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arXiv:2301.06049

Bright, low-noise source of single photons at 780 nm with improved phase-matching in rubidium vapor

Omri Davidson, Yogev, Ohad, Eilon Poem, Ofer Firstenberg

Published Jan 15, 2023• 2 citations
arXivHTMLPDF

Abstract

Future optical quantum networks could benefit from single photons that couple well to atoms, for realizing, e.g., quantum memories and deterministic photonic gates. However, the efficient generation of such photons remains a difficult challenge. Recently, we demonstrated a bright multiplexed source of indistinguishable single photons with tunable GHz-bandwidth based on four-wave-mixing in rubidium vapor [Davidson et al. 2021 New J. Phys. 23 073050]. Here we report on an improved implementation of this photon source. The new implementation employs a frequency-detuning regime that is better phase matched, a spatial-alignment procedure using single-mode fibers, a different rubidium isotope, and higher vapor-cell transmission. Characterization of the source is performed using superconducting-nanowire detectors with higher detection efficiency and lower jitter. Our source produces single photons with detected heralding efficiency of over 20%, Hong-Ou-Mandel interference visibility of 88%, generation rate of over 100 kilo-counts per second, and signal-to-noise ratio greater than 100, making it suitable for quantum information processing with photons.

DOI
10.48550/arxiv.2301.06049

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Future optical quantum networks could benefit from single photons that couple well to atoms, for realizing, e.g., quantum memories and deterministic photonic gates. However, the efficient generation of such photons remains a difficult challenge. Recently, we demonstrated a bright multiplexed source of indistinguishable single photons with tunable GHz-bandwidth based on four-wave-mixing in rubidium vapor [Davidson et al. 2021 New J. Phys. 23 073050]. Here we report on an improved implementation of this photon source. The new implementation employs a frequency-detuning regime that is better phase matched, a spatial-alignment procedure using single-mode fibers, a different rubidium isotope, and higher vapor-cell transmission. Characterization of the source is performed using superconducting-nanowire detectors with higher detection efficiency and lower jitter. Our source produces single photons with detected heralding efficiency of over 20%, Hong-Ou-Mandel interference visibility of 88%, generation rate of over 100 kilo-counts per second, and signal-to-noise ratio greater than 100, making it suitable for quantum information processing with photons.
Abstract Narrowband single photons that couple well to atomic ensembles could prove essential for future quantum networks, but the efficient generation of such photons remains an outstanding challenge. We realize a spatially-multiplexed heralded source of single photons that are inherently compatible with the commonly employed D2 line of rubidium. Our source is based on four-wave mixing in hot rubidium vapor, requiring no laser cooling or optical cavities, and generates single photons with high rate and low noise. We use Hong–Ou–Mandel interference to verify the indistinguishability of the photons generated in two different (multiplexed) channels. We further demonstrate a five-fold tunability of the photons’ temporal width. The experimental results are well reproduced by a theoretical model.
The generation of entangled photon pairs which are compatible with quantum devices and standard telecommunication channels are critical for the development of long range fiber quantum networks. Aside from wavelength, bandwidth matching and high fidelity of produced pairs are necessary for high interfacing efficiency. High-rate, robust entanglement sources that satisfy all these conditions remain an outstanding experimental challenge. In this work, we study an entanglement source based on four-wave mixing in a diamond configuration in a warm rubidium vapor. We theoretically and experimentally investigate a new operating regime and demonstrate an entanglement source which produces highly non-degenerate 795795795 and 132413241324-nm photon pairs. With this source we are able to achieve in-fiber entangled pair generation rates greater than 107 /s10^7\, /s107/s, orders of magnitude higher than previously reported atomic sources. Additionally, given our source's native compatibility with telecom infrastructure and atomic systems, it is an important step towards scalable quantum networks.
Summary form only given. Hybrid quantum technologies seek to combine the advantages of two individual quantum architectures by transferring the information between the two systems. We want to benefit from the high mobility and ease of transmission of photons for quantum communication and exploit the excellent readout and storage capabilities of atomic qubits as a quantum memory, which is essential to build up quantum repeater networks for quantum data processing. Efficient interaction of photons with atoms requires a match of the photons spectral properties to those of the resonances of the atomic species. The atomic transition usually has a much narrower bandwidth than single photons generated by spontaneous parametric down-conversion (SPDC), the current gold standard of producing high-purity heralded single photons at flexible wavelengths. To develop hybrid quantum technologies therefore requires significantly reducing the single photon emission spectra to fulfill these requirements. The way we try to achieve this is by using an optical cavity to