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arXiv:2301.04411 · Physical Review Applied

Controllable Tunneling of Single Flux Quanta Mediated by Quantum Phase Slip in Disordered Superconducting Loops

Jamie Potter, J. C. Fenton, Paul A. Warburton

Published Feb 1, 2023• 5 citations
arXivHTMLPDF

Abstract

Quantum phase slip (QPS) is the exact dual to the well-known Josephson effect. Although there are numerous proposals for applications of QPS devices, experimental work to develop these remains in the relatively early stages. Significant barriers to exploiting QPS nanowires for useful technologies still exist, such as establishing robust nanowire-fabrication methods that allow coupling to low-loss circuits, and demonstrating control over the QPS process with an experimenter-controlled external bias. Here we report experiments that show that both of these barriers have been overcome. We present measurements at 300 mK of $\mathrm{Nb}\mathrm{N}$ coplanar-waveguide (CPW) resonators embedded with nanowires fabricated using a neon focused ion beam. The internal quality factor exceeds $2\ifmmode\times\else\texttimes\fi{}{10}^{4}$---significantly higher than previously reported in comparable experiments. The resonator frequency tunes periodically with an applied magnetic field, revealing tunneling of the order parameter that always occurs at half-integer values of the applied flux. In contrast to previous studies of single QPS, the order-parameter tunneling is shown to be adiabatic, demonstrating improved control over energy dissipation in nanowire QPS circuits. Our results highlight a promising pathway towards realizing low-loss nanowire-based QPS devices.

DOI
10.1103/physrevapplied.19.024002

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Quantum phase slips (QPS) or the macroscopic quantum tunneling (MQT) of a nanowire’s order parameter through an activation energy barrier have remained the subject of intense debate for many years. They are expected to occur at low enough temperature where thermally activated phase slips (TAPS) have been frozen out in analogy with Josephson junctions where the macroscopic tunneling of phase at low temperatures has been conclusively experimentally demonstrated. We address this question by following a similar experimental strategy to that employed for establishing MQT in JJs. By measuring switching current distributions, we can probe the phase slip rate and determine if it corresponds to thermal activation or quantum tunneling. Having established that the behavior we see is consistent with being in the quantum regime, we can alter properties of the nanowires and see if the response is consistent with the expectations of the quantum model. To do this we employ an in-situ modification technique using high bias voltage pulses. Using these pulses, we can change resistance, critical temperature, critical current and morphology of the nanowire. We can also change the shunting capacitance of the nanowire by altering the photolithography step used to create the nanowires electrodes. The resulting response of the nanowires agrees well with being in the quantum tunneling dominated regime. An interesting side benefit of the pulsing technique is that we can exactly set the nanowires switching current to a desired value. This may be instrumental in the development of superconducting nanowire qubits.
Quantum circuits based on superconducting nanowires have recently made an impact in the development of devices harnessing phase slip, superinductance, and Josephson effects. Exploiting this rich physics is difficult, though, due to fabrication-induced, parasitic two-level systems, which cause high levels of loss and decoherence. Using a focused beam of neon ions, the authors embed superconducting nanowires into coplanar waveguide resonators and realize much lower losses than in previous devices. This achievement suggests excellent prospects for this class of circuitry.
In thin superconducting wires, phase-slip by thermal activation near the critical temperature is a well-known effect. It has recently become clear that phase-slip by quantum tunnelling through the energy barrier can also have a significant rate at low temperatures. In this paper, it is suggested that quantum phase-slip can be used to realize a superconducting quantum bit without Josephson junctions. A loop containing very thin nanofabricated wire is biased with an externally applied magnetic flux of half a flux quantum, resulting in two states with opposite circulating current and equal energy. Quantum phase-slip should provide coherent coupling between these two macroscopic states. Numbers are given for a wire of amorphous niobium-silicon that can be fabricated with advanced electron beam lithography.
Abstract Quantum phase slip (QPS) is an important effect that occurs in one-dimensional (1D) or quasi-1D superconducting (SC) materials. Due to the extremely high requirements on the uniformity and quality of SC nanowires, it is currently very challenging to obtain repeatable and controllable QPS devices. Here, we report a systematic study of the QPS effect in NbN SC nanowires. High-quality NbN nanowires with different widths are fabricated by combining the processes of photo-lithography, electron beam lithography, and inductively coupled plasma etching. It is found that the electrical transport of the nanowires showed a systematic variation with the wire width, and a clear evolution from single to multiple QPS events with the decrease in wire width is uncovered at low temperatures. Based on these experimental results, the phase diagram reflecting the evolution of the physical states of the nanowires with wire width and temperature is obtained. In addition, we observed the features of the critical voltage, which is a characteristic of the occurrence of coherent QPS (cQPS), in samples with a width of 36 nm in the multiple QPS region. It is worth noting that this cQPS behavior was detected in a non-high-impedance environment.
We present a detailed report of microwave irradiation of ultranarrow superconducting nanowires. In our nanofabricated circuits containing a superconducting NbSi nanowire, a dc blockade of current flow was observed at low temperatures below a critical voltage Vc{V}_{\mathrm{c}}Vc​, a strong indicator of the existence of quantum phase-slip (QPS) in the nanowire. We describe the results of applying microwaves to these samples, using a range of frequencies and both continuous-wave and pulsed drive, in order to search for dual Shapiro steps which would constitute an unambiguous demonstration of quantum phase-slip. We observed no steps, and our subsequent thermal analysis suggests that the electron temperature in the series CrO resistors was significantly elevated above the substrate temperature, resulting in sufficient Johnson noise to wash out the steps. To understand the system and inform future work, we have constructed a numerical model of the dynamics of the circuit for dc and ac bias (both continuous-wave and pulsed drive signals) in the presence of Johnson noise. Using this model, we outline important design considerations for device and measurement parameters which should be used in any future experiment to enable the observation of dual Shapiro steps at experimentally accessible temperatures and, thus, lead to the development of a QPS-based quantum current standard.