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Conference on Lasers and Electro-Optics Europe & European Quantum Electronics Conference (CLEO/Europe-EQEC)

Sub-megahertz linewidth single photon source suitable for quantum memories

Markus Rambach, W. Y. Sarah Lau, Aleksandrina Nikolova, Till J. Weinhold, Andrew G. White

Published Jun 1, 2017• 1 citation
Publisher

Abstract

Summary form only given. Hybrid quantum technologies seek to combine the advantages of two individual quantum architectures by transferring the information between the two systems. We want to benefit from the high mobility and ease of transmission of photons for quantum communication and exploit the excellent readout and storage capabilities of atomic qubits as a quantum memory, which is essential to build up quantum repeater networks for quantum data processing. Efficient interaction of photons with atoms requires a match of the photons spectral properties to those of the resonances of the atomic species. The atomic transition usually has a much narrower bandwidth than single photons generated by spontaneous parametric down-conversion (SPDC), the current gold standard of producing high-purity heralded single photons at flexible wavelengths. To develop hybrid quantum technologies therefore requires significantly reducing the single photon emission spectra to fulfill these requirements. The way we try to achieve this is by using an optical cavity to enhance the probability of creating the photons in the spectral and spatial resonator mode.We report 100% duty cycle generation of sub-MHz single photon pairs at the Rubidium D1 line using cavityenhanced spontaneous parametric down-conversion [3]. The double exponential decay of the temporal intensity cross-correlation function exhibits a bandwidth of 666 ± 16 kHz for the single photons, an order of magnitude below the natural linewidth of the target transition. This is, to our knowledge, the narrowest bandwidth of single photons from SPDC to date. A new method of placing a half-wave plate inside the cavity helps to achieve triple resonance between pump, signal and idler photon, reducing the bandwidth and simplifying the locking scheme. Additionally, stabilisation of the cavity to the pump frequency enables the 100% duty cycle. The quantum nature of the source is confirmed by the idler-triggered second-order autocorrelation function at τ = 0 to be g(2) s,s (0) = 0.016 ± 0.002 for a heralding rate of 5 kHz and antibunching below 0.5 is observed up to heralding rates of 250 kHz [3]. The high purity of the source is matched by high indistinguishability of the photons demonstrated in a Hong-Ou-Mandel (HOM) interference experiment with a visibility V = 96.5 ± 0.5 %. Additionally, the modelocked two-photon state of the generated pairs leads to revivals of the HOM dip. We observe these revivals up to 100 m path difference between signal and idler photon, independently proofing the long coherence length of our photons.

DOI
10.1109/cleoe-eqec.2017.8087343

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We report 100% duty cycle generation of sub-MHz single photon pairs at the rubidium D1 line using cavity-enhanced spontaneous parametric downconversion. The temporal intensity cross correlation function exhibits a bandwidth of 666±16 kHz for the single photons, an order of magnitude below the natural linewidth of the target transition. A half-wave plate inside our cavity helps to achieve triple resonance between pump, signal, and idler photon, reducing the bandwidth and simplifying the locking scheme. Additionally, stabilisation of the cavity to the pump frequency enables the 100% duty cycle. The quantum nature of the source is confirmed by the idler-triggered second-order autocorrelation function at τ=0 to be gs,s(2)(0)= 0.016±0.002 for a heralding rate of 5 kHz. The generated photons are well-suited for storage in quantum memory schemes with sub-natural linewidths, such as gradient echo memories.

