Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Log inSign up
Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Blog
Job Board
Q3AS

© 2026 Aqora Quantum S.A.S.

TermsPrivacyLegal Notice

arXiv:2303.15150

High-dimensional frequency conversion in hot atomic system

Weihang Zhang, Ying-Hao Ye, Lei Zeng, Enze Li, Jingyuan Peng, Dong-Sheng Ding, Bao‐Sen Shi

Published Mar 27, 2023• 1 citation
arXivHTMLPDF

Abstract

One of the major difficulties in realizing a high-dimensional frequency converter for conventional optical vortex (COV) stems from the difference in ring diameter of COV modes with different topological charge numbers l. Here, we implement a high-dimensional frequency convertor for perfect optical vortex (POV) modes with invariant size through the four-wave mixing (FWM) process by utilizing Bessel-Gaussian beams instead of Laguerre-Gaussian beams. The measured conversion efficiency from 1530 nm to 795 nm is independent of l at least in subspace of {-6,...,6}, and the achieved conversion fidelities for two-dimensional (2D) superposed POV states exceed 97%. We further realize the frequency conversion of 3D, 5D and 7D superposition states with fidelities as high as 96.70%, 89.16% and 88.68%, respectively. The reported scheme is implemented in hot atomic vapor, it's also compatible with the cold atomic system and may find applications in high-capacity and long-distance quantum communication.

DOI
10.48550/arxiv.2303.15150

Related papers

High-dimensional frequency conversion in a hot atomic system

Weihang Zhang, Ying-Hao Ye, Lei Zeng +4 more

One of the major difficulties in realizing a high-dimensional frequency converter for conventional optical vortex (COV) modes stems from the difference in ring diameter of the COV modes with different topological charge numbers l.Here, we implement a high-dimensional frequency converter for perfect optical vortex (POV) modes with invariant sizes by way of the four-wave mixing (FWM) process using Bessel-Gaussian beams instead of Laguerre-Gaussian beams.The measured conversion efficiency from 1530 to 795 nm is independent of l at least in subspace l ∈ f-6, : : : , 6g, and the achieved conversion fidelities for two-dimensional (2D) superposed POV states exceed 97%.We further realize the frequency conversion of 3D, 5D, and 7D superposition states with fidelities as high as 96.70%, 89.16%, and 88.68%, respectively.The proposed scheme is implemented in hot atomic vapor.It is also compatible with the cold atomic system and may find applications in high-capacity and long-distance quantum communication.

Chinese Optics Letters•Jan 1, 2023•4 citations

Size-invariant twisted optical modes for the efficient generation of higher-dimensional quantum states

Ali Anwar, Shashi Prabhakar, Ravindra Pratap Singh

Optical vortex beams are profiled as helical wavefronts with a phase singularity carrying an orbital angular momentum (OAM) associated with their spatial distribution. The transverse intensity distribution of a conventional optical vortex has a strong dependence on the carried topological charge. However, perfect optical vortex (POV) beams have their transverse intensity distribution independent of their charge. Such “size-invariant” POV beams have found exciting applications in optical manipulation, imaging, and communication. In this paper, we investigate the use of POV modes in the efficient generation of high-dimensional quantum states of light. We generate heralded single photons carrying OAM using spontaneous parametric downconversion (SPDC) of POV beams. We show that the heralding efficiency of the SPDC single photons generated with a POV pump is greater than that with normal optical vortex beams. The dimensionality of the two-photon OAM states is increased with POV modes in the pump and projective measurements using Bessel–Gaussian vortex modes that give POV, instead of Laguerre–Gaussian modes.

arXiv:2107.02227•Journal of the Optical Society of America B•Aug 17, 2021•8 citations

Generation and manipulation of frequency-converted Airy vortex beam via atomic four-wave mixing

Sandan Wang, Jingyi Zhou, Xuewen Wang +5 more

Airy vortex beams, which integrate orbital angular momentum with diffraction-resistant and self-accelerating characteristics of Airy beams, offer unique capabilities for high-capacity optical communication and high-resolution imaging. Here, we experimentally demonstrate the generation and manipulation of frequency-converted Airy vortex beams through four-wave mixing in hot Rb vapor. A 780 nm vortex beam and a 776 nm two-dimensional Airy beam coherently participate in the four-wave mixing process, generating a 420 nm output beam that combines the orbital angular momentum of the vortex beam with the spatial structure of the Airy beam. The generated beam exhibits pronounced quasi-nondiffracting propagation and self-acceleration, with an intensity decay rate reduced by a factor of ∼1.88 relative to the input vortex beam and a transverse acceleration ∼1.84 times that of the input Airy beam. Moreover, both the intensity and the spatial profile of the generated beam are flexibly manipulated by varying the Rb vapor temperature and the pump beam power. This work provides a versatile approach for generating and controlling structured light at what we believe are new wavelengths, opening opportunities for short-wavelength optical manipulation and optical information processing.

