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arXiv:2211.08621

Direct comparison of two spin squeezed optical clocks below the quantum projection noise limit

John Martin Robinson, Maya Miklos, Yee Ming Tso, Colin J. Kennedy, Tobias Bothwell, Dhruv Kedar, James K. Thompson, Jun Ye

Published Nov 16, 2022• 5 citations
arXivHTMLPDF

Abstract

Building scalable quantum systems that demonstrate genuine performance enhancement based on entanglement is a major scientific goal for fields including computing, networking, simulations, and metrology. The tremendous challenge arises from the fragility of entanglement in increasingly larger sized quantum systems. Optical atomic clocks utilizing a large number of atoms have pushed the frontier of measurement science, building on precise engineering of quantum states and control of atomic interactions. However, today's state-of-the-art optical atomic clocks are limited by the quantum projection noise (QPN) defined by many uncorrelated atoms. Pioneering work on producing spin squeezed states of atoms has shown a path towards integrating entanglement into the best performing clocks. However, to directly demonstrate advantage of quantum entanglement in a working clock we must prevent backaction effects that degrade quantum coherence and introduce uncontrolled perturbations, as well as minimize the influence of technical noise arising from the interrogating clock laser. Here we present a new optical clock platform integrated with collective strong-coupling cavity QED for quantum non-demolition (QND) measurement. Optimizing the competition between spin measurement precision and loss of coherence, we measure a Wineland parameter of -1.8(7) dB for 1.9x10$^4$ atoms, thus verifying the presence of entanglement. Furthermore, a moving lattice allows the cavity to individually address two independent sub-ensembles, enabling us to spin squeeze two clock ensembles successively and compare their performance. This differential comparison between the two squeezed clocks directly verifies enhanced clock stability of 2.0(3) dB below QPN, and 0.6(3) dB above the standard quantum limit (SQL), at the measurement precision level of 10$^{-17}$, without subtracting any technical noise contributions.

