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arXiv:2206.00570 · Nature Communications

Improved bounds on Lorentz violation from composite pulse Ramsey spectroscopy in a trapped ion

Laura S. Dreissen, Chih-Han Yeh, Henning A. Fürst, Kai C. Grensemann, T. E. Mehlstäubler

Published Nov 27, 2022• 48 citations
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Abstract

Abstract In attempts to unify the four known fundamental forces in a single quantum-consistent theory, it is suggested that Lorentz symmetry may be broken at the Planck scale. Here we search for Lorentz violation at the low-energy limit by comparing orthogonally oriented atomic orbitals in a Michelson-Morley-type experiment. We apply a robust radiofrequency composite pulse sequence in the 2 F 7/2 manifold of an Yb + ion, extending the coherence time from 200 μ s to more than 1 s. In this manner, we fully exploit the high intrinsic susceptibility of the 2 F 7/2 state and take advantage of its exceptionally long lifetime. We match the stability of the previous best Lorentz symmetry test nearly an order of magnitude faster and improve the constraints on the symmetry breaking coefficients to the 10 −21 level. These results represent the most stringent test of this type of Lorentz violation. The demonstrated method can be further extended to ion Coulomb crystals.

DOI
10.1038/s41467-022-34818-0

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Trapped-ion quantum sensors have become highly sensitive tools for the search of physics beyond the Standard Model. Recently, stringent tests of local Lorentz-invariance (LLI) have been conducted with precision spectroscopy in trapped ions. We here elaborate on robust radio-frequency composite-pulse spectroscopy at second long coherence times in the magnetic sublevels of the long-lived $^{2}F_{7/2}$ state of a trapped $^{172}$Yb$^{+}$ ion which is scalable to spatially extended multi-ion systems. We compare two Ramsey-type composite rf pulse sequences, a GSE sequence and a UR10 that decouple the energy levels from magnetic field noise, enabling robust and accurate spectroscopy. Both sequences are characterized theoretically and experimentally in the spin-$1/2$\ $^{2}S_{1/2}$ electronic ground state of $^{172}$Yb$^+$ and results show that the UR10 sequence is 38 (13) times more robust against pulse duration (frequency detuning) errors than the GSE sequence. We extend our simulations to the eight-level manifold of the $^2F_{7/2}$ state, which is highly sensitive to a possible violation of LLI, and show that the UR10 sequence can be used for high-fidelity Ramsey spectroscopy in noisy environments. The UR10 sequence is implemented experimentally in the $^2F_{7/2}$ manifold and a coherent signal of up to 2.5\,s is reached. In reference we have implemented this sequence and used it to perform the most stringent test of LLI in the electron-photon sector to date with a single Yb$^{+}$ ion. Due to the high robustness of the UR10 sequence, it can be applied on larger ion crystals to improve tests of Lorentz symmetry further. We demonstrate that the sequence can also be used to extract the quadrupole moment of the meta-stable $^{2}F_{7/2}$ state, obtaining a value of $Θ\,=\,-0.0298(38)\,ea^{2}_{0}$ which is in agreement with the value deduced from clock measurements.