Optics Express•Oct 5, 2026•0 citations

High-Dimensional Photonic Orbital-Angular-Momentum Frequency Interface

Xiaodong Qiu, Haoxu Guo, Yuan Ren +1 more

Frequency interface, namely, converting the colors of photons while retaining their other features, is indispensable for numerous applications ranging from up-conversion imaging to the multimode quantum network. However, limited by the nonuniform nonlinear frequency-conversion efficiency, constructing the frequency interface for high-dimensional spatial modes is still challenging. Here, to break this fundamental barrier, we construct a high-dimensional (HD) orbital-angular-momentum (OAM) frequency interface via conducting sum-frequency generation between HD OAM states to be converted and a radial structured pump. Specifically, by replacing the conventional Gaussian pump with an optimized coherent superposition of HD Laguerre-Gaussian radial modes (i.e., its azimuthal number is zero), we experimentally achieve the OAM frequency interface in nine dimensions with a record fidelity up to 90.38 %. Additionally, by increasing the number of radial modes, our scheme can be flexibly extended to higher dimension. Such a high-dimensional frequency interface could find potential applications in the high-capacity free-space optical communication and would also pave the way for constructing high-dimensional quantum networks.

Physical Review Applied•Apr 24, 2023•11 citations

High-efficiency telecom frequency conversion via a diamond-type atomic ensemble

Ling-Chun Chen, Meng-Yi Lin, Jiun‐Shiuan Shiu +3 more

Efficient telecom frequency conversion (TFC) in atomic systems is crucial for integrating atom-based quantum nodes into low-loss fiber-optic quantum networks. Here, we demonstrate high-efficiency TFC from 795 nm to 1367 nm in a cold 87Rb ensemble via diamond-type four-wave mixing (FWM), achieving conversion efficiencies of 66% and 80% at optical depths of 75 and 110, respectively, using a weak coherent probe field. These results surpass all previously reported values in atomic systems, enabled by a systematic investigation of the built-in V-type and cascade-type electromagnetically induced transparency spectra that guided the optimization of FWM conditions. Although this work employs coherent fields, our previous theoretical study has shown that quantum states can be preserved with high fidelity during the conversion process, highlighting the promise of diamond-type atomic FWM as a robust interface for long-distance quantum communication.

arXiv:2506.03957•Physical Review A•Jun 16, 2025•2 citations

Spatial Structure and Propagation of Vortex Four-Wave Mixing Signal

Ma Xiaoyu, Sang Suling, Zhao Guohui

Abstract The spatial structure and propagation of vortex Four-Wave mixing (FWM) generated in a cascade three-level atomic system when Laguerre-Gaussian (LG) beams are used as the incident pump fields are studied. Firstly, by solving the third-order density matrix elements in the steady state, the intensity expression of the vortex FWM signal is obtained. Next, their spatial image and phase during the propagation process are researched. It is shown that with the increase of propagation distance, its image of the intensity tends to a Gaussian beam, and the center of the spot gradually deviates from the original optical singularity. Furthermore, after superposing multiple topological charge (TC) numbers, the intensity and phase images present entirely different light spots at various positions. The TC number can rapidly increase the capacity of the signal for carrying information. This type of signal can be utilized in quantum communication and information, offering a scalable light source for high-dimensional quantum storage.

