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arXiv:2306.01486

Robust and scalable rf spectroscopy in first-order magnetic sensitive states at second-long coherence time

Yeh, C. -H., Kai C. Grensemann, Laura S. Dreissen, Henning A. Fürst, T. E. Mehlstäubler

Published Jun 2, 2023• 0 citations
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Abstract

Trapped-ion quantum sensors have become highly sensitive tools for the search of physics beyond the Standard Model. Recently, stringent tests of local Lorentz-invariance (LLI) have been conducted with precision spectroscopy in trapped ions. We here elaborate on robust radio-frequency composite-pulse spectroscopy at second long coherence times in the magnetic sublevels of the long-lived $^{2}F_{7/2}$ state of a trapped $^{172}$Yb$^{+}$ ion which is scalable to spatially extended multi-ion systems. We compare two Ramsey-type composite rf pulse sequences, a GSE sequence and a UR10 that decouple the energy levels from magnetic field noise, enabling robust and accurate spectroscopy. Both sequences are characterized theoretically and experimentally in the spin-$1/2$\ $^{2}S_{1/2}$ electronic ground state of $^{172}$Yb$^+$ and results show that the UR10 sequence is 38 (13) times more robust against pulse duration (frequency detuning) errors than the GSE sequence. We extend our simulations to the eight-level manifold of the $^2F_{7/2}$ state, which is highly sensitive to a possible violation of LLI, and show that the UR10 sequence can be used for high-fidelity Ramsey spectroscopy in noisy environments. The UR10 sequence is implemented experimentally in the $^2F_{7/2}$ manifold and a coherent signal of up to 2.5\,s is reached. In reference we have implemented this sequence and used it to perform the most stringent test of LLI in the electron-photon sector to date with a single Yb$^{+}$ ion. Due to the high robustness of the UR10 sequence, it can be applied on larger ion crystals to improve tests of Lorentz symmetry further. We demonstrate that the sequence can also be used to extract the quadrupole moment of the meta-stable $^{2}F_{7/2}$ state, obtaining a value of $Θ\,=\,-0.0298(38)\,ea^{2}_{0}$ which is in agreement with the value deduced from clock measurements.

