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arXiv:2501.16771

Tunable quantum light by modulated free electrons

Valerio Di Giulio, Rudolf Haindl, Claus Ropers

Published Jan 28, 2025• 0 citations
arXivHTMLPDF

Abstract

Nonclassical states of light are fundamental in various applications, spanning quantum computation to enhanced sensing. Fast free electrons, which emit light into photonic structures through the mechanism of spontaneous emission, represent a promising platform for generating diverse types of states. Indeed, the intrinsic connection between the input electron wave function and the output light field suggests that electron-shaping schemes, based on light-induced scattering, facilitates their synthesis. In this article, we present a theoretical framework capable of predicting the final optical density matrix of a generic N-electron state that can also account for post-sample energy filtering. By using such framework, we study the modulation-dependent fluctuations of the N-electron emission and identify regions of Poissonian and super-Poissonian statistics. In the single-electron case, we show how coherent states with nearly 90% purity can be formed by pre-filtering a portion of the spectrum after modulation, and how non-Gaussian states are generated after a precise energy measurement. Furthermore, we present a strategy combining a single-stage electron modulation and post-filtering to harness tailored light states, such as squeezed vacuum, cat, and triangular cat states, with fidelity close to 100%.

DOI
10.48550/arxiv.2501.16771

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Nonclassical states of light are fundamental in various applications, spanning quantum computation to enhanced sensing. Fast free electrons, which emit light into photonic structures through the mechanism of spontaneous emission, represent a promising platform for generating diverse types of states. Indeed, the intrinsic connection between the input electron wave function and the output light field suggests that electron-shaping schemes, based on light-induced scattering, facilitates their synthesis. In this article, we present a theoretical framework capable of predicting the final optical density matrix of a generic N-electron state that can also account for post-sample energy filtering. By using such framework, we study the modulation-dependent fluctuations of the N-electron emission and identify regions of Poissonian and super-Poissonian statistics. In the single-electron case, we show how coherent states with nearly 90% purity can be formed by pre-filtering a portion of the spectrum after modulation, and how non-Gaussian states are generated after a precise energy measurement. Furthermore, we present a strategy combining a single-stage electron modulation and post-filtering to harness tailored light states, such as squeezed vacuum, cat, and triangular cat states, with fidelity close to 100%.
Abstract Nonclassical states of light are fundamental in various applications, spanning quantum computation to enhanced sensing. Fast free electrons, which emit light into photonic structures through the mechanism of spontaneous emission, represent a promising platform for generating diverse types of states. Indeed, the intrinsic connection between the input electron wave function and the output light field suggests that electron‐shaping schemes, based on light‐induced scattering, facilitate their synthesis. In this article, we present a theoretical framework capable of predicting the final optical density matrix emitted by a generic N ‐electron state that can also account for post‐sample energy filtering. By using such a framework, we study the modulation‐dependent fluctuations of the N ‐electron emission and identify regions of superradiant scaling characterized by Poissonian and super‐Poissonian statistics. In this context, we predict that high‐ N modulated electron pulses can yield a tenfold shot‐noise suppression in the estimation of the electron‐light coupling when the output radiation intensity is analyzed. In the single‐electron case, we show how coherent states with nearly 90 % purity can be formed by pre‐filtering a portion of the spectrum after modulation, and how non‐Gaussian states are generated after a precise energy measurement. Furthermore, we present a strategy combining a single‐stage electron modulation and post‐filtering to harness tailored light states, such as squeezed vacuum, cat, and triangular cat states, with fidelities close to 100 %.
Harnessing a beam of slow free electrons in artificial photonic structures offers a powerful, tunable platform for generating nonclassical light without the need for heavy physical equipment. Here we present a theory of nonclassical lasing, demonstrating how incoherent electrons in photonic crystal cavities can coherently emit photons through collective dynamics. When photon emission rate exceeds cavity losses, nonclassical lasing with sub-Poissonian photon statistics emerges, driven by multi-photon Rabi oscillations. At specific coupling strengths, quantum state trapping effect emerges, producing high-fidelity Fock states at room temperature (e.g. nearly 90%-fidelity of four photon Fock state). Notably, the frequency of the emitted photons can be readily tuned via the velocity of the injected electrons to match cavity modes. This approach supports photonic integration and offers a scalable, energy-efficient platform for room-temperature quantum light sources and advanced studies in quantum electrodynamics.