•Nov 21, 2025•0 citations
One of the major difficulties in realizing a high-dimensional frequency converter for conventional optical vortex (COV) stems from the difference in ring diameter of COV modes with different topological charge numbers l. Here, we implement a high-dimensional frequency convertor for perfect optical vortex (POV) modes with invariant size through the four-wave mixing (FWM) process by utilizing Bessel-Gaussian beams instead of Laguerre-Gaussian beams. The measured conversion efficiency from 1530 nm to 795 nm is independent of l at least in subspace of {-6,...,6}, and the achieved conversion fidelities for two-dimensional (2D) superposed POV states exceed 97%. We further realize the frequency conversion of 3D, 5D and 7D superposition states with fidelities as high as 96.70%, 89.16% and 88.68%, respectively. The reported scheme is implemented in hot atomic vapor, it's also compatible with the cold atomic system and may find applications in high-capacity and long-distance quantum communication.
One of the major difficulties in realizing a high-dimensional frequency converter for conventional optical vortex (COV) modes stems from the difference in ring diameter of the COV modes with different topological charge numbers l.Here, we implement a high-dimensional frequency converter for perfect optical vortex (POV) modes with invariant sizes by way of the four-wave mixing (FWM) process using Bessel-Gaussian beams instead of Laguerre-Gaussian beams.The measured conversion efficiency from 1530 to 795 nm is independent of l at least in subspace l ∈ f-6, : : : , 6g, and the achieved conversion fidelities for two-dimensional (2D) superposed POV states exceed 97%.We further realize the frequency conversion of 3D, 5D, and 7D superposition states with fidelities as high as 96.70%, 89.16%, and 88.68%, respectively.The proposed scheme is implemented in hot atomic vapor.It is also compatible with the cold atomic system and may find applications in high-capacity and long-distance quantum communication.
Optical vortex beams are profiled as helical wavefronts with a phase singularity carrying an orbital angular momentum (OAM) associated with their spatial distribution. The transverse intensity distribution of a conventional optical vortex has a strong dependence on the carried topological charge. However, perfect optical vortex (POV) beams have their transverse intensity distribution independent of their charge. Such “size-invariant” POV beams have found exciting applications in optical manipulation, imaging, and communication. In this paper, we investigate the use of POV modes in the efficient generation of high-dimensional quantum states of light. We generate heralded single photons carrying OAM using spontaneous parametric downconversion (SPDC) of POV beams. We show that the heralding efficiency of the SPDC single photons generated with a POV pump is greater than that with normal optical vortex beams. The dimensionality of the two-photon OAM states is increased with POV modes in the pump and projective measurements using Bessel–Gaussian vortex modes that give POV, instead of Laguerre–Gaussian modes.
Airy vortex beams, which integrate orbital angular momentum with diffraction-resistant and self-accelerating characteristics of Airy beams, offer unique capabilities for high-capacity optical communication and high-resolution imaging. Here, we experimentally demonstrate the generation and manipulation of frequency-converted Airy vortex beams through four-wave mixing in hot Rb vapor. A 780 nm vortex beam and a 776 nm two-dimensional Airy beam coherently participate in the four-wave mixing process, generating a 420 nm output beam that combines the orbital angular momentum of the vortex beam with the spatial structure of the Airy beam. The generated beam exhibits pronounced quasi-nondiffracting propagation and self-acceleration, with an intensity decay rate reduced by a factor of ∼1.88 relative to the input vortex beam and a transverse acceleration ∼1.84 times that of the input Airy beam. Moreover, both the intensity and the spatial profile of the generated beam are flexibly manipulated by varying the Rb vapor temperature and the pump beam power. This work provides a versatile approach for generating and controlling structured light at what we believe are new wavelengths, opening opportunities for short-wavelength optical manipulation and optical information processing.
Frequency interface, namely, converting the colors of photons while retaining their other features, is indispensable for numerous applications ranging from up-conversion imaging to the multimode quantum network. However, limited by the nonuniform nonlinear frequency-conversion efficiency, constructing the frequency interface for high-dimensional spatial modes is still challenging. Here, to break this fundamental barrier, we construct a high-dimensional (HD) orbital-angular-momentum (OAM) frequency interface via conducting sum-frequency generation between HD OAM states to be converted and a radial structured pump. Specifically, by replacing the conventional Gaussian pump with an optimized coherent superposition of HD Laguerre-Gaussian radial modes (i.e., its azimuthal number is zero), we experimentally achieve the OAM frequency interface in nine dimensions with a record fidelity up to 90.38 %. Additionally, by increasing the number of radial modes, our scheme can be flexibly extended to higher dimension. Such a high-dimensional frequency interface could find potential applications in the high-capacity free-space optical communication and would also pave the way for constructing high-dimensional quantum networks.
Efficient telecom frequency conversion (TFC) in atomic systems is crucial for integrating atom-based quantum nodes into low-loss fiber-optic quantum networks. Here, we demonstrate high-efficiency TFC from 795 nm to 1367 nm in a cold 87Rb ensemble via diamond-type four-wave mixing (FWM), achieving conversion efficiencies of 66% and 80% at optical depths of 75 and 110, respectively, using a weak coherent probe field. These results surpass all previously reported values in atomic systems, enabled by a systematic investigation of the built-in V-type and cascade-type electromagnetically induced transparency spectra that guided the optimization of FWM conditions. Although this work employs coherent fields, our previous theoretical study has shown that quantum states can be preserved with high fidelity during the conversion process, highlighting the promise of diamond-type atomic FWM as a robust interface for long-distance quantum communication.
Abstract The spatial structure and propagation of vortex Four-Wave mixing (FWM) generated in a cascade three-level atomic system when Laguerre-Gaussian (LG) beams are used as the incident pump fields are studied. Firstly, by solving the third-order density matrix elements in the steady state, the intensity expression of the vortex FWM signal is obtained. Next, their spatial image and phase during the propagation process are researched. It is shown that with the increase of propagation distance, its image of the intensity tends to a Gaussian beam, and the center of the spot gradually deviates from the original optical singularity. Furthermore, after superposing multiple topological charge (TC) numbers, the intensity and phase images present entirely different light spots at various positions. The TC number can rapidly increase the capacity of the signal for carrying information. This type of signal can be utilized in quantum communication and information, offering a scalable light source for high-dimensional quantum storage.