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This dissertation reports on precision measurements of the atomic structure of calcium ions (40Ca+), application of trapped 40Ca+ ions as a probe for a violation of fundamental symmetry and prospects of performing quantum simulations with trapped ion.We demonstrate a novel technique to perform spectroscopy on the dipole transition of 40Ca+ that circumvents usual difficulties from dark resonances and Doppler heating. The center of the atomic transition can be detected to a precision of 200 kHz or less with an integration time of 10 minutes. We apply this method to directly measure the influence of micromotion on the fluorescence spectra and confirm the dependence of the modulation index on the radial trap frequency. We measure the branching fraction of the excited 2P1/2 state of 40Ca+ to be 0.93565(7) using a simple experimental scheme readily applicable to many other ion species. Our result for 40Ca+ distinguishes well among various theoretically calculated values, which is important in guiding further developments of the theoretical work.We apply the Ramsey spectroscopy technique based on a pair of correlated ions to probe the effect of the violation of local Lorentz invariance (LLI). The energy difference between the two components of the Bell state |PsiB> = |mJ=5/2,mJ=-5/2>+|mJ=1/2,mJ=-1/2> in the D5/2 manifold of 40Ca+ is monitored for 12 hours. We found that the energy component related to the violation of LLI varies less than 17±22 mHz. Assuming a hydrogen-like model of 40Ca+, the measurement result provides us the bound of the LLI parameter C(2)0 to be 1.7±2.2x10-17.Based on numerical simulations, we show that the Aubry transition in the Frenkel-Kontorova model with trapped ion can be observed for practical experimental parameters such as the strength and wavelength of the optical lattice, which serves as an external perturbing periodic potential. Moreover, we also show that the normal mode structure of ion chain can change significantly as we vary the strength of the optical lattice.

