The novel quantum effects induced by the free-electron-photons interaction have attracted increasing interest due to their potential applications in ultrafast quantum information processing. Here, we propose a scheme to generate optical cat states based on the quantum interference of multi-path free-electron-photons interactions that take place simultaneously with strong coupling strength. By performing a projection measurement on the electron, the state of light changes significantly from a coherent state into a non-Gaussian state with either Wigner negativity or squeezing property, both possess metrological power to achieve quantum advantage. More importantly, we show that the Wigner negativity oscillates with the coupling strength, and the optical cat states are successfully generated with high fidelity at all the oscillation peaks. This oscillation reveals the quantum interference effect of the multiple quantum pathways in the interaction of the electron with photons, by that various nonclassical states of light are promising to be fast prepared and manipulated. These findings inspire further exploration of emergent quantum phenomena and advanced quantum technologies with free electrons.
The novel quantum effects induced by the free-electron-photons interaction have attracted increasing interest due to their potential applications in ultrafast quantum information processing. Here, we propose a scheme to generate optical cat states based on the quantum interference of multi-path free-electron-photons interactions that take place simultaneously with strong coupling strength. By performing a projection measurement on the electron, the state of light changes significantly from a coherent state into a non-Gaussian state with either Wigner negativity or squeezing property, both possess metrological power to achieve quantum advantage. More importantly, we show that the Wigner negativity oscillates with the coupling strength, and the optical cat states are successfully generated with high fidelity at all the oscillation peaks. This oscillation reveals the quantum interference effect of the multiple quantum pathways in the interaction of the electron with photons, by that various nonclassical states of light are promising to be fast prepared and manipulated. These findings inspire further exploration of emergent quantum phenomena and advanced quantum technologies with free electrons.
Optical cat states, the nonclassical superposition of two quasi-classical coherent states, serve as a basis for gedankenexperiments testing quantum physics on mesoscopic scales and are increasingly recognized as a resource for quantum information processing. Here, we report the first experimental realization of optical cat states by adding a photon to a squeezed vacuum state; so far only photon-subtraction protocols have been realized. Photon addition gives us the advantage of using heralded signal photons as experimental triggers, and we can generate cat states at rates exceeding $2.3\ifmmode\times\else\texttimes\fi{}{10}^{5}$ counts per second. Our most highly squeezed vacuum input state shows \ensuremath{-}8.9 dB squeezing, but such squeezing entails some degradation---in this case, 15.1 dB antisqueezing. Even so, our approach enables us to synthesize a state with a maximum cat amplitude of $|\ensuremath{\alpha}|\ensuremath{\approx}1.77$ whose Wigner distribution still shows pronounced negative parts. Our experimental implementation with controlled photon addition demonstrates a powerful and robust building block for advanced quantum state engineering and shows that heralded photon addition can be controlled well and performed at high rates.
Schrödinger cat states, representing coherent superpositions of macroscopically distinguishable states, are indispensable nonclassical resources for continuous-variable quantum information processing. Existing generation protocols typically rely on strong nonlinear interactions, complicated control techniques, or engineered dissipation, posing challenges for experimental implementation. Here, we propose a simple measurement-based protocol for generating Schrödinger cat states in a cavity-QED system by combining coherent driving, dispersive atom--cavity interactions, and atomic postselection. The atom--cavity interaction establishes coherent correlations between the atomic and photonic degrees of freedom, while the subsequent atomic postselection projects the cavity field onto a non-Gaussian superposition state with pronounced Wigner negativity. Numerical simulations based on the Lindblad master equation show that the generated Schrödinger cat states remain robust against moderate cavity dissipation. Our results demonstrate that conditional atomic measurements provide an effective and experimentally accessible approach for preparing nonclassical cavity states without relying on strong optical nonlinearities or engineered dissipation.
Optical parametric processes underpin quantum photonics, while free-electron--photon interactions offer agile pathways to generate nontrivial quantum photonic states. These threads have so far largely progressed independently, whereas placing free electrons in a driven nonlinear system can potentially activate coherent parametric interaction channels for joint state engineering of both types of particles. Here we unify these paradigms by developing a general theoretical framework for parametric free-electron--photon interactions in a nonlinear optical system driven by degenerate parametric down-conversion. Unlike free electrons in a linear bath, here they can couple to Bogoliubov quasiparticles through two detuned phase-matching channels, where the parametric process and free-electron interactions can quantum amplify each other. Seeding the interaction with squeezed vacuum yields gain-only or loss-only electron energy spectra, and enables electron-heralded squeezed Fock states; with bare vacuum, postselecting electron energy sidebands generates high-fidelity Schrödinger cat states. Our results show how optical parametric interactions can quantum shape free electrons and photons, potentially enabling a quantum parametric dielectric laser accelerator that mitigates the need for temporal phase synchronization, thereby allowing acceleration probabilities to approach unity even for phase-random electrons.
Nonclassical states of light are fundamental in various applications, spanning quantum computation to enhanced sensing. Fast free electrons, which emit light into photonic structures through the mechanism of spontaneous emission, represent a promising platform for generating diverse types of states. Indeed, the intrinsic connection between the input electron wave function and the output light field suggests that electron-shaping schemes, based on light-induced scattering, facilitates their synthesis. In this article, we present a theoretical framework capable of predicting the final optical density matrix of a generic N-electron state that can also account for post-sample energy filtering. By using such framework, we study the modulation-dependent fluctuations of the N-electron emission and identify regions of Poissonian and super-Poissonian statistics. In the single-electron case, we show how coherent states with nearly 90% purity can be formed by pre-filtering a portion of the spectrum after modulation, and how non-Gaussian states are generated after a precise energy measurement. Furthermore, we present a strategy combining a single-stage electron modulation and post-filtering to harness tailored light states, such as squeezed vacuum, cat, and triangular cat states, with fidelity close to 100%.
A "Schrödinger cat" state of free-propagating light can be defined as a quantum superposition of well separated coherent states. 1, 2 We demonstrated, theoretically and experimentally, a protocol which allows to generate arbitrarily large squeezed Schrödinger cat states, using a homodyne detection and photon number states as resources. We implemented this protocol experimentally with light pulses containing two photons, producing a squeezed Schrödinger cat state with a negative Wigner function. This state clearly presents several quantum phase-space interference fringes between the "dead" and "alive" components, and it is large enough to become useful for experimental tests of quantum theory and quantum information processing.
Abstract Many technologies emerging from quantum information science heavily rely upon the generation and manipulation of entangled quantum states. Here, we propose and demonstrate a new class of quantum interference phenomena that arise when states are created in and coherently converted between the propagating modes of an optical microcavity. The modal coupling introduces several new creation pathways to a nonlinear optical process within the device, which quantum mechanically interfere to drive the system between states in the time domain. The coherent conversion entangles the generated biphotons between propagation pathways, leading to cyclically evolving path-entanglement and the manifestation of coherent oscillations in second-order temporal correlations. Furthermore, the rich device physics is harnessed to tune properties of the quantum states. In particular, we show that the strength of interference between pathways can be coherently controlled, allowing for manipulation of the degree of entanglement, which can even be entirely quenched. The states can likewise be made to flip-flop between exhibiting initially correlated or uncorrelated behavior. The phenomena presented here open a route to creating higher dimensional entanglement and exotic multi-photon states.