for the scattering amplitude in the Bragg regime is presented. We demonstrate distinct interference signatures and relative phase effects when the standing wave contains a fundamental frequency and its second harmonic. The influence of the relative field intensities on the Rabi oscillation dynamics is also discussed.
Electron spin dynamics in Kapitza-Dirac scattering from a standing laser wave of high frequency and high intensity is studied. We develop a fully relativistic quantum theory of the electron motion based on the time-dependent Dirac equation. Distinct spin dynamics, with Rabi oscillations and complete spin-flip transitions, is demonstrated for Kapitza-Dirac scattering involving three photons in a parameter regime accessible to future high-power x-ray laser sources. The Rabi frequency and, thus, the diffraction pattern is shown to depend crucially on the spin degree of freedom.
We discuss electron diffraction from two standing waves with two different frequencies. The effects of increasing the frequency of the second laser beam and changing the laser amplitudes on the form and period of the Rabi oscillation are studied theoretically. The corresponding scattering probabilities for certain incident electron momenta are obtained by an analytical Rabi matrix and numerical solution of the Dirac equation. We show that at high intensities, $\ensuremath{\ge}{10}^{20}$ W ${\mathrm{cm}}^{\ensuremath{-}2}$, the process with an even number of photons involved in the Kapitza-Dirac effect can be used as a spin filter for free electrons. On the other hand, the process with an odd number photons and an electron with momentum along the laser polarization preserves the initial spin of the electron.