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arXiv:cond-mat/0508440 · New Journal of Physics

Phase-slip flux qubits

Johan E. Mooij, C. J. P. M. Harmans

Published Oct 11, 2005• 185 citations
arXivHTMLPDF

Abstract

In thin superconducting wires, phase-slip by thermal activation near the critical temperature is a well-known effect. It has recently become clear that phase-slip by quantum tunnelling through the energy barrier can also have a significant rate at low temperatures. In this paper, it is suggested that quantum phase-slip can be used to realize a superconducting quantum bit without Josephson junctions. A loop containing very thin nanofabricated wire is biased with an externally applied magnetic flux of half a flux quantum, resulting in two states with opposite circulating current and equal energy. Quantum phase-slip should provide coherent coupling between these two macroscopic states. Numbers are given for a wire of amorphous niobium-silicon that can be fabricated with advanced electron beam lithography.

DOI
10.1088/1367-2630/7/1/219

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In thin superconducting wires, phase-slip by thermal activation near the critical temperature is a well-known effect. It has recently become clear that phase-slip by quantum tunnelling through the energy barrier can also have a significant rate at low temperatures. In this paper, it is suggested that quantum phase-slip can be used to realize a superconducting quantum bit without Josephson junctions. A loop containing very thin nanofabricated wire is biased with an externally applied magnetic flux of half a flux quantum, resulting in two states with opposite circulating current and equal energy. Quantum phase-slip should provide coherent coupling between these two macroscopic states. Numbers are given for a wire of amorphous niobium-silicon that can be fabricated with advanced electron beam lithography.
Abstract Superconducting circuits represent a versatile playground to explore novel quantum phenomena and a platform to realize quantum bits (qubits). Superconducting qubits hinge on the coherent tunneling of Cooper pairs across the insulating barrier of a Josephson junction. This qubit implementation is, however, plagued with the variability of the fabricated junction, along with the need for magnetic tunability of the qubit transition frequency. Alternatively, a dual to the Josephson effect—referred to as quantum phase slips—allows for a coherent coupling of flux states and has been used to build phase-slip qubits. In this paper, we propose coupling flux states of a superconducting ring using a bias voltage. By solving the time-dependent Ginzburg–Landau equations, we demonstrate that the bias voltage locally suppresses the density of Cooper pairs, thereby forming a weak link where phase slips occur. Moreover, we show that a voltage-biased superconducting ring serves as an electrically-controlled magnetic memory. The work presented in this paper is an important step towards realizing electrically-tunable superconducting devices, such as qubits and SQUIDs.
Abstract Quantum phase slips represent a coherent mechanism to couple flux states of a superconducting loop. Since their first direct observation, there have been substantial developments in building charge-insensitive quantum phase-slip circuits. At the heart of these devices is a weak link, often a nanowire, interrupting a superconducting loop. Owing to the very small cross-sectional area of such a nanowire, quantum phase slip rates in the gigahertz range can be achieved. Instead, here we present the use of a bias voltage across a superconducting loop to electrostatically induce a weak link, thereby amplifying the rate of quantum phase slips without physically interrupting the loop. Our simulations reveal that the bias voltage modulates the free energy barrier between subsequent flux states in a very controllable fashion, providing a route towards a phase-slip flux qubit with a broadly tunable transition frequency.
Quantum phase slips (QPS) or the macroscopic quantum tunneling (MQT) of a nanowire’s order parameter through an activation energy barrier have remained the subject of intense debate for many years. They are expected to occur at low enough temperature where thermally activated phase slips (TAPS) have been frozen out in analogy with Josephson junctions where the macroscopic tunneling of phase at low temperatures has been conclusively experimentally demonstrated. We address this question by following a similar experimental strategy to that employed for establishing MQT in JJs. By measuring switching current distributions, we can probe the phase slip rate and determine if it corresponds to thermal activation or quantum tunneling. Having established that the behavior we see is consistent with being in the quantum regime, we can alter properties of the nanowires and see if the response is consistent with the expectations of the quantum model. To do this we employ an in-situ modification technique using high bias voltage pulses. Using these pulses, we can change resistance, critical temperature, critical current and morphology of the nanowire. We can also change the shunting capacitance of the nanowire by altering the photolithography step used to create the nanowires electrodes. The resulting response of the nanowires agrees well with being in the quantum tunneling dominated regime. An interesting side benefit of the pulsing technique is that we can exactly set the nanowires switching current to a desired value. This may be instrumental in the development of superconducting nanowire qubits.
