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arXiv:2212.08508 · Entropy

Coarse-Grained Effective Hamiltonian via the Magnus Expansion for a Three-Level System

Nicola Macrì, Luigi Giannelli, Elisabetta Paladino, G. Falci

Published Jan 27, 2023• 3 citations
arXivHTMLPDF

Abstract

Quantum state processing is one of the main tools of quantum technologies. While real systems are complicated and/or may be driven by non-ideal control, they may nevertheless exhibit simple dynamics approximately confined to a low-energy Hilbert subspace. Adiabatic elimination is the simplest approximation scheme allowing us to derive in certain cases an effective Hamiltonian operating in a low-dimensional Hilbert subspace. However, these approximations may present ambiguities and difficulties, hindering a systematic improvement of their accuracy in larger and larger systems. Here, we use the Magnus expansion as a systematic tool to derive ambiguity-free effective Hamiltonians. We show that the validity of the approximations ultimately leverages only on a proper coarse-graining in time of the exact dynamics. We validate the accuracy of the obtained effective Hamiltonians with suitably tailored fidelities of quantum operations.

DOI
10.3390/e25020234

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Quantum state processing is one of the main tools of quantum technologies. While real systems are complicated and/or may be driven by non-ideal control, they may nevertheless exhibit simple dynamics approximately confined to a low-energy Hilbert subspace. Adiabatic elimination is the simplest approximation scheme allowing us to derive in certain cases an effective Hamiltonian operating in a low-dimensional Hilbert subspace. However, these approximations may present ambiguities and difficulties, hindering a systematic improvement of their accuracy in larger and larger systems. Here, we use the Magnus expansion as a systematic tool to derive ambiguity-free effective Hamiltonians. We show that the validity of the approximations ultimately leverages only on a proper coarse-graining in time of the exact dynamics. We validate the accuracy of the obtained effective Hamiltonians with suitably tailored fidelities of quantum operations.
The Floquet-Magnus expansion is a widely used tool to derive effective descriptions of time-periodic quantum systems by approximating their dynamics with a time-independent Hamiltonian. However, its standard formulation is, strictly speaking, restricted to bounded Hamiltonians. In this work, we extend its definition and analysis to a broad class of time-periodic unbounded Hamiltonians. Our approach is based on an a priori distinct nonperturbative framework for the construction of effective Hamiltonians, which we show to reproduce the Floquet-Magnus expansion. A particular strength of our framework is that it allows us to prove that the resulting effective dynamics approximates the original time evolution propagators to arbitrary order in the high-frequency limit without requiring convergence of the Floquet-Magnus expansion, a condition that is already highly restrictive even in the bounded setting. We illustrate the scope of the method on representative models: the quantum Rabi Hamiltonian in the interaction picture, and the periodically driven quantum harmonic oscillator.
We derive a Magnus expansion for a frequency chirped quantum two-level system. We obtain a time-independent effective Hamiltonian which generates a stroboscopic time evolution. At lowest order the according dynamics is identical to results from using a rotating wave approximation. We determine, furthermore, also the next higher-order corrections within our expansion scheme in correspondence to the Bloch-Siegert shifts for harmonically driven systems. Importantly, our scheme can be extended to more complicated systems, i.e., even many-body systems.
Real-world experiments on quantum systems are always performed with measurement apparatus whose interaction times with the systems are finite. This restricts the observable quantum states to the space of time-coarse-grained density matrices ${\overline{\ensuremath{\rho}}(t)}$, providing motivation for the time-coarse-graining (TCG) approach that solves for $\overline{\ensuremath{\rho}}(t)$ without ever referring to the unobservable $\ensuremath{\rho}(t)$ of infinite time resolution. Phenomenologically, this implies that coherent transitions far outside the bandwidth would be filtered out, leaving only their effective impacts on the ``slow'' dynamics resolvable by the finite time resolution of the measurements. Therefore, the TCG framework provides rigorous justification for many existing effective Hamiltonian methods in the literature that aim at capturing the unitary part of the long-time dynamics. However, since time-coarse-graining is fundamentally irreversible, the resulting effective model allows for secular loss of information and dissipation of energy in general, which cannot be captured by any unitary effective models and has to be treated with explicit time-coarse-graining. Such incoherent effects are particularly prominent in driven nonlinear quantum systems where exchange of information and energy with the drive gives rise to incoherent effective dynamics at all finite time resolutions in general. While rigorous in principle, existing TCG methods in the literature can be applied only to simple systems by one iteratively solving superoperator equations at low orders in the coupling strengths. The complexity of such methods prevents systematic study of the time-coarse-grained dynamics and limits analytical results to the IR (low-resolution) limit in most cases. We address these limitations in this paper, presenting a systematic time-coarse-graining method that overcomes the complexities and restrictions of current techniques, offering a comprehensive and accurate modeling framework for driven nonlinear quantum systems. We derive closed-form formulas as well as diagrammatic representations for both unitary and nonunitary contributions, in the form of an effective Hamiltonian and nonunitary dissipators at arbitrary order in the coupling strengths, and complement this with a computer-algebra software package. We demonstrate the effectiveness of the method using several typical models of driven nonlinear systems in superconducting circuits, and show that it generalizes and improves on existing methods by providing more accurate results and explaining phenomena that have not been accounted for.
Many recent advancements in quantum computing leverage strong drives on nonlinear systems for state preparation, signal amplification, or gate operation. However, the interplay within such strongly driven system introduces multi-scale dynamics that affects the long-time behavior of the system in non-trivial ways that are very difficult to model. Therefore, the analysis of these systems often relies on effective Hamiltonian models that introduce additional nonlinear processes which approximate the long-time dynamics so that highly oscillatory terms may be ignored. However, the removal of such high frequency transitions can only be performed rigorously within a systematic framework of time-coarse graining, which is a fundamentally irreversible operation. This implies that standard approaches with unitary effective models cannot accurately capture the long-time behavior of strongly driven nonlinear quantum systems in general. We introduce a systematic perturbation theory for obtaining the complete non-unitary effective model of the time-coarse grained (TCG) dynamics of a driven quantum system to any order in the coupling strengths. We derive a closed-form analytical formula for both unitary and non-unitary contributions, in the form of an effective Hamiltonian and non-unitary (pseudo-)dissipators. Remarkably, even though the effective theory presumes unitary time evolution at the microscopic level, the time-coarse grained dynamics is found to follow a non-unitary time evolution in general. This occurs even when there is no open heat reservoir for the system to become entangled with or dissipate into. We demonstrate the effectiveness of the new method using several typical models of driven nonlinear systems in superconducting circuits, and show that it generalizes and improves on existing methods by providing more accurate results and explaining phenomena that have not been accounted for.
Various approaches have been used in the literature for eliminating nonresonant levels in atomic systems and deriving effective Hamiltonians. Important among these are elimination techniques at the level of probability amplitudes, operator techniques to project the dynamics on to the subspace of resonant levels, Green’s function techniques, the James’ effective Hamiltonian approach, etc. None of the previous approaches is suitable for deriving effective Hamiltonians in intracavity situations. However, the James’ approach does work in the case of only two-photon transitions in a cavity. A generalization of the James’ approach works in the case of three-photon transitions in a cavity, but only under Raman-like resonant conditions. Another important approach for adiabatic elimination is based on an adaptation of the Markov approximation well-known in the theory of system–bath interactions. However, this approach has not been shown to work in intracavity situations. In this paper, we present a method of adiabatic elimination for atoms inside cavities in the presence of multiphoton transitions. We work in the Heisenberg picture, and our approach has the advantage that it allows one to derive effective Hamiltonians even when Raman-like resonance conditions do not hold.