•Jan 1, 2014•5 citations
Abstract In attempts to unify the four known fundamental forces in a single quantum-consistent theory, it is suggested that Lorentz symmetry may be broken at the Planck scale. Here we search for Lorentz violation at the low-energy limit by comparing orthogonally oriented atomic orbitals in a Michelson-Morley-type experiment. We apply a robust radiofrequency composite pulse sequence in the 2 F 7/2 manifold of an Yb + ion, extending the coherence time from 200 μ s to more than 1 s. In this manner, we fully exploit the high intrinsic susceptibility of the 2 F 7/2 state and take advantage of its exceptionally long lifetime. We match the stability of the previous best Lorentz symmetry test nearly an order of magnitude faster and improve the constraints on the symmetry breaking coefficients to the 10 −21 level. These results represent the most stringent test of this type of Lorentz violation. The demonstrated method can be further extended to ion Coulomb crystals.
Trapped-ion quantum sensors have become highly sensitive tools for the search of physics beyond the Standard Model. Recently, stringent tests of local Lorentz-invariance (LLI) have been conducted with precision spectroscopy in trapped ions. We here elaborate on robust radio-frequency composite-pulse spectroscopy at second long coherence times in the magnetic sublevels of the long-lived 2F7/2^{2}F_{7/2}2F7/2​ state of a trapped 172^{172}172Yb+^{+}+ ion which is scalable to spatially extended multi-ion systems. We compare two Ramsey-type composite rf pulse sequences, a GSE sequence and a UR10 that decouple the energy levels from magnetic field noise, enabling robust and accurate spectroscopy. Both sequences are characterized theoretically and experimentally in the spin-1/21/21/2\ 2S1/2^{2}S_{1/2}2S1/2​ electronic ground state of 172^{172}172Yb+^++ and results show that the UR10 sequence is 38 (13) times more robust against pulse duration (frequency detuning) errors than the GSE sequence. We extend our simulations to the eight-level manifold of the 2F7/2^2F_{7/2}2F7/2​ state, which is highly sensitive to a possible violation of LLI, and show that the UR10 sequence can be used for high-fidelity Ramsey spectroscopy in noisy environments. The UR10 sequence is implemented experimentally in the 2F7/2^2F_{7/2}2F7/2​ manifold and a coherent signal of up to 2.5\,s is reached. In reference we have implemented this sequence and used it to perform the most stringent test of LLI in the electron-photon sector to date with a single Yb+^{+}+ ion. Due to the high robustness of the UR10 sequence, it can be applied on larger ion crystals to improve tests of Lorentz symmetry further. We demonstrate that the sequence can also be used to extract the quadrupole moment of the meta-stable 2F7/2^{2}F_{7/2}2F7/2​ state, obtaining a value of Θ = −0.0298(38) ea02Θ\,=\,-0.0298(38)\,ea^{2}_{0}Θ=−0.0298(38)ea02​ which is in agreement with the value deduced from clock measurements.
Trapped-ion quantum sensors have become highly sensitive tools for the search of physics beyond the Standard Model. Recently, stringent tests of local Lorentz-invariance (LLI) have been conducted with precision spectroscopy in trapped ions (Pruttivarasin et al 2015 Nature 517 592-5, Megidish et al 2019 Phys. Rev. Lett. 122 123605, Sanner et al 2019 Nature 567 204-8, Dreissen et al 2022 Nat. Commun. 13 1-6) . We here elaborate on robust radio-frequency composite-pulse spectroscopy at second long coherence times in the magnetic sublevels of the long-lived 2F7/2 state of a trapped 172Yb+ ion which is scalable to spatially extended multi-ion systems. We compare two Ramsey-type composite rf pulse sequences, a generalized spin-echo (GSE) sequence (Shaniv et al 2018 Phys. Rev. Lett. 120 103202) and a sequence based on universal rotations with 10 rephasing pulses (UR10) (Genov et al 2017 Phys. Rev. Lett. 118 133202) that decouple the energy levels from magnetic field noise, enabling robust and accurate spectroscopy. Both sequences are characterized theoretically and experimentally in the spin- 1 / 22 S1/2 electronic ground state of 172Yb+ and results show that the UR10 sequence is 38 (13) times more robust against pulse duration (frequency detuning) errors than the GSE sequence. We extend our simulations to the eight-level manifold of the 2F7/2 state, which is highly sensitive to a possible violation of LLI, and show that the UR10 sequence can be used for high-fidelity Ramsey spectroscopy in noisy environments. The UR10 sequence is implemented experimentally in the 2F7/2 manifold and a coherent signal of up to 2.5 s is reached. In (Dreissen et al 2022 Nat. Commun. 13 1-6) we have implemented this sequence and used it to perform the most stringent test of LLI in the electron-photon sector to date with a single Yb+ ion. Due to the high robustness of the UR10 sequence, it can be applied on larger ion crystals to improve tests of Lorentz symmetry further. We demonstrate that the sequence can also be used to extract the quadrupole moment of the meta-stable 2F7/2 state, obtaining a value of Θ = - 0.0298 (38)ea02 which is in agreement with the value deduced from clock measurements (Lange et al 2020 Phys. Rev. Lett. 125 143201).