enhance the probability of creating the photons in the spectral and spatial resonator mode.We report 100% duty cycle generation of sub-MHz single photon pairs at the Rubidium D1 line using cavityenhanced spontaneous parametric down-conversion [3]. The double exponential decay of the temporal intensity cross-correlation function exhibits a bandwidth of 666 ± 16 kHz for the single photons, an order of magnitude below the natural linewidth of the target transition. This is, to our knowledge, the narrowest bandwidth of single photons from SPDC to date. A new method of placing a half-wave plate inside the cavity helps to achieve triple resonance between pump, signal and idler photon, reducing the bandwidth and simplifying the locking scheme. Additionally, stabilisation of the cavity to the pump frequency enables the 100% duty cycle. The quantum nature of the source is confirmed by the idler-triggered second-order autocorrelation function at τ = 0 to be g(2) s,s (0) = 0.016 ± 0.002 for a heralding rate of 5 kHz and antibunching below 0.5 is observed up to heralding rates of 250 kHz [3]. The high purity of the source is matched by high indistinguishability of the photons demonstrated in a Hong-Ou-Mandel (HOM) interference experiment with a visibility V = 96.5 ± 0.5 %. Additionally, the modelocked two-photon state of the generated pairs leads to revivals of the HOM dip. We observe these revivals up to 100 m path difference between signal and idler photon, independently proofing the long coherence length of our photons.
The generation of entangled photon pairs, which are compatible with quantum devices and standard telecommunication channels are critical for the development of long-range fiber quantum networks. Aside from wavelength, bandwidth matching, and high fidelity of produced pairs are necessary for high interfacing efficiency. High-rate, robust entanglement sources that satisfy all these conditions remain an outstanding experimental challenge. In this work, we study an entanglement source based on four-wave mixing in a diamond configuration in a warm rubidium vapor. We theoretically and experimentally investigate an alternative operating regime and demonstrate an entanglement source, which produces highly nondegenerate 795- and 1324-nm photon pairs. With this source we are able to achieve in-fiber pair-generation rates greater than 107/s{10}^{7}/\mathrm{s}107/s, orders of magnitude higher than previously reported atomic entanglement sources. Additionally, given our source's native compatibility with telecom infrastructure and atomic systems, it is a step towards scalable quantum networks.
Deterministic generation of single photons is essential for many quantum information technologies. A bulk optical nonlinearity emitting a photon pair, where the measurement of one of the photons heralds the presence of the other, is commonly used with the caveat that the single-photon emission rate is constrained due to a trade-off between multiphoton events and pair emission rate. Using an efficient and low noise photon-number-resolving superconducting nanowire detector we herald, in real time, a single photon at telecommunication wavelength. We perform a second-order photon correlation g2(0){g}^{2}(0)g2(0) measurement of the signal mode conditioned on the measured photon number of the idler mode for various pump powers and demonstrate an improvement of a heralded single-photon source. We develop an analytical model using a phase-space formalism that encompasses all multiphoton effects and relevant imperfections, such as loss and multiple Schmidt modes. We perform a maximum-likelihood fit to test the agreement of the model to the data and extract the best-fit mean photon number $\ensuremath{\mu}$ of the pair source for each pump power. A maximum reduction of $0.118\ifmmode\pm\else\textpm\fi{}0.012$ in the photon g2(0){g}^{2}(0)g2(0) correlation function at $\ensuremath{\mu}=0.327\ifmmode\pm\else\textpm\fi{}0.007$ is obtained, indicating a strong suppression of multiphoton emissions. For a fixed ${g}^{2}(0)=7\ifmmode\times\else\texttimes\fi{}{10}^{\ensuremath{-}3}$, we increase the single pair generation probability by 25%. Our experiment, built using fiber-coupled and off-the-shelf components, delineates a path to engineering ideal sources of single photons.
Quantum memories matched to single photon sources will form an important cornerstone of future quantum network technology. We demonstrate such a memory in warm Rb vapor with on-demand storage and retrieval, based on electromagnetically induced transparency. With an acceptance bandwidth of δf=0.66 GHz, the memory is suitable for single photons emitted by semiconductor quantum dots. In this regime, vapor cell memories offer an excellent compromise between storage efficiency, storage time, noise level, and experimental complexity, and atomic collisions have negligible influence on the optical coherences. Operation of the memory is demonstrated using attenuated laser pulses on the single photon level. For a 50 ns storage time, we measure η_{e2e}^{50 ns}=3.4(3)% end-to-end efficiency of the fiber-coupled memory, with a total intrinsic efficiency η_{int}=17(3)%. Straightforward technological improvements can boost the end-to-end-efficiency to η_{e2e}≈35%; beyond that, increasing the optical depth and exploiting the Zeeman substructure of the atoms will allow such a memory to approach near unity efficiency. In the present memory, the unconditional read-out noise level of 9×10^{-3} photons is dominated by atomic fluorescence, and for input pulses containing on average μ_{1}=0.27(4) photons, the signal to noise level would be unity.