The novel quantum effects induced by the free-electron-photons interaction have attracted increasing interest due to their potential applications in ultrafast quantum information processing. Here, we propose a scheme to generate optical cat states based on the quantum interference of multi-path free-electron-photons interactions that take place simultaneously with strong coupling strength. By performing a projection measurement on the electron, the state of light changes significantly from a coherent state into a non-Gaussian state with either Wigner negativity or squeezing property, both possess metrological power to achieve quantum advantage. More importantly, we show that the Wigner negativity oscillates with the coupling strength, and the optical cat states are successfully generated with high fidelity at all the oscillation peaks. This oscillation reveals the quantum interference effect of the multiple quantum pathways in the interaction of the electron with photons, by that various nonclassical states of light are promising to be fast prepared and manipulated. These findings inspire further exploration of emergent quantum phenomena and advanced quantum technologies with free electrons.
It has been shown that the spontaneous emission rate of photons by free electrons, unlike stimulated emission, is independent of the shape or modulation of the quantum electron wavefunction (QEW). Nevertheless, here we show that the quantum state of the emitted photons is non-classical and does depend on the QEW shape. This non-classicality originates from the shape dependent off-diagonal terms of the photon density matrix. This is manifested in the Wigner distribution function and would be observable experimentally through homodyne detection techniques as a squeezing effect. Considering a scheme of electrons interaction with a single microcavity mode, we present a QED formulation of spontaneous emission by multiple modulated QEWs through a build-up process. Our findings indicate that in the case of a density modulated QEWs beam, the phase of the off-diagonal terms of the photon state emitted by the modulated QEWs is the harbinger of bunched beam superradiance, where the spontaneous emission is proportional toNe2. This observation offers a potential for enhancement of other quantum electron interactions with quantum systems by a modulated QEWs beam carrying coherence and quantum properties of the modulation.
It has been shown that the spontaneous emission rate of photons by free electrons, unlike stimulated emission, is independent of the shape or modulation of the quantum electron wavefunction (QEW). Nevertheless, here we show that the quantum state of the emitted photons is non-classical and does depend on the QEW shape. This non-classicality originates from the shape dependent off-diagonal terms of the photon density matrix. This is manifested in the Wigner distribution function and would be observable experimentally through Homodyne detection techniques as a squeezing effect. Considering a scheme of electrons interaction with a single microcavity mode, we present a QED formulation of spontaneous emission by multiple modulated QEWs through a build-up process. Our findings indicate that in the case of a density modulated QEWs beam, the phase of the off-diagonal terms of the photon state emitted by the modulated QEWs is the harbinger of bunched beam superradiance, where the spontaneous emission is proportional to N_e^2. This observation offers a potential for enhancement of other quantum electron interactions with quantum systems by a modulated QEWs beam carrying coherence and quantum properties of the modulation.
A versatile quantum light source capable of programmably generating a variety of quantum light is a key enabler for photonic quantum technologies. In particular, independent control over both the output quantum state and its temporal waveform is essential for realizing diverse functionalities and enhancing processing performance. However, conventional sources of optical non-Gaussian states, a crucial resource for photonic quantum information processing, typically emit fixed states with predetermined temporal waveforms, lacking their programmability. Here, we propose a programmable non-Gaussian quantum light source that offers independent and arbitrary tunability of both the quantum state and the temporal waveform within a single platform. As a distinctive feature, our approach employs a heralding scheme in which these two properties are indirectly engineered to user-defined targets by manipulating the light in the heralding channel, thereby avoiding optical losses associated with direct manipulation of the heralded quantum light. We develop a prototype and demonstrate the generation of single-photon, Schrödinger cat, and two-photon states in a variety of unconventional temporal waveforms without degradation in state quality. This platform provides a versatile tool for tailoring quantum light to specific applications, significantly expanding the capabilities of photonic quantum technologies.