Abstract Trapped-ion quantum sensors have become highly sensitive tools for the search of physics beyond the Standard Model. Recently, stringent tests of local Lorentz-invariance (LLI) have been conducted with precision spectroscopy in trapped ions (Pruttivarasin et al 2015 Nature 517 592–5, Megidish et al 2019 Phys. Rev. Lett. 122 123605, Sanner et al 2019 Nature 567 204–8, Dreissen et al 2022 Nat. Commun. 13 1–6) . We here elaborate on robust radio-frequency composite-pulse spectroscopy at second long coherence times in the magnetic sublevels of the long-lived 2 F 7 / 2 state of a trapped 172Yb+ ion which is scalable to spatially extended multi-ion systems. We compare two Ramsey-type composite rf pulse sequences, a generalized spin-echo (GSE) sequence (Shaniv et al 2018 Phys. Rev. Lett. 120 103202) and a sequence based on universal rotations with 10 rephasing pulses (UR10) (Genov et al 2017 Phys. Rev. Lett. 118 133202) that decouple the energy levels from magnetic field noise, enabling robust and accurate spectroscopy. Both sequences are characterized theoretically and experimentally in the spin- 1 / 2 2 S 1 / 2 electronic ground state of 172Yb+ and results show that the UR10 sequence is 38 (13) times more robust against pulse duration (frequency detuning) errors than the GSE sequence. We extend our simulations to the eight-level manifold of the 2 F 7 / 2 state, which is highly sensitive to a possible violation of LLI, and show that the UR10 sequence can be used for high-fidelity Ramsey spectroscopy in noisy environments. The UR10 sequence is implemented experimentally in the 2 F 7 / 2 manifold and a coherent signal of up to 2.5 s is reached. In (Dreissen et al 2022 Nat. Commun. 13 1–6) we have implemented this sequence and used it to perform the most stringent test of LLI in the electron–photon sector to date with a single Yb+ ion. Due to the high robustness of the UR10 sequence, it can be applied on larger ion crystals to improve tests of Lorentz symmetry further. We demonstrate that the sequence can also be used to extract the quadrupole moment of the meta-stable 2 F 7 / 2 state, obtaining a value of Θ = − 0.0298 ( 38 ) e a 0 2 which is in agreement with the value deduced from clock measurements (Lange et al 2020 Phys. Rev. Lett. 125 143201).
We develop a theory of composite Ramsey sequences of rf pulses interacting with the Zeeman structure at the long-lived atomic level, beyond the rotating wave approximation. Such sequences are proposed in experiments to detect the violation of local Lorentz invariance [R. Shaniv, R. Ozeri, M.S. Safronova, S.G. Porsev, V.A. Dzuba, V.V. Flambaum, and H. Häffner, Phys. Rev. Lett. 120, 103202 (2018)]. Based on Fourier analysis, we have shown that taking into account non-resonant contributions leads to a radical change in the dynamics of the quantum system (with respect to the rotating wave approximation) in the case when the number of Ramsey pulses exceeds several tens. As a result, the effectiveness of using such rf pulses sequences to test local Lorentz invariance has not yet been fully determined and requires additional research.
Since extensions of the standard model have been developed that predict violations of local Lorentz invariance (LLI), precision measurement groups have been working to reduce experimental bounds of the associated matrix element. Using an analogue of the Michelson-Morley test with trapped Ca+ ions, the current bound has been set at one part in 1018. However, by instead using Yb+ ions, which have highly stable electronic states for storing quantum information compared to their counterparts and exhibit enhanced effects of LLI breaking asymmetries, we can push the bounds to one part in 1023. In this article, we outline a configuration for such an experiment and offer solutions to experimental concerns. We develop an algorithm for state creation, manipulation, and measurement that minimizes measurement time and transition uncertainty. We also discuss necessary hardware for trapping and manipulating ions including a vacuum system, a Paul trap and the associated electrode voltage supplies, and an optics system for generating and applying transition pulses. The experiment is specifically designed to utilize the existing ion trap hardware in place at the Richerme lab at Indiana University Bloomington.
This dissertation reports on precision measurements of the atomic structure of calcium ions (40Ca+), application of trapped 40Ca+ ions as a probe for a violation of fundamental symmetry and prospects of performing quantum simulations with trapped ion.We demonstrate a novel technique to perform spectroscopy on the dipole transition of 40Ca+ that circumvents usual difficulties from dark resonances and Doppler heating. The center of the atomic transition can be detected to a precision of 200 kHz or less with an integration time of 10 minutes. We apply this method to directly measure the influence of micromotion on the fluorescence spectra and confirm the dependence of the modulation index on the radial trap frequency. We measure the branching fraction of the excited 2P1/2 state of 40Ca+ to be 0.93565(7) using a simple experimental scheme readily applicable to many other ion species. Our result for 40Ca+ distinguishes well among various theoretically calculated values, which is important in guiding further developments of the theoretical work.We apply the Ramsey spectroscopy technique based on a pair of correlated ions to probe the effect of the violation of local Lorentz invariance (LLI). The energy difference between the two components of the Bell state |PsiB> = |mJ=5/2,mJ=-5/2>+|mJ=1/2,mJ=-1/2> in the D5/2 manifold of 40Ca+ is monitored for 12 hours. We found that the energy component related to the violation of LLI varies less than 17±22 mHz. Assuming a hydrogen-like model of 40Ca+, the measurement result provides us the bound of the LLI parameter C(2)0 to be 1.7±2.2x10-17.Based on numerical simulations, we show that the Aubry transition in the Frenkel-Kontorova model with trapped ion can be observed for practical experimental parameters such as the strength and wavelength of the optical lattice, which serves as an external perturbing periodic potential. Moreover, we also show that the normal mode structure of ion chain can change significantly as we vary the strength of the optical lattice.