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Summary form only given. Hybrid quantum technologies seek to combine the advantages of two individual quantum architectures by transferring the information between the two systems. We want to benefit from the high mobility and ease of transmission of photons for quantum communication and exploit the excellent readout and storage capabilities of atomic qubits as a quantum memory, which is essential to build up quantum repeater networks for quantum data processing. Efficient interaction of photons with atoms requires a match of the photons spectral properties to those of the resonances of the atomic species. The atomic transition usually has a much narrower bandwidth than single photons generated by spontaneous parametric down-conversion (SPDC), the current gold standard of producing high-purity heralded single photons at flexible wavelengths. To develop hybrid quantum technologies therefore requires significantly reducing the single photon emission spectra to fulfill these requirements. The way we try to achieve this is by using an optical cavity to enhance the probability of creating the photons in the spectral and spatial resonator mode.We report 100% duty cycle generation of sub-MHz single photon pairs at the Rubidium D1 line using cavityenhanced spontaneous parametric down-conversion [3]. The double exponential decay of the temporal intensity cross-correlation function exhibits a bandwidth of 666 ± 16 kHz for the single photons, an order of magnitude below the natural linewidth of the target transition. This is, to our knowledge, the narrowest bandwidth of single photons from SPDC to date. A new method of placing a half-wave plate inside the cavity helps to achieve triple resonance between pump, signal and idler photon, reducing the bandwidth and simplifying the locking scheme. Additionally, stabilisation of the cavity to the pump frequency enables the 100% duty cycle. The quantum nature of the source is confirmed by the idler-triggered second-order autocorrelation function at τ = 0 to be g(2) s,s (0) = 0.016 ± 0.002 for a heralding rate of 5 kHz and antibunching below 0.5 is observed up to heralding rates of 250 kHz [3]. The high purity of the source is matched by high indistinguishability of the photons demonstrated in a Hong-Ou-Mandel (HOM) interference experiment with a visibility V = 96.5 ± 0.5 %. Additionally, the modelocked two-photon state of the generated pairs leads to revivals of the HOM dip. We observe these revivals up to 100 m path difference between signal and idler photon, independently proofing the long coherence length of our photons.
We report 100% duty cycle generation of sub-MHz single photon pairs at the rubidium D1 line using cavity-enhanced spontaneous parametric downconversion. The temporal intensity cross correlation function exhibits a bandwidth of 666±16 kHz for the single photons, an order of magnitude below the natural linewidth of the target transition. A half-wave plate inside our cavity helps to achieve triple resonance between pump, signal, and idler photon, reducing the bandwidth and simplifying the locking scheme. Additionally, stabilisation of the cavity to the pump frequency enables the 100% duty cycle. The quantum nature of the source is confirmed by the idler-triggered second-order autocorrelation function at τ=0 to be gs,s(2)(0)= 0.016±0.002 for a heralding rate of 5 kHz. The generated photons are well-suited for storage in quantum memory schemes with sub-natural linewidths, such as gradient echo memories.
Photons as flying qubits are ideal carriers of quantum information. However, efficient quantum interfaces which transfer flying into stationary qubits and vice versa are needed to realize complex quantum networks. Stationary qubit systems (atoms, ions, or solid state implementations) couple to photons via characteristic optical transitions. In order to establish key quantum operations, such as coherent photon storage, entanglement swapping, etc., high-quality photons with a tailored spectral, spatial, and temporal mode are needed. One way to generate these photons is to use the stationary qubit systems themselves. Another approach which does not impose limitations in terms of the photon’s wavelength or bandwidth relies on all-optical single photon sources. An example is spontaneous parametric down conversion (SPDC) inside an optical cavity with well-defined linewidth. In SPDC, a pump photon incident on a nonlinear medium is split into two photons of lower energy that are often referred to as signal and idler. Resonating the fluorescent fields, the setup becomes an optical parametric oscillator (OPO) far below the threshold. The usually THz broad emission spectrum of SPDC then follows the Airy function of the resonator. The spectral bandwidth of the generated photons can easily reach values of several MHz, which is comparable to atom resonance linewidths. By introducing additional losses or simply changing the cavity mirror reflectivities the bandwidth is tunable up to several 100 MHz. This is comparable to the bandwidth of single photons generated by e.g. quantum dots.