DOI
10.48550/arxiv.2306.01486

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Trapped-ion quantum sensors have become highly sensitive tools for the search of physics beyond the Standard Model. Recently, stringent tests of local Lorentz-invariance (LLI) have been conducted with precision spectroscopy in trapped ions. We here elaborate on robust radio-frequency composite-pulse spectroscopy at second long coherence times in the magnetic sublevels of the long-lived 2F7/2^{2}F_{7/2}2F7/2​ state of a trapped 172^{172}172Yb+^{+}+ ion which is scalable to spatially extended multi-ion systems. We compare two Ramsey-type composite rf pulse sequences, a GSE sequence and a UR10 that decouple the energy levels from magnetic field noise, enabling robust and accurate spectroscopy. Both sequences are characterized theoretically and experimentally in the spin-1/21/21/2\ 2S1/2^{2}S_{1/2}2S1/2​ electronic ground state of 172^{172}172Yb+^++ and results show that the UR10 sequence is 38 (13) times more robust against pulse duration (frequency detuning) errors than the GSE sequence. We extend our simulations to the eight-level manifold of the 2F7/2^2F_{7/2}2F7/2​ state, which is highly sensitive to a possible violation of LLI, and show that the UR10 sequence can be used for high-fidelity Ramsey spectroscopy in noisy environments. The UR10 sequence is implemented experimentally in the 2F7/2^2F_{7/2}2F7/2​ manifold and a coherent signal of up to 2.5,s is reached. In reference we have implemented this sequence and used it to perform the most stringent test of LLI in the electron-photon sector to date with a single Yb+^{+}+ ion. Due to the high robustness of the UR10 sequence, it can be applied on larger ion crystals to improve tests of Lorentz symmetry further. We demonstrate that the sequence can also be used to extract the quadrupole moment of the meta-stable 2F7/2^{2}F_{7/2}2F7/2​ state, obtaining a value of Θ = −0.0298(38) ea02Θ\,=\,-0.0298(38)\,ea^{2}_{0}Θ=−0.0298(38)ea02​ which is in agreement with the value deduced from clock measurements.
Trapped-ion quantum sensors have become highly sensitive tools for the search of physics beyond the Standard Model. Recently, stringent tests of local Lorentz-invariance (LLI) have been conducted with precision spectroscopy in trapped ions (Pruttivarasin et al 2015 Nature 517 592-5, Megidish et al 2019 Phys. Rev. Lett. 122 123605, Sanner et al 2019 Nature 567 204-8, Dreissen et al 2022 Nat. Commun. 13 1-6) . We here elaborate on robust radio-frequency composite-pulse spectroscopy at second long coherence times in the magnetic sublevels of the long-lived 2F7/2 state of a trapped 172Yb+ ion which is scalable to spatially extended multi-ion systems. We compare two Ramsey-type composite rf pulse sequences, a generalized spin-echo (GSE) sequence (Shaniv et al 2018 Phys. Rev. Lett. 120 103202) and a sequence based on universal rotations with 10 rephasing pulses (UR10) (Genov et al 2017 Phys. Rev. Lett. 118 133202) that decouple the energy levels from magnetic field noise, enabling robust and accurate spectroscopy. Both sequences are characterized theoretically and experimentally in the spin- 1 / 22 S1/2 electronic ground state of 172Yb+ and results show that the UR10 sequence is 38 (13) times more robust against pulse duration (frequency detuning) errors than the GSE sequence. We extend our simulations to the eight-level manifold of the 2F7/2 state, which is highly sensitive to a possible violation of LLI, and show that the UR10 sequence can be used for high-fidelity Ramsey spectroscopy in noisy environments. The UR10 sequence is implemented experimentally in the 2F7/2 manifold and a coherent signal of up to 2.5 s is reached. In (Dreissen et al 2022 Nat. Commun. 13 1-6) we have implemented this sequence and used it to perform the most stringent test of LLI in the electron-photon sector to date with a single Yb+ ion. Due to the high robustness of the UR10 sequence, it can be applied on larger ion crystals to improve tests of Lorentz symmetry further. We demonstrate that the sequence can also be used to extract the quadrupole moment of the meta-stable 2F7/2 state, obtaining a value of Θ = - 0.0298 (38)ea02 which is in agreement with the value deduced from clock measurements (Lange et al 2020 Phys. Rev. Lett. 125 143201).
Abstract Trapped-ion quantum sensors have become highly sensitive tools for the search of physics beyond the Standard Model. Recently, stringent tests of local Lorentz-invariance (LLI) have been conducted with precision spectroscopy in trapped ions (Pruttivarasin et al 2015 Nature 517 592–5, Megidish et al 2019 Phys. Rev. Lett. 122 123605, Sanner et al 2019 Nature 567 204–8, Dreissen et al 2022 Nat. Commun. 13 1–6) . We here elaborate on robust radio-frequency composite-pulse spectroscopy at second long coherence times in the magnetic sublevels of the long-lived 2 F 7 / 2 state of a trapped 172Yb+ ion which is scalable to spatially extended multi-ion systems. We compare two Ramsey-type composite rf pulse sequences, a generalized spin-echo (GSE) sequence (Shaniv et al 2018 Phys. Rev. Lett. 120 103202) and a sequence based on universal rotations with 10 rephasing pulses (UR10) (Genov et al 2017 Phys. Rev. Lett. 118 133202) that decouple the energy levels from magnetic field noise, enabling robust and accurate spectroscopy. Both sequences are characterized theoretically and experimentally in the spin- 1 / 2 2 S 1 / 2 electronic ground state of 172Yb+ and results show that the UR10 sequence is 38 (13) times more robust against pulse duration (frequency detuning) errors than the GSE sequence. We extend our simulations to the eight-level manifold of the 2 F 7 / 2 state, which is highly sensitive to a possible violation of LLI, and show that the UR10 sequence can be used for high-fidelity Ramsey spectroscopy in noisy environments. The UR10 sequence is implemented experimentally in the 2 F 7 / 2 manifold and a coherent signal of up to 2.5 s is reached. In (Dreissen et al 2022 Nat. Commun. 13 1–6) we have implemented this sequence and used it to perform the most stringent test of LLI in the electron–photon sector to date with a single Yb+ ion. Due to the high robustness of the UR10 sequence, it can be applied on larger ion crystals to improve tests of Lorentz symmetry further. We demonstrate that the sequence can also be used to extract the quadrupole moment of the meta-stable 2 F 7 / 2 state, obtaining a value of Θ = − 0.0298 ( 38 ) e a 0 2 which is in agreement with the value deduced from clock measurements (Lange et al 2020 Phys. Rev. Lett. 125 143201).
