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arXiv:2211.00653 · Communications Physics

Trimer quantum spin liquid in a honeycomb array of Rydberg atoms

Milan Kornjača, Rhine Samajdar, Tommaso Macrì, Nathan Gemelke, Sheng-Tao Wang, Fangli Liu

Published Dec 13, 2023• 19 citations
arXivHTMLPDF

Abstract

Abstract Quantum spin liquids are elusive but paradigmatic examples of strongly correlated quantum states that are characterized by long-range quantum entanglement. Recently, signatures of a gapped topological $${{\mathbb{Z}}}_{2}$$ Z 2 spin liquid have been observed in a system of Rydberg atoms; however, the full capability of these platforms to realize quantum spin liquids extends far beyond this state alone. Here, we propose the realization of a different class of spin liquids in a honeycomb array of Rydberg atoms. Exploring the system’s quantum phase diagram using density-matrix renormalization group and exact diagonalization calculations, we identify several density-wave-ordered phases and a trimer spin liquid ground state with an emergent U(1) × U(1) local symmetry. This liquid state originates from superpositions of classical trimer configurations on the dual triangular lattice in the regime where third-nearest-neighbor atoms lie within the Rydberg blockade radius. Finally, we discuss the conditions to enhance the preparation fidelity of this state by a general Rydberg-blockade-based projection mechanism, test the robustness of the trimer spin liquid phase in a range of realistic parameters, and outline methods for its experimental detection.