Cavity-enhanced spontaneous parametric down-conversion (SPDC) can be used to implement heralded single-photon sources with narrow bandwidth down to tens of megahertz, thus compatible with atom-based quantum memories. In this work, we propose and study the cavities that are either singly resonant at the frequency of only one of the generated photons or doubly resonant at the frequency of one generated photon and for the pump field. We derive analytical expressions for the generation rate and the spectral brightness as a function of the main structure parameters. Our analysis shows that by exploiting counterpropagating SPDC inside a cavity with properly designed distributed Bragg reflectors, pure narrow-band heralded single photons can be generated. In particular, when a pulsed pump illuminates a 1-mm-long singly resonant cavity, the bandwidth of the resonant and the nonresonant photons will be 120 MHz and 5.7 GHz, respectively, with heralded single-photon purity as high as 0.993. Due to its small absorption probability inside the cavity, the heralding efficiency can approach unity if the nonresonant partner is used as a heralded single photon. Finally, we also show that continuous-wave excitation of a 1-cm-long cavity resonant for the pump and copropagating fields can provide photon pairs in a narrow bandwidth of 10 MHz with spectral brightness as high as $2\ifmmode\times\else\texttimes\fi{}{10}^{6}$ $({\text{s}\phantom{\rule{4.pt}{0ex}}\text{mW}\phantom{\rule{4.pt}{0ex}}\text{MHz})}^{\ensuremath{-}1}$. This source can efficiently couple with quantum memories and can find applications in quantum information processing and communication.
A single-photon source with narrow bandwidth, high purity, and large brightness can efficiently interact with material qubits strongly coupled to an optical microcavity for quantum information processing. Here, we experimentally demonstrate a degenerate doubly resonant single-photon source at 852 nm by the cavity-enhanced spontaneous parametric down-conversion process with a 100% duty cycle of generation. The single photon source possesses both high purity with a second-order correlation g (2) (0) = 0.021 and narrow linewidth with Δνsp = (800 ± 13) kHz. The single-photon source is compatible with the cesium atom D2 line and can be used for cesium-based quantum information processing.
Abstract In long-distance quantum communication using quantum repeaters with quantum memories, entangled photons at telecommunication wavelengths that can be coupled to quantum memory with high efficiency are required. Typically, entangled photons are generated via spontaneous parametric down conversion (SPDC). However, the phase-matching bandwidth of SPDC is more than 100 GHz, which is much broader than the bandwidth of a Pr 3+ :Y 2 SiO 5 quantum memory (with overall bandwidth of ∼10 GHz while the bandwidth of each frequency channel is ∼10 MHz) suitable for frequency-multiplexed quantum repeaters. In this study, nondegenerate SPDC (1550 nm and 995 nm) inside an optical cavity is used to obtain a narrow linewidth and cluster width of SPDC to match the Pr 3+ :Y 2 SiO 5 bandwidth. We also developed a cavity control mechanism that can fulfill the doubly resonant condition. The developed two-photon source can maximize the coupling efficiency with Pr 3+ :Y 2 SiO 5 by introducing wavelength conversion and is promising for use in a quantum repeater.
Abstract We demonstrate an ultrabright, narrow-band and frequency-tunable photon-pair source based on cavity-enhanced spontaneous parametric down conversion (SPDC) which is compatible with atomic transition of rubidium D 2 -line (780 nm) or cesium D 2 -line (852 nm). With the pump beam alternating between a high and a low power phase, the output is switching between the optical parametric oscillator (OPO) and photon-pair generation mode. We utilize the OPO output light to lock the cavity length to maintain the double resonances of signal and idler, as well as to lock the signal frequency to cesium atomic transition. With a type-II phase matching and a double-passed pump scheme such that the cluster frequency spacing is larger than the SPDC bandwidth, the photon-pair output is in a nearly single-mode operation as confirmed by a scanning Fabry–Perot interferometer with its output detected by a photomultiplier. The achieved generation and detection rates are 7.24 × 10 5 and 6142 s −1 mW −1 , respectively. The correlation time of the photon pair is 21.6(2.2) ns, corresponding to a bandwidth of 2 π × 6.6(6) MHz. The spectral brightness is 1.06 × 10 5 s −1 mW −1 MHz −1 . This is a relatively high value under a single-mode operation with the cavity-SPDC scheme. The generated single photons can be readily used in experiments related to atomic quantum memories.