DOI
10.48550/arxiv.2211.08621

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Optical atomic clocks with unrivaled precision and accuracy have advanced the frontier of precision measurement science and opened new avenues for exploring fundamental physics. A fundamental limitation on clock precision is the standard quantum limit (SQL), which stems from the uncorrelated projection noise of each atom. State-of-the-art optical lattice clocks interrogate large ensembles to minimize the SQL, but density-dependent frequency shifts pose challenges to scaling the atom number. The SQL can be surpassed, however, by leveraging entanglement, though it remains an open problem to achieve quantum advantage from spin squeezing at state-of-the-art stability levels. Here, we demonstrate clock performance beyond the SQL, achieving a fractional frequency precision of 1.1×10^{-18} for a single spin-squeezed clock. With cavity-based quantum nondemolition measurements, we prepare two spin-squeezed ensembles of ∼30 000 strontium atoms confined in a two-dimensional optical lattice. A synchronous clock comparison with an interrogation time of 61 ms achieves a metrological improvement of 2.0(2) dB beyond the SQL, after correcting for state preparation and measurement errors. These results establish the most precise entanglement-enhanced clock to date and offer a powerful platform for exploring the interplay of gravity and quantum entanglement.
Large ensembles of uncorrelated atoms are extensively used as precise sensors of time, rotation, and gravity, and for tests of fundamental physics. The quantum nature of the sensors imposes a limit on their ultimate precision. Larger ensembles of N atoms can be used to average the quantum noise as 1/√N, a scaling known as the standard quantum limit. However, the ensemble size may be limited by technical constraints and/or atom-atom collisions -- a fundamental distinction from photon-based sensors. Learning to prepare entangled states of large ensembles with noise properties below the standard quantum limit will be key to extending both the precision and/or bandwidth of atomic sensors. More broadly, the generation and application of entanglement to solve problems is a core goal of quantum information science being pursued in both atomic and solid state systems.\nIn this thesis, we utilize the tools of cavity-QED to prepare entangled spin-squeezed states with 3.4(6) dB improvement in spectroscopic sensitivity over the standard quantum limit. The collective atomic spin is composed of the two-level clock states of 87Rb confined in a medium finesse F = 710 optical cavity. We employ cavity-aided quantum non-demolition measurements of the vacuum Rabi splitting to measure and subtract out the quantum projection noise of the collective spin state, preparing states with collective atomic spin projection noise 4.9(6) dB below the projection noise level. The conditionally reduced spin noise combined with the measured 1.5(3) dB reduction in the mean spin length implies a net 3.4(6) dB spectroscopic enhancement or conditional squeezing as defined by the Wineland criterion. Our method does not require single particle addressability and is applied to a spectroscopically large ensemble of N = 7 x 105 atoms using two collective population measurements, with the whole squeezing operation taking ~ 150 μs. The gain in sensitivity is spectroscopically equivalent to the enhancement obtained had we created > 105 pairs of maximally entangled qubits, demonstrating the power of a top-down approach for entangling large ensembles. The nondemolition probing of atomic populations via the vacuum Rabi splitting is also of broad interest for non-destructively reading out a wide variety of both atomic and solid state qubits.
Quantum projection noise will soon limit the best achievable precision of optical atomic clocks based on lattice-confined neutral atoms. Squeezing the collective atomic pseudo-spin via measurement of the clock state populations during Ramsey interrogation suppresses the projection noise. We show here that the lattice laser field can be used to perform ideal quantum non-demolition measurements without clock shifts or decoherence and explore the feasibility of such an approach in theory with the lattice field confined in a ring-resonator. Detection of the motional sideband due to the atomic vibration in the lattice wells can yield signal sizes a hundredfold above the projection noise limit.
Atomic clocks have reached the Standard Quantum Limit (SQL) of precision,1 set by the projection noise inherent in measurements on uncorrelated atoms. It is possible to overcome this limit by entangling the atoms to generate a "squeezed state" of the atomic ensemble. We use the collective interaction of an atomic ensemble with a far-detuned light field in an optical resonator to prepare squeezed states by two different methods: quantum non-demolition (QND) measurement and Hamiltonian evolution. We apply both methods to an ensemble of 5 x 104 87Rb atoms in a superposition of hyperfine clock states. We measure the suppression of projection noise and compare it to the accompanying reduction in signal, thereby quantifying the net gain in spectroscopic sensitivity. By QND measurement, with resolution up to 9 dB below the projection noise level, we achieve 3.0(8) dB of metrologically relevant squeezing. Whereas the measurement-based approach relies on knowledge of the (randomly distributed) measurement outcome to produce a conditionally squeezed state, the method of Hamiltonian evolution produces a known squeezed state independent of detector performance. We mimic the dynamics of the one-axis twisting Hamiltonian, proposed as a generator of squeezed states by Kitagawa and Ueda,2 by using the atom-induced frequency shift of the resonator mode and the corresponding resonator-field-induced shift of the atomic transition frequency to introduce an effective interaction among the atoms. The resulting deterministic squeezing is sufficient to allow a 6.0(4) dB improvement in spectroscopic sensitivity over the SQL.
Many-body entangled states allow precision measurement beyond the standard quantum limit. Yet they have not been effectively exploited in optical lattice clocks except for proof-of-principle demonstrations. Under the current experimental conditions, taking into account the lattice perturbation, atom-atom interactions, and local oscillator noise, we theoretically evaluate the performance of spin-squeezing-based shallow-lattice Yb optical clocks. The numerical simulation shows that the stability of differential frequency comparison between two Yb ensembles in squeezed spin states potentially accesses the ${10}^{\ensuremath{-}19}$ level at the averaging time of 1 s. The resultant Wineland parameter may be as low as ${\ensuremath{\xi}}_{\text{W}}^{2}=0.027$, corresponding to a reduction of averaging time by a factor of 37, and is limited by the collision-induced degradation of spin squeezing. The metrological gain provided by spin squeezing opens up new opportunities for precision measurement and fundamental physics.
Abstract Optical lattice clocks are the world's most accurate and stable timepieces. Thus far, the differential clock comparison has reached a stability limited by the quantum projection noise of uncorrelated atoms. Overcoming this limit relies on using spin squeezing, where quantum fluctuations of the collective spin undergo a strong suppression in one direction while being enhanced in the conjugation direction. The recent differential comparison of spin‐squeezed clocks mainly employs multiple atomic clouds or sub‐ensembles within one cloud, complicating the clock operation. Here, it is numerically investigated the differential comparison of conditionally and unconditionally spin‐squeezed states of one lattice‐trapped cloud of neutral atoms. The simulation results in a comparison stability of at the averaging time for atoms. The metrological gain reaches dB, primarily limited by the decoherence induced by quantum jumps of intracavity probe photons during quantum non‐demolition measurements. Besides the quantum precision enhancement, our scheme paves the way to using one spin squeezing protocol to appraise the other.