Abstract In attempts to unify the four known fundamental forces in a single quantum-consistent theory, it is suggested that Lorentz symmetry may be broken at the Planck scale. Here we search for Lorentz violation at the low-energy limit by comparing orthogonally oriented atomic orbitals in a Michelson-Morley-type experiment. We apply a robust radiofrequency composite pulse sequence in the 2 F 7/2 manifold of an Yb + ion, extending the coherence time from 200 μ s to more than 1 s. In this manner, we fully exploit the high intrinsic susceptibility of the 2 F 7/2 state and take advantage of its exceptionally long lifetime. We match the stability of the previous best Lorentz symmetry test nearly an order of magnitude faster and improve the constraints on the symmetry breaking coefficients to the 10 −21 level. These results represent the most stringent test of this type of Lorentz violation. The demonstrated method can be further extended to ion Coulomb crystals.
Quantum magnetometry represents a fundamental component of quantum metrology, where trapped-ion systems have achieved pT/Hz\rm{pT}/\sqrt{\rm{Hz}}pT/Hz​ sensitivity in single-ion radio-frequency magnetic field measurements via dressed states based dynamical decoupling. Here we propose a scalable trapped-ion magnetometer utilizing the mixed dynamical decoupling method, combining dressed states with periodic sequences to suppress decoherence and spatial magnetic field inhomogeneity. With numerical simulations for a 10410^4104 ion system with realistic experimental parameters, we demonstrate that a sensitivity of 13 fT/Hz\rm{fT}/\sqrt{\rm{Hz}}fT/Hz​ for the radio-frequency field could be reached. Such a sensitivity could be obtained via robust resilience to magnetic field drift noise and inhomogeneity, where coherence time could be extended to the order of several minutes on average. This method enables scalable trapped-ion magnetometry, demonstrating its potential as a robust and practical solution for advancing quantum sensing applications.
This thesis describes an ion trap magnetometer, in which experimental hardware and theory for trapped ion magnetometry has been developed and demonstrated. Quantum magnetometry has been a fast expanding field in recent years due to the plethora of military, medical and security applications. The current quantum magnetometer literature has shown great improvements on the standard magnetometer success metrics such as sensitivity, spacial resolution, frequency tuneability, noise shielding and vector field resolution. Ion trap magnetometry could potentially boast several advantages over some of the better established methods such as, nano-meter spatial resolution, broadband tuneability over radio-frequency (RF) and microwave frequencies, and magnetic field noise shielding and sensitivity improvements through dynamic decoupling methods; all in room temperature environments. The experimental setup discussed uses a micro-fabricated Paul trap for ion confinement due to the scalability of this technology. The method for sensing that was demonstrated utilises long-wavelength radiation dressed states to extend the coherence time of a single 171Yb+ ion beyond the bare states and to allow for a high level of frequency tuneability. The coherence times measured were T2 = 0:645 s for RF field sensing at 15.616 MHz and T2 = 1.153 s for microwave field sensing at 12.658466 GHz. Sensitivities of SB = 125.857 ± 26.155 pT/ vHz for RF magnetic fields and SB = 102.054 ± 11.046 pT/ vHz for microwave magnetic fields were achieved experimentally. A novel micro-fabricated Paul trap for trapping multiple ion clusters was developed to improve sensitivity values by increasing the total number of trapped ions. The design confines ions over a two-dimensional surface spanning 0.65 x 1.00 mm which would also allow for magnetic field gradient measurements. Efforts have been made to miniaturise certain experimental hardware to further the development of portable trapped ion experiments. For this, a miniaturised RF resonator that could be used for radial confinement of ions within Paul traps has been developed. At the current stage of development it is capable of applying a peak RF voltage of 114.9 V with a Q value of 70 at a resonant frequency of O/2p = 12.65 MHz.
Scalability is a challenging yet key aspect required for large scale quantum computing and simulation using ions trapped in radio-frequency (rf) Paul traps. In this thesis 171Yb+ ions are used to demonstrate a magnetic field insensitive qubit which has a measured coherence time of 1.5 s, making it an ideal candidate to use for storing quantum information. A magnetic field sensitive qubit is also characterised which can be used for the implementation of multi-qubit gates using a potentially very scalable scheme based on microwaves in conjunction with a static magnetic field gradient instead of using lasers. However, the measured coherence time is limited by magnetic field fluctuations and will prohibit high fidelity gate operations from being performed. To address this issue, the preparation of a dressed-state qubit using a microwave based stimulated rapid adiabatic passage (STIRAP) pulse sequence will be presented. This qubit is protected against the noisy environment making it less sensitive to magnetic field fluctuations. The lifetime of this qubit is measured to demonstrate its suitability for storing quantum information. A powerful method for manipulating the dressed-state qubit will be presented and is used to measure a coherence time of the qubit of 500 ms which is two orders of magnitude longer compared to the magnetic field sensitive qubit. It will also be shown that our method allows for the implementation of arbitrary rotations of the dressed-state qubit on the Bloch sphere using only a single rf field. This substantially simplifies the experimental setup for single and multi-qubit gates. Furthermore, this thesis will present a experimental setup capable of successfully operating microfabricated surface ion traps. This setup is then used to operate and characterise the first two-dimensional (2D) lattice of ion traps on a microchip. A unique feature of the microfabrication technique used for this device is the extremely large voltage that can be applied which allows long ion lifetimes along with large secular frequencies to be measured, demonstrating the robustness of this device. Rudimentary shuttling between neighbouring lattice sites will be shown which could be used as part of a efficient scheme to load a large lattice of ions. One of the many applications of a 2D lattice of ions lies in the field of quantum simulations where many-body systems such as quantum magnetism, high temperature superconductivity, the fractional quantum hall effect and synthetic gauge fields can be simulated. It will be shown how making only minor modifications to the microchip the ion-ion separation can be reduced sufficiently to offer an exciting platform for the successful implementation of 2D quantum simulations. A theoretical investigation on the optimal 2D ion trap lattice geometry will also be presented with the aim to maximise the ratio of ion-ion coupling strength to decoherence from motional heating of the ions and to laser induced off-resonant coupling.