DOI
10.1038/s42005-023-01470-z

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Abstract Quantum spin liquids are elusive but paradigmatic examples of strongly correlated quantum states that are characterized by long-range quantum entanglement. Recently, signatures of a gapped topological Z2{{\mathbb{Z}}}_{2}Z2​ Z 2 spin liquid have been observed in a system of Rydberg atoms; however, the full capability of these platforms to realize quantum spin liquids extends far beyond this state alone. Here, we propose the realization of a different class of spin liquids in a honeycomb array of Rydberg atoms. Exploring the system’s quantum phase diagram using density-matrix renormalization group and exact diagonalization calculations, we identify several density-wave-ordered phases and a trimer spin liquid ground state with an emergent U(1) × U(1) local symmetry. This liquid state originates from superpositions of classical trimer configurations on the dual triangular lattice in the regime where third-nearest-neighbor atoms lie within the Rydberg blockade radius. Finally, we discuss the conditions to enhance the preparation fidelity of this state by a general Rydberg-blockade-based projection mechanism, test the robustness of the trimer spin liquid phase in a range of realistic parameters, and outline methods for its experimental detection.
Trimers are defined as two adjacent edges on a graph. We study the quantum states obtained as equal-weight superpositions of all trimer coverings of a lattice, with the constraint of having a trimer on each vertex: the so-called trimer resonating-valence-bond (tRVB) states. Exploiting their tensor network representation, we show that these states can host Z3{\mathbb{Z}}_{3}Z3​ topological order or can be gapless liquids with $\mathrm{U}(1)\ifmmode\times\else\texttimes\fi{}\mathrm{U}(1)$ local symmetry. We prove that this continuous symmetry emerges whenever the lattice can be tripartite such that each trimer covers all the three sublattices. In the gapped case, we demonstrate the stability of topological order against dilution of maximal trimer coverings, which is relevant for realistic models where the density of trimers can fluctuate. Furthermore, we clarify the connection between gapped tRVB states and Z3{\mathbb{Z}}_{3}Z3​ lattice gauge theories by smoothly connecting the former to the Z3{\mathbb{Z}}_{3}Z3​ toric code, and discuss the nonlocal excitations on top of tRVB states. Finally, we analyze via exact diagonalization the zero-temperature phase diagram of a diluted trimer model on the square lattice and demonstrate that the ground state exhibits topological properties in a narrow region in parameter space. We show that a similar model can be implemented in Rydberg atom arrays exploiting the blockade effect. We investigate dynamical preparation schemes in this setup and provide a viable route for probing experimentally Z3{\mathbb{Z}}_{3}Z3​ quantum spin liquids.
We show that the nonlinear transport of bosonic excitations in a two-dimensional honeycomb lattice of spin-orbit-coupled Rydberg atoms gives rise to disordered quantum phases which are topological and may be candidates for quantum spin liquids. As recently demonstrated by Lienhard et al. [Phys. Rev. X 10, 021031 (2020)] the spin-orbit coupling breaks time-reversal and chiral symmetries and leads to a tunable density-dependent complex hopping of spin excitations which behave as hard-core bosons. Using exact diagonalization (ED), we numerically investigate the phase diagram resulting from the competition between density-dependent and direct transport terms as well as density-density interactions. In mean-field approximation there is a phase transition from a condensate to a ${120}^{\ensuremath{\circ}}$ phase when the amplitude of the complex hopping exceeds that of the direct one. In the full model a new phase emerges close to the mean-field critical point as a result of quantum correlations induced by the density dependence of the complex hopping. We show that without density-density interactions this phase is a genuine disordered one, has large spin chirality, and is characterized by a nontrivial many-body Chern number. The Chern number is found to be robust to disorder. ED simulations of small lattices with up to 30 lattice sites give indications for a nondegenerate ground state with finite spin and collective gaps and thus for a bosonic integer quantum Hall phase, protected by U(1)\mathrm{U}(1)U(1) symmetry. On the other hand, while staying finite, the many-body gap varies substantially when different twisted boundary conditions are applied, which points to a gapless phase. For very strong negative nonlinear hopping amplitudes we find another disordered regime with vanishing spin gap. This phase also has a large spin chirality and could be a gapless spin liquid but lies outside the parameter regime experimentally accessible in the Rydberg system.
Quantum phases with topological order, such as quantum spin liquids, have been the focus of explorations for several decades. Such phases feature a number of remarkable properties including long-range quantum entanglement. Moreover, they can be potentially exploited for the realization of robust quantum computation, as exemplified by the paradigmatic toric code model. While some indications that such phases may be present in frustrated condensed matter systems have been previously reported, so far quantum spin liquids have eluded direct experimental detection. In this talk, I will show how a programmable quantum simulator based on Rydberg atom arrays can be used to realize and probe quantum spin liquid states. In our approach, atoms are placed on the links of a kagome lattice and coherent evolution under Rydberg blockade enables the transition into frustrated quantum states with no local order. We detect the onset of a quantum spin liquid phase of the toric code type by measuring topological string operators in two complementary bases. The properties of this state are further revealed using a lattice with non-trivial topology, representing a step towards the realization of a topological qubit. Our observations open the door to the controlled experimental exploration of topological quantum matter, and could enable the investigation of new methods for topologically protected quantum information processing.
We investigate the nature of quantum phases arising in chiral interacting Hamiltonians recently realized in Rydberg atom arrays. We classify all possible fermionic chiral spin liquids with U(1)\mathrm{U}(1)U(1) global symmetry using parton construction on the honeycomb lattice. The resulting classification includes six distinct classes of gapped quantum spin liquids: the corresponding variational wavefunctions obtained from two of these classes accurately describe the Rydberg many-body ground state at 1/21/21/2 and 1/41/41/4 particle density. Complementing this analysis with tensor network simulations, we conclude that both particle filling sectors host a spin liquid with the same topological order of a $\ensuremath{\nu}\phantom{\rule{0.16em}{0ex}}=\phantom{\rule{0.16em}{0ex}}1/2$ fractional quantum Hall effect. At density 1/21/21/2, our results clarify the phase diagram of the model, while at density 1/41/41/4, they provide an explicit construction of the ground-state wavefunction with almost unit overlap with the microscopic one. These findings pave the way to the use of parton wavefunctions to guide the discovery of quantum spin liquids in chiral Rydberg models.
Quantum spin liquids, exotic phases of matter with topological order, have been a major focus in physics for the past several decades. Such phases feature long-range quantum entanglement that can potentially be exploited to realize robust quantum computation. We used a 219-atom programmable quantum simulator to probe quantum spin liquid states. In our approach, arrays of atoms were placed on the links of a kagome lattice, and evolution under Rydberg blockade created frustrated quantum states with no local order. The onset of a quantum spin liquid phase of the paradigmatic toric code type was detected by using topological string operators that provide direct signatures of topological order and quantum correlations. Our observations enable the controlled experimental exploration of topological matter and protected quantum information processing.
Rydberg atom arrays have recently emerged to be a promising platform for the exploration of exotic quantum phases of matter and quantum phenomena. In this work, we map out the ground-state phase diagram of Rydberg atoms on a honeycomb lattice as a function of the Rydberg blockade radius and the laser detuning by performing large-scale finite-size density matrix renormalization group simulations. Apart from a featureless disordered phase, we find five other intricate long-range density-wave-ordered phases within a relatively wide parameter space. The properties of these quantum phases are analyzed by calculating their Rydberg excitation profiles and static structure factors. In addition, a continuous quantum phase transition belonging to the (2+1)-dimensional Ising universality class is explored by a standard finite-size scaling analysis. Our work implies some different physics, such as the possible nontrivial quantum phase transitions and a highly degenerate string ordered phase, that a honeycomb geometry could bring to the Rydberg system and serves as a numerical guide for possible real experiments.