We study quantum phase-slip (QPS) processes in a superconducting ring containing NNN Josephson junctions and threaded by an external static magnetic flux ${\ensuremath{\Phi}}_{B}$. In such a system, a QPS consists of a quantum tunneling event connecting two distinct classical states of the phases with different persistent currents [Matveev et al., Phys. Rev. Lett. 89, 096802 (2002)]. When the Josephson coupling energy EJ{E}_{J}EJ​ of the junctions is larger than the charging energy EC=e2/2C{E}_{C}={e}^{2}/2CEC​=e2/2C, where CCC is the junction capacitance, the quantum amplitude for the QPS process is exponentially small in the ratio EJ/EC{E}_{J}/{E}_{C}EJ​/EC​. At given magnetic flux, each QPS can be described as the tunneling of the phase difference of a single junction of almost $2\ensuremath{\pi}$, accompanied by a small harmonic displacement of the phase difference of the other $N\ensuremath{-}1$ junctions. As a consequence, the total QPS amplitude ${\ensuremath{\nu}}_{\mathrm{ring}}$ is a global property of the ring. Here, we study the dependence of ${\ensuremath{\nu}}_{\mathrm{ring}}$ on the ring size NNN, taking into account the effect of a finite capacitance C0{C}_{0}C0​ to ground, which leads to the appearance of low-frequency dispersive modes. Josephson and charging effects compete and lead to a nonmonotonic dependence of the ring's critical current on NNN. For $N\ensuremath{\rightarrow}\ensuremath{\infty}$, the system converges either towards a superconducting or an insulating state, depending on the ratio between the charging energy E0=e2/2C0{E}_{0}={e}^{2}/2{C}_{0}E0​=e2/2C0​ and the Josephson coupling energy EJ{E}_{J}EJ​.
Superconducting circuits combine zero electrical resistance with macroscopic quantum coherence, making them a versatile platform for both fundamental studies and technological applications. Modern thin-film deposition and lithography allow precise control over geometry, material composition, and dimensional scales, enabling the fabrication of complex superconducting structures with tailored properties. These capabilities give access to phenomena not achievable with conventional electronic components, establishing superconducting circuits as a unique tool for exploring quantum physics and developing devices with unique functionalities. In superconducting rings, macroscopic quantum coherence manifests as discrete circulating currents. Fluxoid quantization restricts these currents to discrete winding states. Transitions between winding states occur via phase-slip events. A phase slip event requires overcoming an energy barrier, which can be crossed either through thermal activation, resulting in thermally activated phase slips (TAPS), or via quantum tunneling, resulting in quantum phase slips (QPS) that have no classical analogue. Both processes depend sensitively on temperature, loop geometry, material properties, and the intrinsic properties of the superconductor. Embedding weak links or nanowires in a superconducting ring provides localized regions where phase slips preferentially occur, enabling controlled TAPS and QPS dynamics. When the QPS rate becomes sufficiently high, coherent tunneling between neighboring winding states generates an energy splitting, forming the basis of qubit states. The discrete winding states can thus be exploited for device applications: serving as robust memory elements when the energy barrier is high and phase slips are rare and well controlled, and as qubits when coherent quantum phase slips allow the system to occupy superpositions of distinct winding states, marking the transition from a classical bit to a quantum bit. Phase-slip dynamics in superconducting rings have traditionally been studied using switching-current measurements, in which the bias current is ramped until the ring or nanowire becomes resistive. While this approach provides statistical information about phase-slip rates, it is inherently dissipative and cannot detect events that do not drive the system in the normal state, leaving many phase slips hidden and preventing their unambiguous classification by origin or rate.This thesis develops a non-invasive, radio-frequency resonator-based platform for studying phase-slip dynamics in superconducting rings. Building on magnetooptical imaging of flux penetration in superconducting resonators, we first established methods to apply a local magnetic field to a loop without perturbing the resonator and couple it to the resonator, linking changes in circulating currents to shifts in the resonance frequency. This enabled continuous, timeresolved detection of individual phase-slip events on microsecond-to-nanosecond timescales. Using this platform, we systematically investigated how loop geometry, weak-link properties, kinetic inductance, and temperature govern phase-slip rates and dynamics. Deterministic control of discrete winding states in high-kinetic-inductance aluminum loops, our chosen material platform, was demonstrated, realizing a superconducting memory based on fluxoid quantization. By progressively reducing loop dimensions and introducing weak links, we observed quantum phase-slip events at millikelvin temperatures, providing the first experimental signatures of coherent tunneling between winding states, a first step toward realizing phase-slip-based qubits. Collectively, these results establish a robust experimental pathway from conventional DC measurements to non-invasive RF probing, provide a framework for controlled studies of superconducting phase-slip dynamics, and open the door to exploring and utilizing coherent phase slips in circuit-QED-compatible architectures with device geometries that are simple and easy to fabricate.
Superconducting order in a sufficiently narrow and infinitely long wire is destroyed at zero temperature by quantum fluctuations, which induce $2\ensuremath{\pi}$ slips of the phase of the order parameter. However, in a finite-length wire, coherent quantum phase slips would manifest themselves simply as shifts of energy levels in the excitation spectrum of an electrical circuit incorporating this wire. The higher the phase slips' probability amplitude, the larger are the shifts. Phase slips occurring at different locations along the wire interfere with each other. Due to the Aharonov-Casher effect, the resulting full amplitude of a phase slip depends on the offset charges surrounding the wire. Slow temporal fluctuations of the offset charges make the phase-slip amplitudes random functions of time, and therefore turn energy level shifts into linewidths. We experimentally observed this effect on a long Josephson junction array acting as a ``slippery'' wire. The slip-induced linewidths, despite being only of order 100kHz100\phantom{\rule{0.28em}{0ex}}\phantom{\rule{4pt}{0ex}}\mathrm{kHz}100kHz, were resolved from the flux-dependent dephasing of the fluxonium qubit.