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arXiv:2212.12350 · Physical Review A

NMR investigations of dynamical tunneling in spin systems

V. R. Krithika, M. S. Santhanam, T. S. Mahesh

Published Sep 8, 2023• 5 citations

Abstract

In the usual quantum tunneling, a low-energy quantum particle penetrates across a physical barrier of higher potential energy, by traversing a classically forbidden region, and finally escapes into another region. In an analogous scenario, a classical particle inside a closed regular region in the phase space is dynamically bound from escaping to other regions of the phase space. Here, the physical potential barrier is replaced by dynamical barriers which separate different regions of the phase space. However, in the quantum regime, the system can overcome such dynamical barriers and escape through them, giving rise to dynamical tunneling. In chaotic Hamiltonian systems, dynamical tunneling refers to quantum tunneling between states whose classical limits correspond to symmetry-related regular regions separated by a chaotic zone between which any classical transport is prohibited. Here, an experimental realization of dynamical tunneling in spin systems is reported using nuclear magnetic resonance (NMR) architecture. In particular, dynamical tunneling in quantum kicked tops of spin-1 and spin-3/2 systems using two- and three-qubit NMR registers is investigated. By extracting time-dependent expectation values of the angular momentum operator components, size-dependent tunneling behavior for various initial states is systematically investigated. Further, by monitoring the adverse effects of dephasing noise on the tunneling oscillations, we assert the importance of quantum coherence in enabling dynamical tunneling.

DOI: 10.1103/physreva.108.032207

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Since the early days of quantum mechanics, tunneling has been recognized as one of the hallmarks of the wave character of microscopic physics. The possibility of a quantum particle to penetrate an energetic barrier represents certainly one of the most spectacular implications of quantum theory and has led to various applications in nuclear, atomic, and molecular physics as well as in mesoscopic science. Typical scenarios in which tunneling manifests are the escape route of a quantum particle from a quasibounded region, the transition between two or more symmetry-related, but classically disconnected wells (which we shall focus on in the following), as well as scattering or transport through potential barriers. The spectrum of scenarios becomes even richer when the concept of tunneling is generalized to any kind of classically forbidden transitions in phase space, that is, to transitions that are not necessarily inhibited by static potential barriers but by some other constraints of the underlying classical dynamics (such as integrals of motion). Such “dynamical tunneling” processes arise frequently in molecular systems [1] and were realized with cold atoms propagating in periodically modulated optical lattices [2-4]. Moreover, the electromagnetic analog of dynamical tunneling was also obtained with microwaves in billiards [5].

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Tunneling as a quantum mechanical effect takes place in a classically forbidden region between two regions of classically allowed motion. While the term “dynamical tunneling” typically refers to tunneling of quantum states across dynamical barriers in classical phase space [1], the original problem simply intended tunneling across a potential barrier. Both types of tunneling are addressed in this chapter, with major focus on situations in which external forces make the studied systems intrinsically time-dependent and allow for a dynamical control of tunneling through potential barriers or across band gaps which are dynamically explored by the system.

Quantum chaotic kicked top model is implemented experimentally in a two-qubit system comprising of a pair of spin-1/2 nuclei using nuclear magnetic resonance techniques. The essential nonlinear interaction was realized using indirect spin-spin coupling, while the linear kicks were realized using radio-frequency pulses. After a variable number of kicks, quantum state tomography was employed to reconstruct the single-qubit reduced density matrices, using which we could extract von Neumann entropies and Husimi distributions. These measures enabled the study of correspondence with classical phase space as well as probing distinct features of quantum chaos, such as symmetries and temporal periodicity in the two-qubit kicked top.